=== Generating (published_papers) ===
=== Generating (research_interests) ===
=== Generating (education) ===
=== Generating (research_experience) ===
=== Generating (misc) ===
=== Generating (research_projects) ===
=== Generating (books_etc) ===
=== Generating (industrial_property_rights) ===
=== Generating (awards) ===
=== Generating (association_memberships) ===
=== Generating (teaching_experience) ===
=== Generating (committee_memberships) ===
=== Generating (presentations) ===
==== begin registerFile(/WWW/pub2/data/ERD/person/10694/researchmap/published_papers.jsonl) ====
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line:82, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=144482","label":"url"}],"paper_title":{"en":"Effect of components in electrodes on sintering characteristics of Ce0.9Gd0.1O1.95 electrolyte in intermediate-temperature solid oxide fuel cells during fabrication","ja":"Effect of components in electrodes on sintering characteristics of Ce0.9Gd0.1O1.95 electrolyte in intermediate-temperature solid oxide fuel cells during fabrication"},"authors":{"en":[{"name":"Mori Masashi"},{"name":"Suda Eisaku"},{"name":"Pacaud Bernard"},{"name":"Murai Kei-ichiro"},{"name":"Moriga Toshihiro"}],"ja":[{"name":"森 昌史"},{"name":"須田 栄作"},{"name":"パコー バーナード"},{"name":"村井 啓一郎"},{"name":"森賀 俊広"}]},"publication_date":"2006-07-03","publication_name":{"en":"Journal of Power Sources","ja":"Journal of Power Sources"},"volume":"Vol.157","number":"No.2","starting_page":"688","ending_page":"694","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1016/j.jpowsour.2006.01.062"],"issn":["0378-7753"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:83, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=140528","label":"url"}],"paper_title":{"en":"7Li-NMR study on Li+ ionic diffusion and phase transition in LixCoO2","ja":"7Li-NMR study on Li+ ionic diffusion and phase transition in LixCoO2"},"authors":{"en":[{"name":"Nakamura Koichi"},{"name":"Ohno, Hideki"},{"name":"Okamura, Kazuhiro"},{"name":"Michihiro Yoshitaka"},{"name":"Moriga Toshihiro"},{"name":"Nakabayashi Ichiro"},{"name":"Kanashiro Tatsuo"}],"ja":[{"name":"中村 浩一"},{"name":"Ohno, Hideki"},{"name":"Okamura, Kazuhiro"},{"name":"道廣 嘉隆"},{"name":"森賀 俊広"},{"name":"中林 一朗"},{"name":"金城 辰夫"}]},"publication_date":"2006-03","publication_name":{"en":"Solid State Ionics","ja":"Solid State Ionics"},"volume":"Vol.177","number":"No.9-10","starting_page":"821","ending_page":"826","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1016/j.ssi.2006.02.021"],"issn":["0167-2738"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:84, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"http://ci.nii.ac.jp/naid/110002548561/","label":"url"},{"@id":"https://cir.nii.ac.jp/crid/1390001205276966912/","label":"url"},{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-31144440664&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=135482","label":"url"}],"paper_title":{"en":"Development of Mass Production of Ce0.9Gd0.1O1.95 Nanopowder with High-Sintering Characteristics","ja":"易焼結性Ce0.9Gd0.1O1.95ナノ粒子の量産技術の開発"},"authors":{"en":[{"name":"Suda Eisaku"},{"name":"Mori Masashi"},{"name":"Murai Kei-ichiro"},{"name":"Pacaud Bernard"},{"name":"Moriga Toshihiro"}],"ja":[{"name":"須田 栄作"},{"name":"森 昌史"},{"name":"村井 啓一郎"},{"name":"バーナード パコー"},{"name":"森賀 俊広"}]},"description":{"en":"The mass production process of Ce_<0.9>Gd_<0.1>O_<1.95>(CGO) nanopowder with high-sintering characteristics has been studied. Although CGO powders were fabricated using a large scale coprecipitation bath with a capacity of 65kg/batch, particle size distribution curve of this powder showed two peaks for the agglomeration and this powder showed lower sintering characteristics, compared to the CGO nanopowder by a small scale bath with a capacity of 0.1kg/batch. It was found that when the impurity of NO_3^- in the powder was removed by water using the rate of 50L/kg, the formation of oval shape particles was observed and it is easy to crush the agglomerations in the powder by hammer-type mill. The sintering characteristics of this powder are almost same to those of the powder synthesized by the small scale bath.","ja":"The mass production process of Ce_<0.9>Gd_<0.1>O_<1.95>(CGO) nanopowder with high-sintering characteristics has been studied. Although CGO powders were fabricated using a large scale coprecipitation bath with a capacity of 65kg/batch, particle size distribution curve of this powder showed two peaks for the agglomeration and this powder showed lower sintering characteristics, compared to the CGO nanopowder by a small scale bath with a capacity of 0.1kg/batch. It was found that when the impurity of NO_3^- in the powder was removed by water using the rate of 50L/kg, the formation of oval shape particles was observed and it is easy to crush the agglomerations in the powder by hammer-type mill. The sintering characteristics of this powder are almost same to those of the powder synthesized by the small scale bath."},"publication_date":"2005-12-01","publication_name":{"en":"Journal of Ceramic Society of Japan","ja":"日本セラミックス協会学術論文誌"},"volume":"Vol.113","number":"No.1324","starting_page":"793","ending_page":"798","languages":["jpn"],"referee":true,"identifiers":{"doi":["10.2109/jcersj.113.793"],"issn":["0914-5400"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:85, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=115466","label":"url"}],"paper_title":{"en":"Effects of introduction of argon on structural and transparent conducting properties of ZnO-In2O3 thin films prepared by pulsed laser deposition","ja":"Effects of introduction of argon on structural and transparent conducting properties of ZnO-In2O3 thin films prepared by pulsed laser deposition"},"authors":{"en":[{"name":"Moriga Toshihiro"},{"name":"Mikawa Michio"},{"name":"Sakakibara Yuji"},{"name":"Misaki Yukinori"},{"name":"Murai Kei-ichiro"},{"name":"Nakabayashi Ichiro"},{"name":"Tominaga Kikuo"}],"ja":[{"name":"森賀 俊広"},{"name":"三河 通男"},{"name":"榊原 友士"},{"name":"三崎 幸典"},{"name":"村井 啓一郎"},{"name":"中林 一朗"},{"name":"富永 喜久雄"}]},"description":{"en":"パルスレーザー蒸着法により酸化亜鉛-酸化インジウム透明導電膜を作製した．蒸着中にArガスをO2ガスとともに導入することにより，アモルファス相が現れる領域が広くなることが明らかになった．また，膜表面の平滑性が格段に向上することを示した．","ja":"パルスレーザー蒸着法により酸化亜鉛-酸化インジウム透明導電膜を作製した．蒸着中にArガスをO2ガスとともに導入することにより，アモルファス相が現れる領域が広くなることが明らかになった．また，膜表面の平滑性が格段に向上することを示した．"},"publication_date":"2005-08-22","publication_name":{"en":"Thin Solid Films","ja":"Thin Solid Films"},"volume":"Vol.486","number":"No.1","starting_page":"53","ending_page":"57","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1016/j.tsf.2004.11.241"],"issn":["0040-6090"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:86, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"http://ci.nii.ac.jp/naid/130000065952/","label":"url"},{"@id":"https://cir.nii.ac.jp/crid/1390282680167790848/","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=122446","label":"url"}],"paper_title":{"en":"Catalytic Activity of Iron Oxides Supported on γ-Al2O3 for Methane Oxidation","ja":"Catalytic Activity of Iron Oxides Supported on γ-Al2O3 for Methane Oxidation"},"authors":{"en":[{"name":"Tanaka Suminori"},{"name":"Nakagawa Kazunori"},{"name":"Kanezaki Eiji"},{"name":"Katoh Masahiro"},{"name":"Murai Kei-ichiro"},{"name":"Moriga Toshihiro"},{"name":"Nakabayashi Ichiro"},{"name":"Sugiyama Shigeru"},{"name":"Kidoguchi Yoshiyuki"},{"name":"Miwa Kei"}],"ja":[{"name":"田中 住典"},{"name":"中川 和憲"},{"name":"金崎 英二"},{"name":"加藤 雅裕"},{"name":"村井 啓一郎"},{"name":"森賀 俊広"},{"name":"中林 一朗"},{"name":"杉山 茂"},{"name":"木戸口 善行"},{"name":"三輪 惠"}]},"description":{"en":"Three kinds of catalysts of goethites supported on γ-Al2O3 (Fe/γ-Al2O3), SiO2-Al2O3 (Fe/SiO2-Al2O3) and SiO2 (Fe/SiO2) were investigated in terms of the catalytic activity of methane oxidation. The specific surface areas of these catalysts were larger in common than the area of goethite with no supports. The Fe/γ-Al2O3 catalyst has the highest performance in the low-temperature activity of methane oxidation which started at 623 K and completed at 923 K. When the Fe-content in Fe/γ-Al2O3 was increased, the formation of goethite was observed by the X-ray analyses and the activity of this catalyst increased up to 6 mol%. After the catalytic methane oxidation at 823 K, it was observed that goethite in Fe/γ-Al2O3 transformed to hematite which has been known as an active iron oxide in methane oxidation. The activity of Fe/γ-Al2O3 was enhanced by the addition of sodium up to the Na-content of 5 mol% although it descended above the content due to the decrease of the specific surface area of the catalyst.","ja":"Three kinds of catalysts of goethites supported on γ-Al2O3 (Fe/γ-Al2O3), SiO2-Al2O3 (Fe/SiO2-Al2O3) and SiO2 (Fe/SiO2) were investigated in terms of the catalytic activity of methane oxidation. The specific surface areas of these catalysts were larger in common than the area of goethite with no supports. The Fe/γ-Al2O3 catalyst has the highest performance in the low-temperature activity of methane oxidation which started at 623 K and completed at 923 K. When the Fe-content in Fe/γ-Al2O3 was increased, the formation of goethite was observed by the X-ray analyses and the activity of this catalyst increased up to 6 mol%. After the catalytic methane oxidation at 823 K, it was observed that goethite in Fe/γ-Al2O3 transformed to hematite which has been known as an active iron oxide in methane oxidation. The activity of Fe/γ-Al2O3 was enhanced by the addition of sodium up to the Na-content of 5 mol% although it descended above the content due to the decrease of the specific surface area of the catalyst."},"publication_date":"2005-07","publication_name":{"en":"Journal of the Japan Petroleum Institute","ja":"Journal of the Japan Petroleum Institute"},"volume":"Vol.48","number":"No.4","starting_page":"223","ending_page":"228","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1627/jpi.48.223"],"issn":["1346-8804"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:87, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=118804","label":"url"}],"paper_title":{"en":"Characterization of ZnO-In2O3 transparent conducting films by pulsed laser deposition","ja":"Characterization of ZnO-In2O3 transparent conducting films by pulsed laser deposition"},"authors":{"en":[{"name":"Mikawa Michio"},{"name":"Moriga Toshihiro"},{"name":"Sakakibara Yuji"},{"name":"Misaki Yukinori"},{"name":"Murai Kei-ichiro"},{"name":"Nakabayashi Ichiro"},{"name":"Tominaga Kikuo"}],"ja":[{"name":"三河 通男"},{"name":"森賀 俊広"},{"name":"榊原 友士"},{"name":"三崎 幸典"},{"name":"村井 啓一郎"},{"name":"中林 一朗"},{"name":"富永 喜久雄"}]},"description":{"en":"パルスレーザー蒸着法により酸化亜鉛-酸化インジウム透明導電膜を作製した．蒸着中にO2ガスとともに導入することにより，可視光領域の透明性を確保することが可能となった．酸化インジウム相からアモルファス相に移行する組成[Zn]/([Zn]+[In])=0.2∼0.3付近で最小抵抗値を示すことが明らかとなった．","ja":"パルスレーザー蒸着法により酸化亜鉛-酸化インジウム透明導電膜を作製した．蒸着中にO2ガスとともに導入することにより，可視光領域の透明性を確保することが可能となった．酸化インジウム相からアモルファス相に移行する組成[Zn]/([Zn]+[In])=0.2∼0.3付近で最小抵抗値を示すことが明らかとなった．"},"publication_date":"2005-06-15","publication_name":{"en":"Materials Research Bulletin","ja":"Materials Research Bulletin"},"volume":"Vol.40","number":"No.6","starting_page":"1052","ending_page":"1058","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1016/j.materresbull.2005.02.019"],"issn":["0025-5408"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:88, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"http://ci.nii.ac.jp/naid/150000045181/","label":"url"},{"@id":"https://cir.nii.ac.jp/crid/1390001206266720896/","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=24766","label":"url"}],"paper_title":{"en":"Phonon Echo Study on Lithium Ionic Diffusion in LiNbO3 Powder","ja":"Phonon Echo Study on Lithium Ionic Diffusion in LiNbO3 Powder"},"authors":{"en":[{"name":"Nakamura Koichi"},{"name":"Michihiro Yoshitaka"},{"name":"Fumiaki Katayama"},{"name":"Moriga Toshihiro"},{"name":"Mahbubar Md."},{"name":"Nakabayashi Ichiro"},{"name":"Kanashiro Tatsuo"}],"ja":[{"name":"中村 浩一"},{"name":"道廣 嘉隆"},{"name":"片山 史章"},{"name":"森賀 俊広"},{"name":"マハブバル モハマド"},{"name":"中林 一朗"},{"name":"金城 辰夫"}]},"description":{"en":"Two-pulse phonon echo measurements were performed from room temperature to 900 K in micro particles of polycrystalline and single crystalline LiNbO3 to investigate the relationship between lithium ionic diffusion and decay time, $T_{2}$, in a phonon echo study. Decay time was dependent on temperature, showing a rapid decrease above 800 K in the polycrystalline sample. The origin of this anomaly is interpreted in terms of a simple Debye-type relaxation due to lithium ionic diffusion. The activation energy, which was evaluated as 0.93 eV in the polycrystalline samples, was comparable with reported values from ionic conductivity and NMR studies. On the other hand, single crystalline LiNbO3 showed no signs of lithium ionic diffusion up to 900 K. The contribution to $T_{2}$ from lithium ionic diffusion would be dominant at higher temperatures than 900 K because of the much higher activation energy in a single crystalline sample. It is shown that phonon echo decay time is strongly connected with ionic diffusion in the particles.","ja":"Two-pulse phonon echo measurements were performed from room temperature to 900 K in micro particles of polycrystalline and single crystalline LiNbO3 to investigate the relationship between lithium ionic diffusion and decay time, $T_{2}$, in a phonon echo study. Decay time was dependent on temperature, showing a rapid decrease above 800 K in the polycrystalline sample. The origin of this anomaly is interpreted in terms of a simple Debye-type relaxation due to lithium ionic diffusion. The activation energy, which was evaluated as 0.93 eV in the polycrystalline samples, was comparable with reported values from ionic conductivity and NMR studies. On the other hand, single crystalline LiNbO3 showed no signs of lithium ionic diffusion up to 900 K. The contribution to $T_{2}$ from lithium ionic diffusion would be dominant at higher temperatures than 900 K because of the much higher activation energy in a single crystalline sample. It is shown that phonon echo decay time is strongly connected with ionic diffusion in the particles."},"publication_date":"2005-06-10","publication_name":{"en":"Japanese Journal of Applied Physics, Part 1 (Regular Papers & Short Notes)","ja":"Japanese Journal of Applied Physics, Part 1 (Regular Papers & Short Notes)"},"volume":"Vol.44","number":"No.6A","starting_page":"4043","ending_page":"4046","referee":true,"identifiers":{"doi":["10.1143/JJAP.44.4043"],"issn":["0021-4922"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:89, {"insert":{"user_id":"1000038966","type":"published_papers","id":"30376434"},"force":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=122257","label":"url"}],"paper_title":{"en":"Sunthesis of Divalent metalNitrides Zn3N2 and Mg3N2 and Enhancement of Their Bandgap by Insertuin of Lithium","ja":"Sunthesis of Divalent metalNitrides Zn3N2 and Mg3N2 and Enhancement of Their Bandgap by Insertuin of Lithium"},"authors":{"en":[{"name":"Moriga Toshihiro"},{"name":"Takahara Keiko"},{"name":"Saki Ryoji"},{"name":"Sakamoto Takashi"},{"name":"Murai Kei-ichiro"},{"name":"Nakabayashi Ichiro"}],"ja":[{"name":"森賀 俊広"},{"name":"高原 恵子"},{"name":"﨑 亮二"},{"name":"坂本 考史"},{"name":"村井 啓一郎"},{"name":"中林 一朗"}]},"publication_date":"2005-06","publication_name":{"en":"Processing and Fabrication of Advanced Materials XIII","ja":"Processing and Fabrication of Advanced Materials XIII"},"volume":"Vol.1","starting_page":"496","ending_page":"507","languages":["eng"],"referee":true,"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:90, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=116249","label":"url"}],"paper_title":{"en":"Amorphous Transparent Conductive Oxide Films of In2O3-ZnO with Additional Al2O3 Impurities","ja":"Amorphous Transparent Conductive Oxide Films of In2O3-ZnO with Additional Al2O3 Impurities"},"authors":{"en":[{"name":"Tominaga Kikuo"},{"name":"Fukumoto Hidenori"},{"name":"Kondo Kumiko"},{"name":"Hayashi Yukako"},{"name":"Murai Kei-ichiro"},{"name":"Moriga Toshihiro"},{"name":"Nakabayashi Ichiro"}],"ja":[{"name":"富永 喜久雄"},{"name":"Fukumoto Hidenori"},{"name":"Kondo Kumiko"},{"name":"林 由佳子"},{"name":"村井 啓一郎"},{"name":"森賀 俊広"},{"name":"中林 一朗"}]},"description":{"en":"ZnO-In2O3系透明導電膜にAl2O3を不純物として添加することで，新材料を開発し，この系の電気的特性，光学的特性について調べた．Zn/(Zn+In)の組成比を変えていくと，アモルファス相とホモロガス(結晶)相が現れた．これらの電気伝導メカニズムについて検討した．さらに，Al2O3の添加の効果が，Al2O3を添加しないZnO-In2O3アモルファス膜と比較して，電気伝導性を損なわずに光学的バンドギャップを広げる効果があることを発見した．また，アモルファス膜は表面が平坦であることも示した．これらのことは，透明電極への応用において意義のある発見である．というのは，これらの特長は青色や紫外用デバイスでの透明電極の応用にマッチした特性である．また，低温基板上にも作製できる点で，有機基板上への透明電極作製の展望が開けた．","ja":"ZnO-In2O3系透明導電膜にAl2O3を不純物として添加することで，新材料を開発し，この系の電気的特性，光学的特性について調べた．Zn/(Zn+In)の組成比を変えていくと，アモルファス相とホモロガス(結晶)相が現れた．これらの電気伝導メカニズムについて検討した．さらに，Al2O3の添加の効果が，Al2O3を添加しないZnO-In2O3アモルファス膜と比較して，電気伝導性を損なわずに光学的バンドギャップを広げる効果があることを発見した．また，アモルファス膜は表面が平坦であることも示した．これらのことは，透明電極への応用において意義のある発見である．というのは，これらの特長は青色や紫外用デバイスでの透明電極の応用にマッチした特性である．また，低温基板上にも作製できる点で，有機基板上への透明電極作製の展望が開けた．"},"publication_date":"2005-05","publication_name":{"en":"Journal of Vacuum Science & Technology A","ja":"Journal of Vacuum Science & Technology A"},"volume":"Vol.23","number":"No.3","starting_page":"401","ending_page":"407","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1116/1.1874172"],"issn":["0734-2101"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:91, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=82990","label":"url"}],"paper_title":{"en":"Zinc Oxynitride Powders Examined by X-ray Absorption Near Edge Spectroscopy","ja":"Zinc Oxynitride Powders Examined by X-ray Absorption Near Edge Spectroscopy"},"authors":{"en":[{"name":"Moriga Toshihiro"},{"name":"Sakamoto Takashi"},{"name":"Saki Ryoji"},{"name":"Murai Kei-ichiro"},{"name":"Nakabayashi Ichiro"},{"name":"Metson James -B."}],"ja":[{"name":"森賀 俊広"},{"name":"坂本 考史"},{"name":"崎 亮二"},{"name":"村井 啓一郎"},{"name":"中林 一朗"},{"name":"Metson James -B."}]},"description":{"en":"電子転換収率法と蛍光法を用いて，含有酸素量·窒素量の異なる酸窒化亜鉛のXANESスペクトルを測定した．表面に敏感な電子転換収率法とバルクの情報に近い蛍光法では酸窒化亜鉛の窒素K吸収端近傍のXANESスペクトルに違いが見られ，作製した酸窒化亜鉛の酸素は，その粒子の表面近傍に編析していることを示した．","ja":"電子転換収率法と蛍光法を用いて，含有酸素量·窒素量の異なる酸窒化亜鉛のXANESスペクトルを測定した．表面に敏感な電子転換収率法とバルクの情報に近い蛍光法では酸窒化亜鉛の窒素K吸収端近傍のXANESスペクトルに違いが見られ，作製した酸窒化亜鉛の酸素は，その粒子の表面近傍に編析していることを示した．"},"publication_date":"2005-03","publication_name":{"en":"Physica Scripta","ja":"Physica Scripta"},"volume":"Vol.T115","starting_page":"312","ending_page":"313","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1238/Physica.Topical.115a00312"],"issn":["0031-8949"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:92, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=130709","label":"url"}],"paper_title":{"en":"XAFS and XRD Studies of PdO-CeO2 Catalysts on χ-Al2O3","ja":"XAFS and XRD Studies of PdO-CeO2 Catalysts on χ-Al2O3"},"authors":{"en":[{"name":"Li Wei-Bing"},{"name":"Murakami Yuichiro"},{"name":"Orihara Masanao"},{"name":"Tanaka Suminori"},{"name":"Kanaoka Kunio"},{"name":"Murai Kei-ichiro"},{"name":"Moriga Toshihiro"},{"name":"Kanezaki Eiji"},{"name":"Nakabayashi Ichiro"}],"ja":[{"name":"李 衛兵"},{"name":"村上 祐一郎"},{"name":"折原 正直"},{"name":"田中 住典"},{"name":"金岡 邦男"},{"name":"村井 啓一郎"},{"name":"森賀 俊広"},{"name":"金崎 英二"},{"name":"中林 一朗"}]},"publication_date":"2005-03","publication_name":{"en":"Physica Scripta","ja":"Physica Scripta"},"volume":"Vol.T115","starting_page":"749","ending_page":"752","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1238/Physica.Topical.115a00749"],"issn":["0031-8949"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:93, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=81062","label":"url"}],"paper_title":{"en":"NMR study on the Li+ ion diffusion in LiCuO2 with layered structure","ja":"NMR study on the Li+ ion diffusion in LiCuO2 with layered structure"},"authors":{"en":[{"name":"Nakamura Koichi"},{"name":"Moriga Toshihiro"},{"name":"Sumi A."},{"name":"Kashu Y."},{"name":"Michihiro Yoshitaka"},{"name":"Nakabayashi Ichiro"},{"name":"Kanashiro Tatsuo"}],"ja":[{"name":"中村 浩一"},{"name":"森賀 俊広"},{"name":"炭 昭義"},{"name":"Kashu Y."},{"name":"道廣 嘉隆"},{"name":"中林 一朗"},{"name":"金城 辰夫"}]},"description":{"en":"層状構造を持つリチウム遷移金属酸化物LiCuO2はリチウムイオン2次電池材料の候補の一つと考えられる．LiCuO2のリチウムイオン拡散挙動を明らかにするために，7Li核のNMR測定を室温から600Kまでの温度領域で行った．NMRスペクトルの温度依存性においてリチウムイオンの運動にともなう線幅の先鋭化を観測し，リチウムイオン拡散にともなう活性化エネルギーをはじめて明らかにした．LiCuO2におけるスペクトルの先鋭化は370K付近から観測され，活性化エネルギーは0.19eVと評価されたが，それは現行のリチウムイオン2次電池材料であるLiCoO2に匹敵するものであり，高温においてLiCuO2が高速イオン拡散状態にあることが明らかになった．","ja":"層状構造を持つリチウム遷移金属酸化物LiCuO2はリチウムイオン2次電池材料の候補の一つと考えられる．LiCuO2のリチウムイオン拡散挙動を明らかにするために，7Li核のNMR測定を室温から600Kまでの温度領域で行った．NMRスペクトルの温度依存性においてリチウムイオンの運動にともなう線幅の先鋭化を観測し，リチウムイオン拡散にともなう活性化エネルギーをはじめて明らかにした．LiCuO2におけるスペクトルの先鋭化は370K付近から観測され，活性化エネルギーは0.19eVと評価されたが，それは現行のリチウムイオン2次電池材料であるLiCoO2に匹敵するものであり，高温においてLiCuO2が高速イオン拡散状態にあることが明らかになった．"},"publication_date":"2005-02-28","publication_name":{"en":"Solid State Ionics","ja":"Solid State Ionics"},"volume":"Vol.176","number":"No.7-8","starting_page":"837","ending_page":"840","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1016/j.ssi.2004.11.004"],"issn":["0167-2738"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:94, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=82989","label":"url"}],"paper_title":{"en":"Transparent Conducting Amorphous Zn-Sn-O Films Deposited by Simultaneous DC Sputtering","ja":"Transparent Conducting Amorphous Zn-Sn-O Films Deposited by Simultaneous DC Sputtering"},"authors":{"en":[{"name":"Moriga Toshihiro"},{"name":"Hayashi Yukako"},{"name":"Kondo Kumiko"},{"name":"Nishimura Yusuke"},{"name":"Murai Kei-ichiro"},{"name":"Nakabayashi Ichiro"},{"name":"Fukumoto Hidenori"},{"name":"Tominaga Kikuo"}],"ja":[{"name":"森賀 俊広"},{"name":"林 由佳子"},{"name":"近藤 久美子"},{"name":"西村 勇介"},{"name":"村井 啓一郎"},{"name":"中林 一朗"},{"name":"福本 英範"},{"name":"富永 喜久雄"}]},"description":{"en":"酸化亜鉛-酸化スズ系透明導電性アモルファス薄膜について，その組成と透明導電性の関係を明らかにした．アモルファス構造ととっていても，アモルファス中の亜鉛の含有量が増加するに従い，イルメナイト型ZnSnO3に近い構造から逆スピネル型Zn2SnO4に近い構造へと変化していくことを示した．イルメナイト型構造中では亜鉛は6配位であるが，逆スピネル型では4あるいは6配位をとるようになるので，配位数の減少による共有結合性の増加が生じ，その結果酸素欠損が生じにくくなるので，亜鉛含有量が増加するとキャリア濃度が減少し，その結果抵抗率の上昇をもたらすことを示した．","ja":"酸化亜鉛-酸化スズ系透明導電性アモルファス薄膜について，その組成と透明導電性の関係を明らかにした．アモルファス構造ととっていても，アモルファス中の亜鉛の含有量が増加するに従い，イルメナイト型ZnSnO3に近い構造から逆スピネル型Zn2SnO4に近い構造へと変化していくことを示した．イルメナイト型構造中では亜鉛は6配位であるが，逆スピネル型では4あるいは6配位をとるようになるので，配位数の減少による共有結合性の増加が生じ，その結果酸素欠損が生じにくくなるので，亜鉛含有量が増加するとキャリア濃度が減少し，その結果抵抗率の上昇をもたらすことを示した．"},"publication_date":"2004-08","publication_name":{"en":"Journal of Vacuum Science & Technology A","ja":"Journal of Vacuum Science & Technology A"},"volume":"Vol.22","number":"No.4","starting_page":"1705","ending_page":"1710","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1116/1.1765658"],"issn":["0734-2101"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:95, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=79101","label":"url"}],"paper_title":{"en":"Local Structure around Platinum in Pt/C Catalysts Employed for Liquid-phase Dehydrogenation of Decalin in the Liquid-film State under Reactive Distillation Conditions","ja":"Local Structure around Platinum in Pt/C Catalysts Employed for Liquid-phase Dehydrogenation of Decalin in the Liquid-film State under Reactive Distillation Conditions"},"authors":{"en":[{"name":"Shinohara Chiaki"},{"name":"Kawakami Satoshi"},{"name":"Moriga Toshihiro"},{"name":"Hayashi Hiromu"},{"name":"Hidoshima Shinya"},{"name":"Saito Yasukazu"},{"name":"Sugiyama Shigeru"}],"ja":[{"name":"篠原 千明"},{"name":"川上 智"},{"name":"森賀 俊広"},{"name":"林 弘"},{"name":"程島 真哉"},{"name":"斎藤 泰和"},{"name":"杉山 茂"}]},"description":{"en":"水素輸送媒体デカリンからの加熱液膜条件における脱水素反応に高活性を示すPt/Cの白金周りの微細構造がEXAFSで検討された．0価の金属状態にある白金は低活性を示すのに対し，共有結合性の白金が高活性を与えることを明らかにした．担体の塩基処理，白金の還元処理が脱水素触媒活性に大きな影響を与えた．","ja":"水素輸送媒体デカリンからの加熱液膜条件における脱水素反応に高活性を示すPt/Cの白金周りの微細構造がEXAFSで検討された．0価の金属状態にある白金は低活性を示すのに対し，共有結合性の白金が高活性を与えることを明らかにした．担体の塩基処理，白金の還元処理が脱水素触媒活性に大きな影響を与えた．"},"publication_date":"2004-07-20","publication_name":{"en":"Applied Catalysis A: General","ja":"Applied Catalysis A: General"},"volume":"Vol.266","number":"No.2","starting_page":"251","ending_page":"255","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1016/j.apcata.2004.02.014"],"issn":["0926-860X"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:96, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/15293404","label":"url"},{"@id":"https://cir.nii.ac.jp/crid/1520290883444216064/","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=86201","label":"url"}],"paper_title":{"en":"Direct Detection of a Phase Change in PdO/CeO2 Supported on χ-Al2O3 by means of in situ High-Temperature Measurements of XRD and FTIR","ja":"Direct Detection of a Phase Change in PdO/CeO2 Supported on χ-Al2O3 by means of in situ High-Temperature Measurements of XRD and FTIR"},"authors":{"en":[{"name":"Kanezaki Eiji"},{"name":"Tanaka Suminori"},{"name":"Murai Kei-ichiro"},{"name":"Moriga Toshihiro"},{"name":"Motonaka Junko"},{"name":"Katoh Masahiro"},{"name":"Nakabayashi Ichiro"}],"ja":[{"name":"金崎 英二"},{"name":"田中 住典"},{"name":"村井 啓一郎"},{"name":"森賀 俊広"},{"name":"本仲 純子"},{"name":"加藤 雅裕"},{"name":"中林 一朗"}]},"description":{"en":"本論文では，メタン酸化反応におけるc-Al2O3担持PdO/CeO2触媒でのPdOからPdへの変化をXRD及びFT-IRの高温その場測定により直接に観測した．この変化は雰囲気中の酸素分圧変化に対して可逆的であり，この変化がメタン酸化における触媒作用の本質であると結論した．この結論はこれ迄の研究結果をよく説明するものである","ja":"本論文では，メタン酸化反応におけるc-Al2O3担持PdO/CeO2触媒でのPdOからPdへの変化をXRD及びFT-IRの高温その場測定により直接に観測した．この変化は雰囲気中の酸素分圧変化に対して可逆的であり，この変化がメタン酸化における触媒作用の本質であると結論した．この結論はこれ迄の研究結果をよく説明するものである"},"publication_date":"2004-07","publication_name":{"en":"Analytical Sciences","ja":"Analytical Sciences"},"volume":"Vol.20","number":"No.7","starting_page":"1069","ending_page":"1073","languages":["eng"],"referee":true,"identifiers":{"doi":["10.2116/analsci.20.1069"],"issn":["0910-6340"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:97, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=82986","label":"url"}],"paper_title":{"en":"Al-impurity-doped Transparent Conductive Oxide Films of In2O3-ZnO System","ja":"Al-impurity-doped Transparent Conductive Oxide Films of In2O3-ZnO System"},"authors":{"en":[{"name":"Tominaga Kikuo"},{"name":"Fukumoto Hidenori"},{"name":"Kondo Kumiko"},{"name":"Hayashi Yukako"},{"name":"Murai Kei-ichiro"},{"name":"Moriga Toshihiro"},{"name":"Nakabayashi Ichiro"}],"ja":[{"name":"富永 喜久雄"},{"name":"福本 英範"},{"name":"近藤 久美子"},{"name":"林 由佳子"},{"name":"村井 啓一郎"},{"name":"森賀 俊広"},{"name":"中林 一朗"}]},"description":{"en":"ZnO-In2O3系の透明導電膜へのAl2O3の添加効果について調べた．Al2O3を添加しないときには，アモルファス相の膜において，低抵抗率がえられる組成比δ＝Zn/(Zn+In)の範囲は0．2∼0．4と狭いが，A2O3を3wt%添加すると，2∼4x10-4Ωcmの範囲の組成比は0.3∼0．6と広がる．また，Al2O3＝2wt%の膜の光学的バンドギャップが添加しない場合のそれよりも小さくなるband shrinkageを示すが，3wt%添加ではバンドの広がりが観測された．ホモロガス(結晶)相においては，Al2O3の添加量とともに光学的バンドギャップは広がる．これはAl2O3が格子を歪ませている結果であると考えられる．Al2O3の添加はアモルファス膜の抵抗率には大きな変化は与えないが，ホモロガス(結晶)膜ではキャリア密度を減少させ，抵抗率を上昇させた．","ja":"ZnO-In2O3系の透明導電膜へのAl2O3の添加効果について調べた．Al2O3を添加しないときには，アモルファス相の膜において，低抵抗率がえられる組成比δ＝Zn/(Zn+In)の範囲は0．2∼0．4と狭いが，A2O3を3wt%添加すると，2∼4x10-4Ωcmの範囲の組成比は0.3∼0．6と広がる．また，Al2O3＝2wt%の膜の光学的バンドギャップが添加しない場合のそれよりも小さくなるband shrinkageを示すが，3wt%添加ではバンドの広がりが観測された．ホモロガス(結晶)相においては，Al2O3の添加量とともに光学的バンドギャップは広がる．これはAl2O3が格子を歪ませている結果であると考えられる．Al2O3の添加はアモルファス膜の抵抗率には大きな変化は与えないが，ホモロガス(結晶)膜ではキャリア密度を減少させ，抵抗率を上昇させた．"},"publication_date":"2004-04","publication_name":{"en":"Vacuum","ja":"Vacuum"},"volume":"Vol.74","number":"No.3-4","starting_page":"683","ending_page":"687","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1016/j.vacuum.2004.01.042"],"issn":["0042-207X"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:98, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-2442560055&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=81266","label":"url"}],"paper_title":{"en":"ZnO-SnO2 transparent conductive films deposited by opposed target sputtering system of ZnO and SnO2 targets","ja":"ZnO-SnO2 transparent conductive films deposited by opposed target sputtering system of ZnO and SnO2 targets"},"authors":{"en":[{"name":"Hayashi Yukako"},{"name":"Kondo Kumiko"},{"name":"Murai Kei-ichiro"},{"name":"Moriga Toshihiro"},{"name":"Nakabayashi Ichiro"},{"name":"Tominaga Kikuo"}],"ja":[{"name":"林 由佳子"},{"name":"近藤 久美子"},{"name":"村井 啓一郎"},{"name":"森賀 俊広"},{"name":"中林 一朗"},{"name":"富永 喜久雄"}]},"description":{"en":"対向ターゲット式DCマグネトロンスパッタリング法により，酸化亜鉛-酸化スズ系透明導電性薄膜を作製した．薄膜中の亜鉛含有量が増加するに従い，生成相はルチル型相，アモルファス相，ウルツ鉱型相と変化した．アモルファス相では，組成がSnO2·ZnSnO3となる付近で抵抗率が極小値を示し，ZnO·ZnSnO3となる付近で極大値を示すことを明らかにした．","ja":"対向ターゲット式DCマグネトロンスパッタリング法により，酸化亜鉛-酸化スズ系透明導電性薄膜を作製した．薄膜中の亜鉛含有量が増加するに従い，生成相はルチル型相，アモルファス相，ウルツ鉱型相と変化した．アモルファス相では，組成がSnO2·ZnSnO3となる付近で抵抗率が極小値を示し，ZnO·ZnSnO3となる付近で極大値を示すことを明らかにした．"},"publication_date":"2004-03-10","publication_name":{"en":"Vacuum","ja":"Vacuum"},"volume":"Vol.74","number":"No.3-4","starting_page":"607","ending_page":"611","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1016/j.vacuum.2004.01.033"],"issn":["0042-207X"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:99, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"http://ci.nii.ac.jp/naid/110002288181/","label":"url"},{"@id":"https://cir.nii.ac.jp/crid/1390282680226269952/","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=80280","label":"url"}],"paper_title":{"en":"Effect of CeO2 Addition on the Change of Crystal Structure of PdO Supported on x-Al2O3 under the Methane Atmosphere","ja":"メタン雰囲気下におけるx-Al2O3に担持したPdOの結晶構造に及ぼすCeO2添加の影響"},"authors":{"en":[{"name":"Li Wei-Bing"},{"name":"Murakami Yuichiro"},{"name":"Orihara Masanao"},{"name":"Kanaoka Kunio"},{"name":"Tanaka Suminori"},{"name":"Murai Kei-ichiro"},{"name":"Moriga Toshihiro"},{"name":"Kanezaki Eiji"},{"name":"Nakabayashi Ichiro"}],"ja":[{"name":"李 衛兵"},{"name":"村上 祐一郎"},{"name":"折原 正直"},{"name":"金岡 邦夫"},{"name":"田中 住典"},{"name":"村井 啓一郎"},{"name":"森賀 俊広"},{"name":"金崎 英二"},{"name":"中林 一朗"}]},"description":{"en":"本論文では，ギブサイトを前駆体としたc-Al2O3担持PdOを用いたメタン酸化反応におけるPdOの触媒活性とPdOの結晶構造変化との関連を議論した．PdOの触媒活性は，結晶中の格子酸素が反応より消費されることによる．この結果，結晶の(110)面に積層欠陥が生じ，PdOの還元により生じるPdの(100)面がPdOの(110)面と共有していることによってPdの(100)面にも積層欠陥が生じる．この面を介して酸化反応が進行することで，比較的低温で反応が進行することが分かった．CeO2の添加はこの格子不整の維持に役立っていると結論した","ja":"本論文では，ギブサイトを前駆体としたc-Al2O3担持PdOを用いたメタン酸化反応におけるPdOの触媒活性とPdOの結晶構造変化との関連を議論した．PdOの触媒活性は，結晶中の格子酸素が反応より消費されることによる．この結果，結晶の(110)面に積層欠陥が生じ，PdOの還元により生じるPdの(100)面がPdOの(110)面と共有していることによってPdの(100)面にも積層欠陥が生じる．この面を介して酸化反応が進行することで，比較的低温で反応が進行することが分かった．CeO2の添加はこの格子不整の維持に役立っていると結論した"},"publication_date":"2004-03-01","publication_name":{"en":"Journal of Ceramic Society of Japan","ja":"日本セラミックス協会学術論文誌"},"volume":"Vol.112","number":"No.3","starting_page":"149","ending_page":"152","languages":["jpn"],"referee":true,"identifiers":{"doi":["10.2109/jcersj.112.149"],"issn":["0914-5400"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:100, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"http://ci.nii.ac.jp/naid/110002284055/","label":"url"},{"@id":"https://cir.nii.ac.jp/crid/1390001205445575936/","label":"url"},{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-1542364147&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=79102","label":"url"}],"paper_title":{"en":"Effect of Texture and Composition of Microorganisms Carrier for Disposal of Wastewater","ja":"Effect of Texture and Composition of Microorganisms Carrier for Disposal of Wastewater"},"authors":{"en":[{"name":"Hirashima Yasushi"},{"name":"Moriga Toshihiro"},{"name":"Ashida Toshifumi"},{"name":"Kanezaki Eiji"},{"name":"Murai Kei-ichiro"},{"name":"Nakabayashi Ichiro"}],"ja":[{"name":"平島 康"},{"name":"森賀 俊広"},{"name":"芦田 利文"},{"name":"金崎 英二"},{"name":"村井 啓一郎"},{"name":"中林 一朗"}]},"description":{"en":"本論文では，水熱反応により表面処理して種々の多孔性固体を担持したガラス球を用い，排水清浄化を試みた．排水中のCOD測定により，多孔性固体としては珪酸カルシウム，酸化鉄及び酸化カルシウム等が有効であることが分かった．これらの化合物はガラス球表面に付着する微生物の増殖を阻害せず，そのため微生物による排水浄化作用が増大するためであると結論した．又，水熱時間を変えてガラス球表面の微視的構造を変化させその効果を検討したところ，水熱反応が長くなると排水清浄化はほぼ一定の値をとることが明らかになった．","ja":"本論文では，水熱反応により表面処理して種々の多孔性固体を担持したガラス球を用い，排水清浄化を試みた．排水中のCOD測定により，多孔性固体としては珪酸カルシウム，酸化鉄及び酸化カルシウム等が有効であることが分かった．これらの化合物はガラス球表面に付着する微生物の増殖を阻害せず，そのため微生物による排水浄化作用が増大するためであると結論した．又，水熱時間を変えてガラス球表面の微視的構造を変化させその効果を検討したところ，水熱反応が長くなると排水清浄化はほぼ一定の値をとることが明らかになった．"},"publication_date":"2003-12-15","publication_name":{"en":"Materials Science Research International","ja":"Materials Science Research International"},"volume":"Vol.9","number":"No.4","starting_page":"282","ending_page":"286","languages":["eng"],"referee":true,"identifiers":{"doi":["10.2472/jsms.52.12Appendix_282"],"issn":["1341-1683"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:101, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"http://ci.nii.ac.jp/naid/80015896342/","label":"url"},{"@id":"https://cir.nii.ac.jp/crid/1571698601683621632/","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=26415","label":"url"}],"paper_title":{"en":"Enhancement of the Catalytic Activities in Propane Oxidation and H-D Exchangeability of Hydroxyl Groups by the Incorporation with Cobalt into Strontium Hydroxyapatite","ja":"Enhancement of the Catalytic Activities in Propane Oxidation and H-D Exchangeability of Hydroxyl Groups by the Incorporation with Cobalt into Strontium Hydroxyapatite"},"authors":{"en":[{"name":"Sugiyama Shigeru"},{"name":"Shono Tomotaka"},{"name":"Makino Daisaku"},{"name":"Moriga Toshihiro"},{"name":"Hayashi Hiromu"}],"ja":[{"name":"杉山 茂"},{"name":"庄野 友高"},{"name":"牧野 大作"},{"name":"森賀 俊広"},{"name":"林 弘"}]},"description":{"en":"ストロンチウムヒドロキシアパタイトにコバルトカチオンを添加すると，コバルト含有量の増加に伴ってプロパンの酸化活性およびアパタイト中の水酸基プロトンのH-D交換活性が増加した．従って，水酸基が外れて生じる裸の酸素化学種が活性種であることを結論付けた．また通常の手法で構造解析ができなかったコバルトを含有した触媒をXRD,固体NMR,XAFSで解析し，固溶体のヒドロキシアパタイトとしてコバルトが配置されていることを明らかにした．","ja":"ストロンチウムヒドロキシアパタイトにコバルトカチオンを添加すると，コバルト含有量の増加に伴ってプロパンの酸化活性およびアパタイト中の水酸基プロトンのH-D交換活性が増加した．従って，水酸基が外れて生じる裸の酸素化学種が活性種であることを結論付けた．また通常の手法で構造解析ができなかったコバルトを含有した触媒をXRD,固体NMR,XAFSで解析し，固溶体のヒドロキシアパタイトとしてコバルトが配置されていることを明らかにした．"},"publication_date":"2003-02-15","publication_name":{"en":"Journal of Catalysis","ja":"Journal of Catalysis"},"volume":"Vol.214","number":"No.1","starting_page":"8","ending_page":"14","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1016/S0021-9517(02)00101-X"],"issn":["0021-9517"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:102, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"http://ci.nii.ac.jp/naid/10013412309/","label":"url"},{"@id":"https://cir.nii.ac.jp/crid/1390282679541438720/","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=26316","label":"url"}],"paper_title":{"en":"Effects of Redox of Cu-Species in Copper-Strontium Hydroxyapatites on the Oxidative Dehydrogenation of Propane","ja":"Effects of Redox of Cu-Species in Copper-Strontium Hydroxyapatites on the Oxidative Dehydrogenation of Propane"},"authors":{"en":[{"name":"Sugiyama Shigeru"},{"name":"Mitsuoka, Hiromichi"},{"name":"Shono, Tomotaka"},{"name":"Moriga Toshihiro"},{"name":"Hayashi Hiromu"}],"ja":[{"name":"杉山 茂"},{"name":"光岡 宏倫"},{"name":"庄野 友高"},{"name":"森賀 俊広"},{"name":"林 弘"}]},"description":{"en":"プロパンの脱水素酸化反応において四塩化炭素存在下ヒドロキシアパタイトを触媒として反応した場合，活性が激減する．しかし，銅で修飾したストロンチウムヒドロキシアパタイトはプロピレンの収率が著しく改善されることを見出した．銅化合物の特異なレドックス挙動がこのような改善挙動を導き出していることをXAFSなどの測定を行い明かにした．","ja":"プロパンの脱水素酸化反応において四塩化炭素存在下ヒドロキシアパタイトを触媒として反応した場合，活性が激減する．しかし，銅で修飾したストロンチウムヒドロキシアパタイトはプロピレンの収率が著しく改善されることを見出した．銅化合物の特異なレドックス挙動がこのような改善挙動を導き出していることをXAFSなどの測定を行い明かにした．"},"publication_date":"2003-02-01","publication_name":{"en":"Journal of Chemical Engineering of Japan","ja":"Journal of Chemical Engineering of Japan"},"volume":"Vol.36","number":"No.2","starting_page":"210","ending_page":"215","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1252/jcej.36.210"],"issn":["0021-9592"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:103, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-0038778408&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=64951","label":"url"}],"paper_title":{"en":"Structural Property and Activity for Methane Oxidation of Iron Oxides Prepared by NaOH and FeSO4 Solution","ja":"Structural Property and Activity for Methane Oxidation of Iron Oxides Prepared by NaOH and FeSO4 Solution"},"authors":{"en":[{"name":"Orihara Masanao"},{"name":"Nakagawa Kazunori"},{"name":"Li Wei-Bing"},{"name":"Moriga Toshihiro"},{"name":"Murai Kei-ichiro"},{"name":"Sugiyama Shigeru"},{"name":"Nakabayashi Ichiro"}],"ja":[{"name":"折原 正直"},{"name":"中川 和憲"},{"name":"李 衛兵"},{"name":"森賀 俊広"},{"name":"村井 啓一郎"},{"name":"杉山 茂"},{"name":"中林 一朗"}]},"description":{"en":"硫酸鉄水溶液と水酸化ナトリウム水溶液を混合することにより酸化鉄触媒を合成した．オキシ水酸化鉄であるゲータイトは混合比が酸性側である1.9以下あるいはアルカリ性側である2.6以上で生成した．酸性側のゲータイトは結晶性が悪く比表面積が低いにもかかわらずメタン酸化活性は低く，これはゲータイト中に残存する硫酸イオンに由来することを示した．","ja":"硫酸鉄水溶液と水酸化ナトリウム水溶液を混合することにより酸化鉄触媒を合成した．オキシ水酸化鉄であるゲータイトは混合比が酸性側である1.9以下あるいはアルカリ性側である2.6以上で生成した．酸性側のゲータイトは結晶性が悪く比表面積が低いにもかかわらずメタン酸化活性は低く，これはゲータイト中に残存する硫酸イオンに由来することを示した．"},"publication_date":"2003-01-20","publication_name":{"en":"International Journal of Modern Physics B","ja":"International Journal of Modern Physics B"},"volume":"Vol.17","number":"No.8&9","starting_page":"1498","ending_page":"1502","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1142/S0217979203019228"],"issn":["0217-9792"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
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line:108, {"insert":{"user_id":"1000038966","type":"published_papers","id":"30376436"},"force":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=64928","label":"url"}],"paper_title":{"en":"Transparent Conducting Amorphous Oxides in Zinc Oxide-Indium Oxide System","ja":"Transparent Conducting Amorphous Oxides in Zinc Oxide-Indium Oxide System"},"authors":{"en":[{"name":"Moriga Toshihiro"},{"name":"Hosokawa Shoji"},{"name":"Sakamoto Takashi"},{"name":"Fukushima Akihiko"},{"name":"Murai Kei-ichiro"},{"name":"Nakabayashi Ichiro"},{"name":"Tominaga Kikuo"}],"ja":[{"name":"森賀 俊広"},{"name":"細川 昌治"},{"name":"坂本 考史"},{"name":"福島 明彦"},{"name":"村井 啓一郎"},{"name":"中林 一朗"},{"name":"富永 喜久雄"}]},"description":{"en":"酸化亜鉛-酸化インジウム系透明導電性酸化物薄膜の構造と透明導電性の関係について述べたものである．とくに薄膜にのみ現れるアモルファス相がその組成に近いホモロガス化合物ZnkIn2Ok+3と基本的な構造は同じであることを，X線回折図形に現れるブロードな回折ピークの組成依存性ピークシフトを解析することにより証明した．","ja":"酸化亜鉛-酸化インジウム系透明導電性酸化物薄膜の構造と透明導電性の関係について述べたものである．とくに薄膜にのみ現れるアモルファス相がその組成に近いホモロガス化合物ZnkIn2Ok+3と基本的な構造は同じであることを，X線回折図形に現れるブロードな回折ピークの組成依存性ピークシフトを解析することにより証明した．"},"publication_date":"2003-01-15","publication_name":{"en":"10th International Ceramics Congress Part D","ja":"10th International Ceramics Congress Part D"},"starting_page":"1051","ending_page":"1060","languages":["eng"],"referee":true,"invited":true,"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:109, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-0037011231&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=24259","label":"url"}],"paper_title":{"en":"Reduction Processes of Rare-Earth Nickelate Perovskites LnNiO3 (Ln=La, Pr, Nd)","ja":"Reduction Processes of Rare-Earth Nickelate Perovskites LnNiO3 (Ln=La, Pr, Nd)"},"authors":{"en":[{"name":"Moriga Toshihiro"},{"name":"Hayashi Masaki"},{"name":"Sakamoto Takashi"},{"name":"Orihara Masanao"},{"name":"Nakabayashi Ichiro"}],"ja":[{"name":"森賀 俊広"},{"name":"林 正樹"},{"name":"坂本 考史"},{"name":"折原 正直"},{"name":"中林 一朗"}]},"description":{"en":"ペロブスカイト型LnNiO3をトポタクティックに還元して生成する化合物を体系的に纏めた．生成する化合物はLnm+n(Ni3+O6/2)m(Ni+O4/2)nと表すことができることを示した．また，中性子回折法により，このことを支持するPr3Ni3O8の超構造をとらえた．","ja":"ペロブスカイト型LnNiO3をトポタクティックに還元して生成する化合物を体系的に纏めた．生成する化合物はLnm+n(Ni3+O6/2)m(Ni+O4/2)nと表すことができることを示した．また，中性子回折法により，このことを支持するPr3Ni3O8の超構造をとらえた．"},"publication_date":"2002-12-01","publication_name":{"en":"Solid State Ionics","ja":"Solid State Ionics"},"volume":"Vol.154-155","number":"No.0","starting_page":"251","ending_page":"255","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1016/S0167-2738(02)00440-X"],"issn":["0167-2738"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:110, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://ci.nii.ac.jp/naid/110002283981/","label":"url"},{"@id":"https://cir.nii.ac.jp/crid/1390001205443656064/","label":"url"},{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-0036614385&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=25841","label":"url"}],"paper_title":{"en":"Performance of Calcium Silicate Hydrate Briquettes Produced from Fly Ash and Slaked Lime in Disposal of Wastewater","ja":"Performance of Calcium Silicate Hydrate Briquettes Produced from Fly Ash and Slaked Lime in Disposal of Wastewater"},"authors":{"en":[{"name":"Hirashima Yasushi"},{"name":"Moriga Toshihiro"},{"name":"Toshifumi Asida"},{"name":"Kanezaki Eiji"},{"name":"Nakabayashi Ichiro"}],"ja":[{"name":"平島 康"},{"name":"森賀 俊広"},{"name":"芦田 利文"},{"name":"金崎 英二"},{"name":"中林 一朗"}]},"description":{"en":"Hydrothermal reaction of fly ash and slaked lime produces a porous briquette which is composed of amorphous calcium silicate, a tobermorite-like compound and hydrogarnet. It is essential for the molar ratio (calcium oxide)/(silicon dioxide) of the briquette to be 0.3 to achieve high performance in the purification of wastewater through improved microorganism-carrying ability. The chemical oxygen demand (COD<sub>Mn</sub>) index in artificial, non-fecal drainage decreases more rapidly with the use of the briquettes than that without the briquettes. The macroscopic configuration of the briquettes is an important factor in the water-purification ability, although the high specific surface area of the briquettes does not affect the performance. By increasing the circulation flow rate of the wastewater, the purification performance is improved considerably.","ja":"本論文では石炭飛灰と消石灰との反応により無定形珪酸カルシウムやトバモライト類似化合物及びハイドロガ-ネット等を含む多孔性煉瓦を水熱反応により合成し，その排水浄化能について検討した．人工排水中にこの多孔正煉瓦を浸し条件を変えながら排水のCODを測定した．その結果，酸化カルシウム/珪酸のモル比が0.3の多孔正煉瓦が最も高い排水浄化能を持つことが分かった．このことは，多孔性煉瓦表面での微生物の生育の容易さに起因すると結論した．"},"publication_date":"2002-06-15","publication_name":{"en":"Materials Science Research International","ja":"Materials Science Research International"},"volume":"Vol.8","number":"No.2","starting_page":"68","ending_page":"73","languages":["eng"],"referee":true,"identifiers":{"doi":["10.2472/jsms.51.6Appendix_68"],"issn":["1341-1683"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:111, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"http://ci.nii.ac.jp/naid/80015451739/","label":"url"},{"@id":"https://cir.nii.ac.jp/crid/1571698601678439936/","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=24615","label":"url"}],"paper_title":{"en":"Amorphous ZnO-In2O3 transparent conductive films by simultaneous sputtering method of ZnO and In2O3 targets","ja":"Amorphous ZnO-In2O3 transparent conductive films by simultaneous sputtering method of ZnO and In2O3 targets"},"authors":{"en":[{"name":"Tominaga Kikuo"},{"name":"Takao Toshimasa"},{"name":"Fukushima Akihiko"},{"name":"Moriga Toshihiro"},{"name":"Nakabayashi Ichiro"}],"ja":[{"name":"富永 喜久雄"},{"name":"高尾 俊公"},{"name":"福島 明彦"},{"name":"森賀 俊広"},{"name":"中林 一朗"}]},"description":{"en":"2元系のZnO-In2O3をDC対向ターゲット式スパッタ法で作製した．この膜中にAl酸化物やSn酸化物を添加したときの影響について調べた．Al酸化物添加では低抵抗のアモルファス膜が250℃以下で作製できた．最小抵抗率は4x10^-4Ωcmである．Sn酸化物の場合はこれより幾分高い値であった．．AlやSnがドナーとして働いていないことを示す．ホモロガス結晶相の膜の場合も，AlやSnの酸化物の添加は電気特性への影響はほとんど見られない．","ja":"2元系のZnO-In2O3をDC対向ターゲット式スパッタ法で作製した．この膜中にAl酸化物やSn酸化物を添加したときの影響について調べた．Al酸化物添加では低抵抗のアモルファス膜が250℃以下で作製できた．最小抵抗率は4x10^-4Ωcmである．Sn酸化物の場合はこれより幾分高い値であった．．AlやSnがドナーとして働いていないことを示す．ホモロガス結晶相の膜の場合も，AlやSnの酸化物の添加は電気特性への影響はほとんど見られない．"},"publication_date":"2002-05-01","publication_name":{"en":"Vacuum","ja":"Vacuum"},"volume":"Vol.66","number":"No.3-4","starting_page":"505","ending_page":"509","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1016/S0042-207X(02)00123-9"],"issn":["0042-207X"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:112, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-0037136148&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=24614","label":"url"}],"paper_title":{"en":"Film properties of ZnO:Al films deposited by co-sputtering of ZnO:Al and contaminated Zn targets with Co, Mn and Cr","ja":"Film properties of ZnO:Al films deposited by co-sputtering of ZnO:Al and contaminated Zn targets with Co, Mn and Cr"},"authors":{"en":[{"name":"Tominaga Kikuo"},{"name":"Takao Toshimasa"},{"name":"Fukushima Akihiko"},{"name":"Moriga Toshihiro"},{"name":"Nakabayashi Ichiro"}],"ja":[{"name":"富永 喜久雄"},{"name":"高尾 俊公"},{"name":"福島 明彦"},{"name":"森賀 俊広"},{"name":"中林 一朗"}]},"description":{"en":"ZnO:Al 透明導電膜中へのCo, Mn, Crの混入の影響について調べた．Znを過剰に添加した条件でZnO:Al膜を作製した．Znの過剰添加が抵抗率の減少に効果がある．この膜を100℃，空気中でアニーリングすると急激に3x10^-4 Ωcmから5x10^-4 Ωcmへ増大してしまう．このことはZnO:Al中の酸素欠損がかなり存在し，酸素と簡単に反応してしまうことを示す．Mn, Co, Crを混入することで抵抗率は幾分増大するものの300℃までの安定性は増す．とくにCrの安定性はよい．","ja":"ZnO:Al 透明導電膜中へのCo, Mn, Crの混入の影響について調べた．Znを過剰に添加した条件でZnO:Al膜を作製した．Znの過剰添加が抵抗率の減少に効果がある．この膜を100℃，空気中でアニーリングすると急激に3x10^-4 Ωcmから5x10^-4 Ωcmへ増大してしまう．このことはZnO:Al中の酸素欠損がかなり存在し，酸素と簡単に反応してしまうことを示す．Mn, Co, Crを混入することで抵抗率は幾分増大するものの300℃までの安定性は増す．とくにCrの安定性はよい．"},"publication_date":"2002-05-01","publication_name":{"en":"Vacuum","ja":"Vacuum"},"volume":"Vol.66","number":"No.3-4","starting_page":"511","ending_page":"515","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1016/S0042-207X(02)00124-0"],"issn":["0042-207X"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:113, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"http://ci.nii.ac.jp/naid/10007768732/","label":"url"},{"@id":"https://cir.nii.ac.jp/crid/1520290883268352000/","label":"url"},{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-2542459427&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=21038","label":"url"}],"paper_title":{"en":"Effects of Sulfate Ion on Crystal Structure and Activity for Methane Oxidation of Iron Oxide Prepared from Goethite","ja":"ゲータイトから調製した酸化鉄の結晶構造とメタン酸化活性に及ぼす硫酸イオンの影響"},"authors":{"en":[{"name":"Orihara Masanao"},{"name":"Tanaka Suminori"},{"name":"Nakagawa Kazunori"},{"name":"Kawakami Shigeo"},{"name":"Katoh Masahiro"},{"name":"Sugiyama Shigeru"},{"name":"Moriga Toshihiro"},{"name":"Nakabayashi Ichiro"}],"ja":[{"name":"折原 正直"},{"name":"田中 住典"},{"name":"中川 和憲"},{"name":"川上 茂雄"},{"name":"加藤 雅裕"},{"name":"杉山 茂"},{"name":"森賀 俊広"},{"name":"中林 一朗"}]},"description":{"en":"ゲータイトを前駆体として合成した酸化鉄を用いてメタン酸化活性試験を行った．酸化鉄によるメタン酸化活性は硫酸イオンの存在で抑制されることを明らかにした．この活性の低下は鉄原子に電子を供与して鉄の酸化力を減少させることにより引き起こされるが，同時に硫酸イオンは酸化鉄中に多くの酸素欠陥を酸化鉄格子中に導入するので，硫酸イオンが脱離するような550℃以上の高温では逆に活性が向上することを見いだした．","ja":"ゲータイトを前駆体として合成した酸化鉄を用いてメタン酸化活性試験を行った．酸化鉄によるメタン酸化活性は硫酸イオンの存在で抑制されることを明らかにした．この活性の低下は鉄原子に電子を供与して鉄の酸化力を減少させることにより引き起こされるが，同時に硫酸イオンは酸化鉄中に多くの酸素欠陥を酸化鉄格子中に導入するので，硫酸イオンが脱離するような550℃以上の高温では逆に活性が向上することを見いだした．"},"publication_date":"2002-01-01","publication_name":{"en":"Nippon Kagaku Kaishi","ja":"日本化学会誌"},"volume":"Vol.2002","number":"No.1","starting_page":"11","ending_page":"18","languages":["jpn"],"referee":true,"identifiers":{"doi":["10.1246/nikkashi.2002.11"],"issn":["0369-4577"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:114, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-0035874153&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=21034","label":"url"}],"paper_title":{"en":"Effect of insertion of thin ZnO layer in transparent conductive ZnO:Al film","ja":"Effect of insertion of thin ZnO layer in transparent conductive ZnO:Al film"},"authors":{"en":[{"name":"Tominaga Kikuo"},{"name":"Murayama Kazutaka"},{"name":"Mori Ichiro"},{"name":"Ushiro Tomoko"},{"name":"Moriga Toshihiro"},{"name":"Nakabayashi Ichiro"}],"ja":[{"name":"富永 喜久雄"},{"name":"村山 和孝"},{"name":"森 一郎"},{"name":"宇城 恭子"},{"name":"森賀 俊広"},{"name":"中林 一朗"}]},"description":{"en":"ZnO:Al透明導電膜のなかにノンドープのZnO層を挿入する効果について調べた．ZnOの挿入はキャリア密度とホール移動度の増大を示した．また，光透過率スペクトルの吸収端付近での透過率の改善もみられた．これらの結果はZnO層の挿入がZnO:Al中の欠陥密度を減少させる効果をもつことを示す．","ja":"ZnO:Al透明導電膜のなかにノンドープのZnO層を挿入する効果について調べた．ZnOの挿入はキャリア密度とホール移動度の増大を示した．また，光透過率スペクトルの吸収端付近での透過率の改善もみられた．これらの結果はZnO層の挿入がZnO:Al中の欠陥密度を減少させる効果をもつことを示す．"},"publication_date":"2001-07-01","publication_name":{"en":"Thin Solid Films","ja":"Thin Solid Films"},"volume":"Vol.386","number":"No.2","starting_page":"267","ending_page":"270","referee":true,"identifiers":{"doi":["10.1016/S0040-6090(00)01679-5"],"issn":["0040-6090"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:115, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-0035270558&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=12354","label":"url"}],"paper_title":{"en":"Structural variation of thin films deposited from Zn3In2O6 target by RF-sputtering","ja":"Structural variation of thin films deposited from Zn3In2O6 target by RF-sputtering"},"authors":{"en":[{"name":"Ushiro Tomoko"},{"name":"Tsuji Daisuke"},{"name":"Fukushima Akihiko"},{"name":"Moriga Toshihiro"},{"name":"Nakabayashi Ichiro"},{"name":"Murayama Kazutaka"},{"name":"Tominaga Kikuo"}],"ja":[{"name":"宇城 恭子"},{"name":"辻 大輔"},{"name":"福島 明彦"},{"name":"森賀 俊広"},{"name":"中林 一朗"},{"name":"村山 和孝"},{"name":"富永 喜久雄"}]},"description":{"en":"ホモロガス化合物のうち最も電気伝導度が高いZn3In2O6を用い，RFスパッタリング法にて酸化亜鉛-酸化インジウム系透明導電性薄膜を作製した．基板温度が高くなるにつれて，生成相はZn3In2O6からZn2In2O5を経てビックスバイト型In2O3へとインジウム含有量が多い相へと変化するが，それに伴い透明導電性も変化することを明らかにした．","ja":"ホモロガス化合物のうち最も電気伝導度が高いZn3In2O6を用い，RFスパッタリング法にて酸化亜鉛-酸化インジウム系透明導電性薄膜を作製した．基板温度が高くなるにつれて，生成相はZn3In2O6からZn2In2O5を経てビックスバイト型In2O3へとインジウム含有量が多い相へと変化するが，それに伴い透明導電性も変化することを明らかにした．"},"publication_date":"2001-04-01","publication_name":{"en":"Materials Research Bulletin","ja":"Materials Research Bulletin"},"volume":"Vol.36","number":"No.5-6","starting_page":"1075","ending_page":"1082","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1016/S0025-5408(01)00583-9"],"issn":["0025-5408"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:116, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/11512931","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=18647","label":"url"}],"paper_title":{"en":"Crystallization Process of Transparent Conductive Oxides ZnkIn2Ok+3","ja":"Crystallization Process of Transparent Conductive Oxides ZnkIn2Ok+3"},"authors":{"en":[{"name":"Moriga Toshihiro"},{"name":"Fukushima Akihiko"},{"name":"Tomonari Yozo"},{"name":"Hosokawa Shoji"},{"name":"Tominaga Kikuo"},{"name":"Nakabayashi Ichiro"}],"ja":[{"name":"森賀 俊広"},{"name":"Fukushima Akihiko"},{"name":"Tomonari Yozo"},{"name":"Hosokawa Shoji"},{"name":"富永 喜久雄"},{"name":"中林 一朗"}]},"description":{"en":"共沈法により作製した酸化亜鉛-酸化インジウム系ホモロガス化合物ZnkIn2Ok+3の結晶化過程をX線回折法およびXAFS法にて追跡した．非晶質前駆体を加熱していくと，まずウルツ鉱型ZnOが結晶化しそのZnOと非晶質のIn2O3が反応してホモロガス化合物が生成することを明らかにした．","ja":"共沈法により作製した酸化亜鉛-酸化インジウム系ホモロガス化合物ZnkIn2Ok+3の結晶化過程をX線回折法およびXAFS法にて追跡した．非晶質前駆体を加熱していくと，まずウルツ鉱型ZnOが結晶化しそのZnOと非晶質のIn2O3が反応してホモロガス化合物が生成することを明らかにした．"},"publication_date":"2001-03-01","publication_name":{"en":"Journal of Synchrotron Radiation","ja":"Journal of Synchrotron Radiation"},"volume":"Vol.8","number":"No.Pt 2","starting_page":"785","ending_page":"787","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1107/S0909049500018264"],"issn":["0909-0495"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:117, {"insert":{"user_id":"1000038966","type":"published_papers","id":"30800925"},"force":{"see_also":[{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-0035122833&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=12125","label":"url"}],"paper_title":{"en":"Characterization of Calcium, Strontium, Barium and Lead Hydroxyapatites: X-ray Diffraction, Photoelectron, Extended X-ray Absorption Fine Structure and MAS NMR Spectroscopies","ja":"Characterization of Calcium, Strontium, Barium and Lead Hydroxyapatites: X-ray Diffraction, Photoelectron, Extended X-ray Absorption Fine Structure and MAS NMR Spectroscopies"},"authors":{"en":[{"name":"Sugiyama Shigeru"},{"name":"Moriga Toshihiro"},{"name":"Hayashi Hiromu"},{"name":"Moffat B. John"}],"ja":[{"name":"杉山 茂"},{"name":"森賀 俊広"},{"name":"林 弘"},{"name":"Moffat B. John"}]},"description":{"en":"カルシウム，ストロンチウム，バリウムおよび鉛ヒドロキシアパタイトを固体材料の先端分析技術であるX線回折法，X線光電子分光分析，広域X線吸収微細構造分析および固体NMRを用いて分析し，特異なアパタイト構造の解析には先端分析技術の採用が不可欠であることを示した．","ja":"カルシウム，ストロンチウム，バリウムおよび鉛ヒドロキシアパタイトを固体材料の先端分析技術であるX線回折法，X線光電子分光分析，広域X線吸収微細構造分析および固体NMRを用いて分析し，特異なアパタイト構造の解析には先端分析技術の採用が不可欠であることを示した．"},"publication_date":"2001-01-01","publication_name":{"en":"Bulletin of the Chemical Society of Japan","ja":"Bulletin of the Chemical Society of Japan"},"volume":"Vol.74","number":"No.1","starting_page":"187","ending_page":"192","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1246/bcsj.74.187"],"issn":["1348-0634"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:118, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-0034810637&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=11934","label":"url"}],"paper_title":{"en":"In Situ XRD and In Situ IR Spectroscopic Analyses of Structural Change of Goethite in Methane Oxidation","ja":"In Situ XRD and In Situ IR Spectroscopic Analyses of Structural Change of Goethite in Methane Oxidation"},"authors":{"en":[{"name":"Katoh Masahiro"},{"name":"Orihara Masanao"},{"name":"Moriga Toshihiro"},{"name":"Nakabayashi Ichiro"},{"name":"Sugiyama Shigeru"},{"name":"Tanaka Suminori"}],"ja":[{"name":"加藤 雅裕"},{"name":"Orihara Masanao"},{"name":"森賀 俊広"},{"name":"中林 一朗"},{"name":"杉山 茂"},{"name":"Tanaka Suminori"}]},"description":{"en":"含水酸化鉄の一種であるゲータイトのメタン酸化活性について調べた．ゲータイトは針状結晶であるが，220∼230℃付近で脱水により比表面積の非常に大きい酸化鉄であるヘマタイトに相変態をすること，その比表面積の大きいヘマタイトがメタン酸化に大きく関わっていることをその場観察X線回折およびその場観察赤外分光法により明らかにした．","ja":"含水酸化鉄の一種であるゲータイトのメタン酸化活性について調べた．ゲータイトは針状結晶であるが，220∼230℃付近で脱水により比表面積の非常に大きい酸化鉄であるヘマタイトに相変態をすること，その比表面積の大きいヘマタイトがメタン酸化に大きく関わっていることをその場観察X線回折およびその場観察赤外分光法により明らかにした．"},"publication_date":"2001-01-01","publication_name":{"en":"Journal of Solid State Chemistry","ja":"Journal of Solid State Chemistry"},"volume":"Vol.156","number":"No.1","starting_page":"225","ending_page":"229","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1006/jssc.2000.8992"],"issn":["0022-4596"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
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line:120, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=11918","label":"url"}],"paper_title":{"en":"Reaction Mechanism of Metal Silicide Mg2Si for Li Insertion","ja":"Reaction Mechanism of Metal Silicide Mg2Si for Li Insertion"},"authors":{"en":[{"name":"Moriga Toshihiro"},{"name":"Watanabe Kozo"},{"name":"Tsuji Daisuke"},{"name":"Massaki Shinichi"},{"name":"Nakabayashi Ichiro"}],"ja":[{"name":"森賀 俊広"},{"name":"渡辺 耕三"},{"name":"辻 大輔"},{"name":"眞崎 伸一"},{"name":"中林 一朗"}]},"description":{"en":"金属ケイ化物Mg2Siの電気化学的Li挿入による結晶構造変化を示した．反応は，Mg2Si+2Li++2e- -> Li2MgSi+Mgの要領で進行すること，生成したLi2MgSiは空間群Fm-3mで2x2x2のホタル石型の超構造を有することを明らかにした．","ja":"金属ケイ化物Mg2Siの電気化学的Li挿入による結晶構造変化を示した．反応は，Mg2Si+2Li++2e- -> Li2MgSi+Mgの要領で進行すること，生成したLi2MgSiは空間群Fm-3mで2x2x2のホタル石型の超構造を有することを明らかにした．"},"publication_date":"2000-09-01","publication_name":{"en":"Journal of Solid State Chemistry","ja":"Journal of Solid State Chemistry"},"volume":"Vol.153","number":"No.2","starting_page":"386","ending_page":"390","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1006/jssc.2000.8787"],"issn":["0022-4596"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:121, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-0034262839&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=11907","label":"url"}],"paper_title":{"en":"Effects of Charge/Discharge of Li1-xNi1-yMnyO2 on Their Crystal Structures and Electronic States","ja":"Effects of Charge/Discharge of Li1-xNi1-yMnyO2 on Their Crystal Structures and Electronic States"},"authors":{"en":[{"name":"Moriga Toshihiro"},{"name":"Okamura Kazuhiro"},{"name":"Watanabe Kozo"},{"name":"Nakabayashi Ichiro"}],"ja":[{"name":"森賀 俊広"},{"name":"岡村 一広"},{"name":"渡辺 耕三"},{"name":"中林 一朗"}]},"description":{"en":"リチウムイオン2次電池正極材料として使用されているLi1-xNi1-yO2へのMn置換が，その充放電特性や充放電時の結晶構造変化に及ぼす影響を議論した．Mn置換により充放電によるLi含有量の変化に伴う結晶構造変化が抑えられることを明らかにした．","ja":"リチウムイオン2次電池正極材料として使用されているLi1-xNi1-yO2へのMn置換が，その充放電特性や充放電時の結晶構造変化に及ぼす影響を議論した．Mn置換により充放電によるLi含有量の変化に伴う結晶構造変化が抑えられることを明らかにした．"},"publication_date":"2000-09-01","publication_name":{"en":"Materials Science Research International","ja":"Materials Science Research International"},"volume":"Vol.6","number":"No.3","starting_page":"221","ending_page":"226","languages":["eng"],"referee":true,"identifiers":{"issn":["1341-1683"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:122, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=12109","label":"url"}],"paper_title":{"en":"The Rietveld analysis of crystal structure of an additive telluromolybdate CoTeMoO6","ja":"The Rietveld analysis of crystal structure of an additive telluromolybdate CoTeMoO6"},"authors":{"en":[{"name":"Hayashi Hiromu"},{"name":"Kokawa Nobuhiro"},{"name":"Moriga Toshihiro"},{"name":"Sugiyama Shigeru"},{"name":"Koto Kichiro"}],"ja":[{"name":"林 弘"},{"name":"古川 伸洋"},{"name":"森賀 俊広"},{"name":"杉山 茂"},{"name":"小藤 吉郎"}]},"description":{"en":"乳酸エチルの気相酸化によるピルビン酸合成に対して，低温活性を示す三元系付加型テルロモリブデン酸CoTeMoO6について，Rietvelt解析により金属三元素の原子座標を明らかにし，気相酸化における触媒機能を考察した．活性座Mo=Oに塩基性のO-Te-Oの隣接する構造が低温活性の発現要因であることを示した．","ja":"乳酸エチルの気相酸化によるピルビン酸合成に対して，低温活性を示す三元系付加型テルロモリブデン酸CoTeMoO6について，Rietvelt解析により金属三元素の原子座標を明らかにし，気相酸化における触媒機能を考察した．活性座Mo=Oに塩基性のO-Te-Oの隣接する構造が低温活性の発現要因であることを示した．"},"publication_date":"1999-10-01","publication_name":{"en":"Journal of Molecular Catalysis A: Chemical","ja":"Journal of Molecular Catalysis A: Chemical"},"volume":"Vol.145","starting_page":"301","ending_page":"307","languages":["eng"],"referee":true,"identifiers":{"issn":["1381-1169"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:123, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=11919","label":"url"}],"paper_title":{"en":"Electrical and Optical Properties of Transparent Conducting Homologous Compounds in the Indium-Gallium -Zinc Oxide System","ja":"Electrical and Optical Properties of Transparent Conducting Homologous Compounds in the Indium-Gallium -Zinc Oxide System"},"authors":{"en":[{"name":"Moriga Toshihiro"},{"name":"Kammler R. Daniel"},{"name":"Mason O. Thomas"},{"name":"Palmer B. George"},{"name":"Poeppelmeier R. Kenneth"}],"ja":[{"name":"森賀 俊広"},{"name":"Kammler R. Daniel"},{"name":"Mason O. Thomas"},{"name":"Palmer B. George"},{"name":"Poeppelmeier R. Kenneth"}]},"description":{"en":"酸化インジウム-酸化ガリウム-酸化亜鉛に現れるホモロガス化合物In1-xGa1+xO3·(ZnO)k (k=1，2，3)での単一相生成領域を明らかにした．これらホモロガス化合物固溶体の組成と格子定数，透明導電性との関係について議論した．","ja":"酸化インジウム-酸化ガリウム-酸化亜鉛に現れるホモロガス化合物In1-xGa1+xO3·(ZnO)k (k=1，2，3)での単一相生成領域を明らかにした．これらホモロガス化合物固溶体の組成と格子定数，透明導電性との関係について議論した．"},"publication_date":"1999-10-01","publication_name":{"en":"Journal of American Ceramic Society","ja":"Journal of American Ceramic Society"},"volume":"Vol.82","number":"No.10","starting_page":"2705","ending_page":"2710","languages":["eng"],"referee":true,"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:124, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/15263375","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=11920","label":"url"}],"paper_title":{"en":"Local Structures around Co and Mn Ions in ZnO-Based Varistors","ja":"Local Structures around Co and Mn Ions in ZnO-Based Varistors"},"authors":{"en":[{"name":"Moriga Toshihiro"},{"name":"Nakabayashi Ichiro"}],"ja":[{"name":"森賀 俊広"},{"name":"中林 一朗"}]},"description":{"en":"蛍光XAFS法を用いて，酸化亜鉛バリスタ中に含まれるCoとMnの局所構造を解析した．Coはウルツ鉱型酸化亜鉛マトリックス中に固溶しているのに対し，Mnは粒界付近に第2相として析出していることが示唆された．","ja":"蛍光XAFS法を用いて，酸化亜鉛バリスタ中に含まれるCoとMnの局所構造を解析した．Coはウルツ鉱型酸化亜鉛マトリックス中に固溶しているのに対し，Mnは粒界付近に第2相として析出していることが示唆された．"},"publication_date":"1999-07-01","publication_name":{"en":"Journal of Synchrotron Radiation","ja":"Journal of Synchrotron Radiation"},"volume":"Vol.6","number":"No.Pt 3","starting_page":"546","ending_page":"548","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1107/S090904959801601X"],"issn":["0909-0495"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:125, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=12110","label":"url"}],"paper_title":{"en":"Preparation, Characterization and Thermal Stability of Lead Hydroxyapatites","ja":"Preparation, Characterization and Thermal Stability of Lead Hydroxyapatites"},"authors":{"en":[{"name":"Sugiyama Shigeru"},{"name":"Nakanishi Tomomi"},{"name":"Ishimura Tomohiro"},{"name":"Moriga Toshihiro"},{"name":"Hayashi Hiromu"},{"name":"Shigemoto Naoya"},{"name":"Moffat B. John"}],"ja":[{"name":"杉山 茂"},{"name":"中西 智美"},{"name":"石村 朋広"},{"name":"森賀 俊広"},{"name":"林 弘"},{"name":"重本 直也"},{"name":"Moffat B. John"}]},"description":{"en":"文献処方が詳細に報告されていない鉛ヒドロキシアパタイトの合成法の詳細を確定し，さらに材料としても注目されているこの物質の熱安定性，微細構造などを詳細に検討した論文．","ja":"文献処方が詳細に報告されていない鉛ヒドロキシアパタイトの合成法の詳細を確定し，さらに材料としても注目されているこの物質の熱安定性，微細構造などを詳細に検討した論文．"},"publication_date":"1999-03-01","publication_name":{"en":"Journal of Solid State Chemistry","ja":"Journal of Solid State Chemistry"},"volume":"Vol.143","starting_page":"296","ending_page":"302","languages":["eng"],"referee":true,"identifiers":{"issn":["0022-4596"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:126, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=12107","label":"url"}],"paper_title":{"en":"Preparative Enhancement of the Thermal Stability of Calcium Hydroxyapatites","ja":"Preparative Enhancement of the Thermal Stability of Calcium Hydroxyapatites"},"authors":{"en":[{"name":"Sugiyama Shigeru"},{"name":"Yasutomi Takayuki"},{"name":"Moriga Toshihiro"},{"name":"Hayashi Hiromu"},{"name":"Moffat B. John"}],"ja":[{"name":"杉山 茂"},{"name":"安冨 貴之"},{"name":"森賀 俊広"},{"name":"林 弘"},{"name":"Moffat B. John"}]},"description":{"en":"カルシウムヒドロキシアパタイトを酢酸カルシウムとリン酸水素二ナトリウムから合成すると973Kで大部分リン酸カルシウムへ変換されるが，合成過程でpHを高く維持すると1473Kでも安定なカルシウムヒドロキシアパタイトが合成できた．EXAFSによる微細構造変化も検討した．","ja":"カルシウムヒドロキシアパタイトを酢酸カルシウムとリン酸水素二ナトリウムから合成すると973Kで大部分リン酸カルシウムへ変換されるが，合成過程でpHを高く維持すると1473Kでも安定なカルシウムヒドロキシアパタイトが合成できた．EXAFSによる微細構造変化も検討した．"},"publication_date":"1999-02-01","publication_name":{"en":"Journal of Solid State Chemistry","ja":"Journal of Solid State Chemistry"},"volume":"Vol.142","starting_page":"319","ending_page":"324","languages":["eng"],"referee":true,"identifiers":{"issn":["0022-4596"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:127, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=16731","label":"url"}],"paper_title":{"en":"Properties of films of multilayered ZnO:Al and ZnO deposited by an alternating sputtering method","ja":"Properties of films of multilayered ZnO:Al and ZnO deposited by an alternating sputtering method"},"authors":{"en":[{"name":"Tominaga Kikuo"},{"name":"Umezu Norio"},{"name":"Mori Ichiro"},{"name":"Ushiro Tomoko"},{"name":"Moriga Toshihiro"},{"name":"Nakabayashi Ichiro"}],"ja":[{"name":"富永 喜久雄"},{"name":"Umezu Norio"},{"name":"Mori Ichiro"},{"name":"Ushiro Tomoko"},{"name":"森賀 俊広"},{"name":"中林 一朗"}]},"description":{"en":"ZnO:Al ターゲットとZnターゲットを一定時間間隔で交互にスパッタする交代式スパッタ法で，ZnO:AlとZnOの多層膜構造を作製した．ZnO:Al 層の間に挟んだZnO層の効果につて調べた．ZnO:Al層の厚さを一定の下でAl2O3を2 wt%添加したZnO:Alの場合，ZnOの厚さの増加によりキャリア密度とホール移動度の両方が増加した．同時に，結晶粒成長も観察された．Al2O3=6 wt%と過剰に酸化アルミニウムを添加したZnO:Al膜に対しては移動度は増すが，キャリア密度は減少した．後者で，ZnO:Al+ZnOの厚さを一定に保ちZnOの厚さを変えると，ZnO:Al/ZnO=0.2/0.8のときZnO:Al(Al2O3=3 wt%)での最小抵抗値に近い抵抗地が得られた．両者はAl2O3の添加量が等しい．これらの結果は，ZnO:Al toZnOが共存するとき，Al2O3の一定比率の添加量で抵抗の最低値をとることを示している．","ja":"ZnO:Al ターゲットとZnターゲットを一定時間間隔で交互にスパッタする交代式スパッタ法で，ZnO:AlとZnOの多層膜構造を作製した．ZnO:Al 層の間に挟んだZnO層の効果につて調べた．ZnO:Al層の厚さを一定の下でAl2O3を2 wt%添加したZnO:Alの場合，ZnOの厚さの増加によりキャリア密度とホール移動度の両方が増加した．同時に，結晶粒成長も観察された．Al2O3=6 wt%と過剰に酸化アルミニウムを添加したZnO:Al膜に対しては移動度は増すが，キャリア密度は減少した．後者で，ZnO:Al+ZnOの厚さを一定に保ちZnOの厚さを変えると，ZnO:Al/ZnO=0.2/0.8のときZnO:Al(Al2O3=3 wt%)での最小抵抗値に近い抵抗地が得られた．両者はAl2O3の添加量が等しい．これらの結果は，ZnO:Al toZnOが共存するとき，Al2O3の一定比率の添加量で抵抗の最低値をとることを示している．"},"publication_date":"1999-01-01","publication_name":{"en":"Thin Solid Films","ja":"Thin Solid Films"},"volume":"Vol.343-344","starting_page":"160","ending_page":"163","referee":true,"identifiers":{"issn":["0040-6090"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:128, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=11921","label":"url"}],"paper_title":{"en":"Crystal Structures and Electrical and Optical Properties of MgIn2-xGaxO4 Solid Solutions","ja":"Crystal Structures and Electrical and Optical Properties of MgIn2-xGaxO4 Solid Solutions"},"authors":{"en":[{"name":"Moriga Toshihiro"},{"name":"Sakamoto Takashi"},{"name":"Sato Yoshiki"},{"name":"Azrul Hisham Khalid Haris"},{"name":"Suenari Ryoichi"},{"name":"Nakabayashi Ichiro"}],"ja":[{"name":"森賀 俊広"},{"name":"Sakamoto Takashi"},{"name":"Sato Yoshiki"},{"name":"Azrul Hisham Khalid Haris"},{"name":"Suenari Ryoichi"},{"name":"中林 一朗"}]},"description":{"en":"逆スピネル型MgIn2O4と同じくMgGa2O4の固溶体を合成し，その透明導電性酸化物としての可能性を探った．両化合物は結晶構造が同じであるにもかかわらず，組成が1:1付近で層状化合物MgInGaO4を生成することを示した．また，MgIn2O4に少量のMgGa2O4を固溶させるだけで電気伝導度は大幅に減少することを明らかにした．","ja":"逆スピネル型MgIn2O4と同じくMgGa2O4の固溶体を合成し，その透明導電性酸化物としての可能性を探った．両化合物は結晶構造が同じであるにもかかわらず，組成が1:1付近で層状化合物MgInGaO4を生成することを示した．また，MgIn2O4に少量のMgGa2O4を固溶させるだけで電気伝導度は大幅に減少することを明らかにした．"},"publication_date":"1999-01-01","publication_name":{"en":"Journal of Solid State Chemistry","ja":"Journal of Solid State Chemistry"},"volume":"Vol.142","starting_page":"206","ending_page":"213","languages":["eng"],"referee":true,"identifiers":{"issn":["0022-4596"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:129, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=18316","label":"url"}],"paper_title":{"en":"Transparent conductive ZnO film preparation by alternative sputtering of ZnO:Al target and either Zn or Al targets","ja":"Transparent conductive ZnO film preparation by alternative sputtering of ZnO:Al target and either Zn or Al targets"},"authors":{"en":[{"name":"Tominaga Kikuo"},{"name":"Umezu Norio"},{"name":"Mori Ichiro"},{"name":"Ushiro Tomoko"},{"name":"Moriga Toshihiro"},{"name":"Nakabayashi Ichiro"}],"ja":[{"name":"富永 喜久雄"},{"name":"Umezu Norio"},{"name":"Mori Ichiro"},{"name":"Ushiro Tomoko"},{"name":"森賀 俊広"},{"name":"中林 一朗"}]},"description":{"en":"本論文は，透明導電膜であるZnO:Al膜作製におけるZnの過剰添加の効果をしらべる一連の研究の中で，ZnO:AlとZnO:OVを層状にしたとき，どのような電気的，光学的特性になるのかについて検討したものである．結果は，ZnO:Alの結晶粒成長が促進され，それに並行してキャリア密度密度と移動度の増大し，光透過率も改善された．酸化アルミニウムをZnO:Alに挟む場合は，Al2O3の膜厚の増加とともにキャリア密度，移動度は減少し，抵抗率は増加した．界面でのキャリアの散乱によるものと考えられる．","ja":"本論文は，透明導電膜であるZnO:Al膜作製におけるZnの過剰添加の効果をしらべる一連の研究の中で，ZnO:AlとZnO:OVを層状にしたとき，どのような電気的，光学的特性になるのかについて検討したものである．結果は，ZnO:Alの結晶粒成長が促進され，それに並行してキャリア密度密度と移動度の増大し，光透過率も改善された．酸化アルミニウムをZnO:Alに挟む場合は，Al2O3の膜厚の増加とともにキャリア密度，移動度は減少し，抵抗率は増加した．界面でのキャリアの散乱によるものと考えられる．"},"publication_date":"1998-09-01","publication_name":{"en":"Thin Solid Films","ja":"Thin Solid Films"},"volume":"Vol.334","starting_page":"35","ending_page":"39","referee":true,"identifiers":{"issn":["0040-6090"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:130, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=16717","label":"url"}],"paper_title":{"en":"Properties of ZnO:In Film prepared by sputtering of Facing ZnO:In and Zn targets","ja":"Properties of ZnO:In Film prepared by sputtering of Facing ZnO:In and Zn targets"},"authors":{"en":[{"name":"Tominaga Kikuo"},{"name":"Umezu Norio"},{"name":"Mori Ichiro"},{"name":"Ushiro Tomoko"},{"name":"Moriga Toshihiro"},{"name":"Nakabayashi Ichiro"}],"ja":[{"name":"富永 喜久雄"},{"name":"Umezu Norio"},{"name":"Mori Ichiro"},{"name":"Ushiro Tomoko"},{"name":"森賀 俊広"},{"name":"中林 一朗"}]},"description":{"en":"透明導電膜であるインジウム添加の酸化亜鉛膜も多く研究されているが，本論文では，対向ターゲット式プレーナマグネトロンスパッタ装置でZnO:In膜を作製するとき，In2O3=1.5, 3, 9 wt%の3種のターゲットから等価的にInの添加量を変えた．キャリア密度nは3wt%の時に達成された．n=kCD-NAの実験結果が得られた．NAは欠陥密度といえる．NA=4x1020cm-3とかなり大きいことがわかった．また，キャリア密度は作製時の基板温度が150℃で最高値を示し，300℃では急激なnの過低下を示した．Inの蒸発が予想された．また，Znの過剰供給の条件でZnO:In膜作製を行っても，ほとんど抵抗率への影響は見られなかった．ZnO:Al膜とは異なる．これは，Znの過剰添加によってもInのドナーになる効率は上昇しないことによる．すなわち，ZnO:Inでは，すでにすべての添加されたInがドナーになっているためであると考えられる．","ja":"透明導電膜であるインジウム添加の酸化亜鉛膜も多く研究されているが，本論文では，対向ターゲット式プレーナマグネトロンスパッタ装置でZnO:In膜を作製するとき，In2O3=1.5, 3, 9 wt%の3種のターゲットから等価的にInの添加量を変えた．キャリア密度nは3wt%の時に達成された．n=kCD-NAの実験結果が得られた．NAは欠陥密度といえる．NA=4x1020cm-3とかなり大きいことがわかった．また，キャリア密度は作製時の基板温度が150℃で最高値を示し，300℃では急激なnの過低下を示した．Inの蒸発が予想された．また，Znの過剰供給の条件でZnO:In膜作製を行っても，ほとんど抵抗率への影響は見られなかった．ZnO:Al膜とは異なる．これは，Znの過剰添加によってもInのドナーになる効率は上昇しないことによる．すなわち，ZnO:Inでは，すでにすべての添加されたInがドナーになっているためであると考えられる．"},"publication_date":"1998-09-01","publication_name":{"en":"Journal of Vacuum Science & Technology A","ja":"Journal of Vacuum Science & Technology A"},"volume":"Vol.A16","number":"No.3","starting_page":"1213","ending_page":"1217","referee":true,"identifiers":{"issn":["0734-2101"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:131, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=12100","label":"url"}],"paper_title":{"en":"Ion-Exchange Properties of Strontium Hydroxyapatite under Acidic Conditions","ja":"Ion-Exchange Properties of Strontium Hydroxyapatite under Acidic Conditions"},"authors":{"en":[{"name":"Sugiyama Shigeru"},{"name":"Nishioka Hitoshi"},{"name":"Moriga Toshihiro"},{"name":"Hayashi Hiromu"},{"name":"Moffat B. John"}],"ja":[{"name":"杉山 茂"},{"name":"西岡 均"},{"name":"森賀 俊広"},{"name":"林 弘"},{"name":"Moffat B. John"}]},"description":{"en":"様々な酸性水溶液中でストロンチウムヒドロキシアパタイトのストロンチウムと鉛とのカチオン交換挙動を検討し，酸の種類によらず酸添加によってカチオン交換が加速されることを示した．XAFSによる局所構造変化についても述べた．","ja":"様々な酸性水溶液中でストロンチウムヒドロキシアパタイトのストロンチウムと鉛とのカチオン交換挙動を検討し，酸の種類によらず酸添加によってカチオン交換が加速されることを示した．XAFSによる局所構造変化についても述べた．"},"publication_date":"1998-09-01","publication_name":{"en":"Separation Science and Technology","ja":"Separation Science and Technology"},"volume":"Vol.33","number":"No.13","starting_page":"1999","ending_page":"2007","languages":["eng"],"referee":true,"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:132, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=12099","label":"url"}],"paper_title":{"en":"Effects of the Thermal Stability and the Fine Structure Changes of Strontium Hydroxyapatites Ion-Exchanged with Lead on Methane Oxidation in the Presence and Absence of Tetrachloromethane","ja":"Effects of the Thermal Stability and the Fine Structure Changes of Strontium Hydroxyapatites Ion-Exchanged with Lead on Methane Oxidation in the Presence and Absence of Tetrachloromethane"},"authors":{"en":[{"name":"Sugiyama Shigeru"},{"name":"Iguchi Yoshimasa"},{"name":"Nishioka Hitoshi"},{"name":"Minami Toshimitsu"},{"name":"Moriga Toshihiro"},{"name":"Hayashi Hiromu"},{"name":"Moffat B. John"}],"ja":[{"name":"杉山 茂"},{"name":"井口 悦将"},{"name":"西岡 均"},{"name":"南 俊充"},{"name":"森賀 俊広"},{"name":"林 弘"},{"name":"Moffat B. John"}]},"description":{"en":"イオン交換法で合成したストロンチウムヒドロキシアパタイトのストロンチウムを鉛に置き換えた触媒の熱安定性と構造を詳細に検討し，構造の特徴をメタンの酸化触媒活性に相関させた．鉛の含有量の増加に伴ってEXAFSから得られる鉛と最近接酸素の距離が短くなり触媒活性に影響を与えていることを示した．","ja":"イオン交換法で合成したストロンチウムヒドロキシアパタイトのストロンチウムを鉛に置き換えた触媒の熱安定性と構造を詳細に検討し，構造の特徴をメタンの酸化触媒活性に相関させた．鉛の含有量の増加に伴ってEXAFSから得られる鉛と最近接酸素の距離が短くなり触媒活性に影響を与えていることを示した．"},"publication_date":"1998-05-01","publication_name":{"en":"Journal of Catalysis","ja":"Journal of Catalysis"},"volume":"Vol.176","number":"No.1","starting_page":"25","ending_page":"34","languages":["eng"],"referee":true,"identifiers":{"issn":["0021-9517"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:133, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=11923","label":"url"}],"paper_title":{"en":"Phase Relationships and Physical Properties of Homologous Compounds in the Zinc Oxide-Indium Oxide System","ja":"Phase Relationships and Physical Properties of Homologous Compounds in the Zinc Oxide-Indium Oxide System"},"authors":{"en":[{"name":"Moriga Toshihiro"},{"name":"Edwards D. Doreen"},{"name":"Mason O. Thomas"},{"name":"Palmer B. George"},{"name":"Poeppelmeier R. Kenneth"},{"name":"Schindler L. Jon"},{"name":"Kannewurf R. Carl"},{"name":"Nakabayashi Ichiro"}],"ja":[{"name":"森賀 俊広"},{"name":"Edwards D. Doreen"},{"name":"Mason O. Thomas"},{"name":"Palmer B. George"},{"name":"Poeppelmeier R. Kenneth"},{"name":"Schindler L. Jon"},{"name":"Kannewurf R. Carl"},{"name":"中林 一朗"}]},"description":{"en":"酸化亜鉛-酸化インジウム系に現れるホモロガス化合物ZnkIn2Ok+3の生成組成領域，温度領域を明らかにした．そのホモロガス化合物が新しい透明導電性酸化物として有望であることを示し，特にZn3In2O6がバルクでも270S/cmの電気伝導率を有することを明らかにした．","ja":"酸化亜鉛-酸化インジウム系に現れるホモロガス化合物ZnkIn2Ok+3の生成組成領域，温度領域を明らかにした．そのホモロガス化合物が新しい透明導電性酸化物として有望であることを示し，特にZn3In2O6がバルクでも270S/cmの電気伝導率を有することを明らかにした．"},"publication_date":"1998-05-01","publication_name":{"en":"Journal of American Ceramic Society","ja":"Journal of American Ceramic Society"},"volume":"Vol.81","number":"No.5","starting_page":"1310","ending_page":"1316","languages":["eng"],"referee":true,"published_paper_type":"scientific_journal"},"priority":"input_data"}
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line:144, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=11931","label":"url"}],"paper_title":{"en":"Characterization of Oxygen-deficient Phases Appearing in Reduction of the Perovskite-type LaNiO3 to La2Ni2O5","ja":"Characterization of Oxygen-deficient Phases Appearing in Reduction of the Perovskite-type LaNiO3 to La2Ni2O5"},"authors":{"en":[{"name":"Moriga Toshihiro"},{"name":"Usaka Osamu"},{"name":"Nakabayashi Ichiro"},{"name":"Kinouchi Tsuneo"},{"name":"Kikkawa Shinichi"},{"name":"Kanamaru Fumikazu"}],"ja":[{"name":"森賀 俊広"},{"name":"Usaka Osamu"},{"name":"中林 一朗"},{"name":"Kinouchi Tsuneo"},{"name":"Kikkawa Shinichi"},{"name":"Kanamaru Fumikazu"}]},"description":{"en":"ペロブスカイト型LaNiO3からトポタクティックな還元によって生じるLa2Ni2O5への反応中間生成物である強磁性体相について，水素による還元ではなくAlを酸素ゲッターとした還元により単一相を合成することに成功しそれを評価した．その結晶は斜方晶系に属し，キュリー温度は約230Kで，組成はLa3Ni3O8と推定された．","ja":"ペロブスカイト型LaNiO3からトポタクティックな還元によって生じるLa2Ni2O5への反応中間生成物である強磁性体相について，水素による還元ではなくAlを酸素ゲッターとした還元により単一相を合成することに成功しそれを評価した．その結晶は斜方晶系に属し，キュリー温度は約230Kで，組成はLa3Ni3O8と推定された．"},"publication_date":"1995-10-01","publication_name":{"en":"Solid State Ionics","ja":"Solid State Ionics"},"volume":"Vol.79","number":"No.2","starting_page":"252","ending_page":"255","languages":["eng"],"referee":true,"identifiers":{"issn":["0167-2738"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:145, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=11932","label":"url"}],"paper_title":{"en":"XAFS Study on Debye-Waller Factor in Tetrahedrally Coordinated Binary Crystals","ja":"XAFS Study on Debye-Waller Factor in Tetrahedrally Coordinated Binary Crystals"},"authors":{"en":[{"name":"Yoshiasa Akira"},{"name":"Maeda Hironobu"},{"name":"Ishii Tadao"},{"name":"Emura Shuichi"},{"name":"Moriga Toshihiro"},{"name":"Koto Kichiro"}],"ja":[{"name":"Yoshiasa Akira"},{"name":"Maeda Hironobu"},{"name":"Ishii Tadao"},{"name":"Emura Shuichi"},{"name":"森賀 俊広"},{"name":"Koto Kichiro"}]},"description":{"en":"酸化亜鉛やヨウ化銀など4配位化合物に関して，EXAFS解析により得られるDebye-Waller因子と，X線回折法から得られる熱振動パラメータから，原子の(2体間)熱振動の相関性とイオン結合性の関係を明らかにした．イオン結合性が大きい程，極低温(23K)の平均自乗相対変位に対する室温(293K)の平均自乗相対変位の比は急激に大きくなることを示した．","ja":"酸化亜鉛やヨウ化銀など4配位化合物に関して，EXAFS解析により得られるDebye-Waller因子と，X線回折法から得られる熱振動パラメータから，原子の(2体間)熱振動の相関性とイオン結合性の関係を明らかにした．イオン結合性が大きい程，極低温(23K)の平均自乗相対変位に対する室温(293K)の平均自乗相対変位の比は急激に大きくなることを示した．"},"publication_date":"1995-07-01","publication_name":{"en":"Solid State Ionics","ja":"Solid State Ionics"},"volume":"Vol.78","number":"No.1","starting_page":"31","ending_page":"33","languages":["eng"],"referee":true,"identifiers":{"issn":["0167-2738"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:146, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=11945","label":"url"}],"paper_title":{"en":"Spectroscopic Study on Plate- and Sponge-type Raney Nickel Electrodes for Fuel Cell","ja":"Spectroscopic Study on Plate- and Sponge-type Raney Nickel Electrodes for Fuel Cell"},"authors":{"en":[{"name":"Nakabayashi Ichiro"},{"name":"Nagao Eiji"},{"name":"Miyata Kazuhisa"},{"name":"Moriga Toshihiro"},{"name":"Ashida Toshifumi"},{"name":"Tomida Tahei"},{"name":"Hyland M. M."},{"name":"Metson B. J."}],"ja":[{"name":"中林 一朗"},{"name":"Nagao Eiji"},{"name":"Miyata Kazuhisa"},{"name":"森賀 俊広"},{"name":"芦田 利文"},{"name":"冨田 太平"},{"name":"Hyland M. M."},{"name":"Metson B. J."}]},"description":{"en":"本論文は，メタノールやヒドラジンを用いた燃料電池用のアノード電極にスポンジ状のラネーニッケル触媒を用いることを検討したものである．プラズマ溶射法によってアルミニウムを被覆したスポンジ状ニッケル板から触媒電極を作成し，触媒の表面組織や結晶構造(XRD, EXAFS, XPS測定)と触媒活性，電極特性との関係を考察した．","ja":"本論文は，メタノールやヒドラジンを用いた燃料電池用のアノード電極にスポンジ状のラネーニッケル触媒を用いることを検討したものである．プラズマ溶射法によってアルミニウムを被覆したスポンジ状ニッケル板から触媒電極を作成し，触媒の表面組織や結晶構造(XRD, EXAFS, XPS測定)と触媒活性，電極特性との関係を考察した．"},"publication_date":"1995-05-01","publication_name":{"en":"Journal of Materials Chemistry","ja":"Journal of Materials Chemistry"},"volume":"Vol.5","number":"No.5","starting_page":"737","ending_page":"742","referee":true,"identifiers":{"doi":["10.1039/JM9950500737"],"issn":["0959-9428"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
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line:149, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=12407","label":"url"}],"paper_title":{"en":"Reduction of the Perovskite-type LnNiO3 (Ln=Pr, Nd) to Ln3Ni3O7 with monovalent nickel ions","ja":"Reduction of the Perovskite-type LnNiO3 (Ln=Pr, Nd) to Ln3Ni3O7 with monovalent nickel ions"},"authors":{"en":[{"name":"Moriga Toshihiro"},{"name":"Usaka Osamu"},{"name":"Nakabayashi Ichiro"},{"name":"Hirashima Yasushi"},{"name":"Kikkawa Shinichi"},{"name":"Kanamaru Fumikazu"}],"ja":[{"name":"森賀 俊広"},{"name":"Usaka Osamu"},{"name":"中林 一朗"},{"name":"平島 康"},{"name":"Kikkawa Shinichi"},{"name":"Kanamaru Fumikazu"}]},"description":{"en":"ペロブスカイト型LaNiO3の場合，トポタクティックな還元によりLa2Ni2O5まで還元することを明らかにしていたが，Laをイオン半径のより小さなPrやNdに置換することにより，還元がNd3Ni3O7まで進むことを示した．この化合物はニッケルの形式的な価数でも1.67とニッケル化合物では非常に珍しく，X線構造解析およびX線光電子分光法を用いて，ニッケルの価数が3価:1価=1:2に不均化していること，基本ペロブスカイト型の格子をもとにすれば3x1x3の構造をとることを明らかにした．","ja":"ペロブスカイト型LaNiO3の場合，トポタクティックな還元によりLa2Ni2O5まで還元することを明らかにしていたが，Laをイオン半径のより小さなPrやNdに置換することにより，還元がNd3Ni3O7まで進むことを示した．この化合物はニッケルの形式的な価数でも1.67とニッケル化合物では非常に珍しく，X線構造解析およびX線光電子分光法を用いて，ニッケルの価数が3価:1価=1:2に不均化していること，基本ペロブスカイト型の格子をもとにすれば3x1x3の構造をとることを明らかにした．"},"publication_date":"1994-12-01","publication_name":{"en":"Solid State Ionics","ja":"Solid State Ionics"},"volume":"Vol.74","starting_page":"211","ending_page":"217","languages":["eng"],"referee":true,"identifiers":{"issn":["0167-2738"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:150, {"insert":{"user_id":"1000038966","type":"published_papers","id":"30376438"},"force":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=12393","label":"url"}],"paper_title":{"en":"Synthesis of ZnO-Based Thin Films for Varistor by Metallic Alkoxide Method","ja":"Synthesis of ZnO-Based Thin Films for Varistor by Metallic Alkoxide Method"},"authors":{"en":[{"name":"Moriga Toshihiro"},{"name":"Umemoto Fusahide"},{"name":"Shima Kentaro"},{"name":"Ashida Toshifumi"},{"name":"Nakabayashi Ichiro"}],"ja":[{"name":"森賀 俊広"},{"name":"Umemoto Fusahide"},{"name":"Shima Kentaro"},{"name":"芦田 利文"},{"name":"中林 一朗"}]},"description":{"en":"金属アルコキシド法を用いて，ガラス基板へディップコーティングを行うことにより酸化亜鉛バリスタ薄膜を作製した．溶媒が2-プロパノールである金属アルコキシド溶液は，2,2'-イミノジエタノールを添加することにより安定性，製膜性が向上した．非オーミックな電流-電圧特性が，1073Kで48時間焼成し酸化亜鉛の粒成長を促すことによって発現した．","ja":"金属アルコキシド法を用いて，ガラス基板へディップコーティングを行うことにより酸化亜鉛バリスタ薄膜を作製した．溶媒が2-プロパノールである金属アルコキシド溶液は，2,2'-イミノジエタノールを添加することにより安定性，製膜性が向上した．非オーミックな電流-電圧特性が，1073Kで48時間焼成し酸化亜鉛の粒成長を促すことによって発現した．"},"publication_date":"1994-09-01","publication_name":{"en":"Surface Modification Technologies","ja":"Surface Modification Technologies"},"volume":"Vol.7","starting_page":"151","ending_page":"160","languages":["eng"],"referee":true,"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:151, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=12391","label":"url"}],"paper_title":{"en":"Synthesis, Crystal Structure, and Properties of Oxygen-Deficient Lanthanum Nickelate LaNiO3-x (0<x<0.5)","ja":"Synthesis, Crystal Structure, and Properties of Oxygen-Deficient Lanthanum Nickelate LaNiO3-x (0<x<0.5)"},"authors":{"en":[{"name":"Moriga Toshihiro"},{"name":"Usaka Osamu"},{"name":"Imamura Tomomi"},{"name":"Nakabayashi Ichiro"},{"name":"Matsubara Ichiro"},{"name":"Kinouchi Tsuneo"},{"name":"Kikkawa Shinichi"},{"name":"Kanamaru Fumikazu"}],"ja":[{"name":"森賀 俊広"},{"name":"Usaka Osamu"},{"name":"Imamura Tomomi"},{"name":"中林 一朗"},{"name":"Matsubara Ichiro"},{"name":"Kinouchi Tsuneo"},{"name":"Kikkawa Shinichi"},{"name":"Kanamaru Fumikazu"}]},"description":{"en":"ペロブスカイト型LaNiO3のトポタクティックな還元により生成する反強磁性体La2Ni2O5の結晶構造をX線リートベルト法により明らかにした．X線光電子分光法によりこのLa2Ni2O5中のNiは，3価と1価の状態に1:1に不均化していることを示した．また，このLaNiO3からLa2Ni2O5への還元途中に強磁性体相が出現することを見いだした．","ja":"ペロブスカイト型LaNiO3のトポタクティックな還元により生成する反強磁性体La2Ni2O5の結晶構造をX線リートベルト法により明らかにした．X線光電子分光法によりこのLa2Ni2O5中のNiは，3価と1価の状態に1:1に不均化していることを示した．また，このLaNiO3からLa2Ni2O5への還元途中に強磁性体相が出現することを見いだした．"},"publication_date":"1994-03-01","publication_name":{"en":"Bulletin of the Chemical Society of Japan","ja":"Bulletin of the Chemical Society of Japan"},"volume":"Vol.67","number":"No.3","starting_page":"687","ending_page":"693","languages":["eng"],"referee":true,"identifiers":{"issn":["0009-2673"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:152, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=12433","label":"url"}],"paper_title":{"en":"Crystal Structure of Basic calcium Carbonate and Its Decomposition Process in Water","ja":"Crystal Structure of Basic calcium Carbonate and Its Decomposition Process in Water"},"authors":{"en":[{"name":"Matsushita Isao"},{"name":"Hamada Yukitoshi"},{"name":"Suzuki Takashi"},{"name":"Nomura Yuji"},{"name":"Moriga Toshihiro"},{"name":"Ashida Toshifumi"},{"name":"Nakabayashi Ichiro"}],"ja":[{"name":"Matsushita Isao"},{"name":"Hamada Yukitoshi"},{"name":"Suzuki Takashi"},{"name":"Nomura Yuji"},{"name":"森賀 俊広"},{"name":"芦田 利文"},{"name":"中林 一朗"}]},"description":{"en":"塩基性炭酸カルシウムの結晶構造をX線回折法と制限視野電子線回折法を用いて決定した．また，その塩基性炭酸カルシウムの水中での分解挙動を検討した結果，分解生成物として水酸化カルシウム，カルサイトおよびアラゴナイトが生じることを示した．生成したカルサイトとアラゴナイトは，分解初期にCa2+イオンの水中への溶出により生成し，塩基性炭酸カルシウムに対し特定の方位を持って成長することが明らかになった．","ja":"塩基性炭酸カルシウムの結晶構造をX線回折法と制限視野電子線回折法を用いて決定した．また，その塩基性炭酸カルシウムの水中での分解挙動を検討した結果，分解生成物として水酸化カルシウム，カルサイトおよびアラゴナイトが生じることを示した．生成したカルサイトとアラゴナイトは，分解初期にCa2+イオンの水中への溶出により生成し，塩基性炭酸カルシウムに対し特定の方位を持って成長することが明らかになった．"},"publication_date":"1993-11-01","publication_name":{"en":"Journal of Ceramic Society of Japan","ja":"Journal of Ceramic Society of Japan"},"volume":"Vol.101","number":"No.12","starting_page":"1335","ending_page":"1339","languages":["eng"],"referee":true,"identifiers":{"issn":["0914-5400"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:153, {"insert":{"user_id":"1000038966","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=12390","label":"url"}],"paper_title":{"en":"Preparation and Superconductivity of the T*-type (PrGd0.8A0.2)CuOz Compounds (A=Ca, Sr)","ja":"Preparation and Superconductivity of the T*-type (PrGd0.8A0.2)CuOz Compounds (A=Ca, Sr)"},"authors":{"en":[{"name":"Moriga Toshihiro"},{"name":"Takemoto Shoichi"},{"name":"Tsukaguchi Hirokazu"},{"name":"Nakabayashi Ichiro"},{"name":"Koto Kichiro"}],"ja":[{"name":"森賀 俊広"},{"name":"Takemoto Shoichi"},{"name":"Tsukaguchi Hirokazu"},{"name":"中林 一朗"},{"name":"Koto Kichiro"}]},"description":{"en":"Cuイオンがピラミッド型5配位であるT*型PrGd0.8Sr{0.2}CuOzにおいて，300℃，7-10MPaの高酸素圧処理を施すことによりPrの価数は変化させることなくCuのみより高い原子価を持たせることに成功し，Tc=60-70Kの超伝導性を示すことを明らかにした．","ja":"Cuイオンがピラミッド型5配位であるT*型PrGd0.8Sr{0.2}CuOzにおいて，300℃，7-10MPaの高酸素圧処理を施すことによりPrの価数は変化させることなくCuのみより高い原子価を持たせることに成功し，Tc=60-70Kの超伝導性を示すことを明らかにした．"},"publication_date":"1993-08-01","publication_name":{"en":"Journal of Ceramic Society of Japan","ja":"Journal of Ceramic Society of Japan"},"volume":"Vol.101","number":"No.8","starting_page":"962","ending_page":"965","languages":["eng"],"referee":true,"identifiers":{"issn":["0914-5400"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
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line:269, {"insert":{"user_id":"1000038966","type":"presentations","id":"30376688"},"force":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=362986","label":"url"}],"presentation_title":{"en":"チタン酸リチウムにおける局所的な構造擾乱とリチウムイオンの運動状態","ja":"チタン酸リチウムにおける局所的な構造擾乱とリチウムイオンの運動状態"},"presenters":{"en":[{"name":"Nakamura Koichi"},{"name":"富本 健介"},{"name":"Inukai Munehiro"},{"name":"Moriga Toshihiro"},{"name":"桑田 直明"},{"name":"河村 純一"}],"ja":[{"name":"中村 浩一"},{"name":"富本 健介"},{"name":"犬飼 宗弘"},{"name":"森賀 俊広"},{"name":"桑田 直明"},{"name":"河村 純一"}]},"event":{"en":"日本物理学会2019年秋季大会 講演概要集","ja":"日本物理学会2019年秋季大会 講演概要集"},"publication_date":"2019-09-12","languages":["jpn"],"promoter":{"en":"The Physical Society of Japan","ja":"日本物理学会"},"location":{"en":"Gifu","ja":"岐阜"},"description":{"en":"リチウムイオン2次電池の負極材料としてのスピネル型チタン酸リチウム(LTO)はLiの挿入脱離反応において体積膨張率が小さいことからひずみの影響を受けにくくサイクル特性が良いとされるが，電子伝導性は高くなく伝導性向上のための取り組みが進められている．LTOにおける電気伝導挙動を明らかにするために，メカニカルミリング法を用いて結晶構造中に構造擾乱を誘起することで局所的に格子ひずみを導入し，局所構造の変化に対する伝導挙動の変化を電気伝導度測定と7Li-NMR測定の結果を議論した．ミリング処理によりXRDパターンは拡がり，回折強度の大きく減少したことからミリングにより結晶構造内にひずみなど擾乱が導入されたことが分かった．ミリングされた試料のstatic NMRスペクトルにはLi+イオンの運動状態を反映した2つのスペクトルが重畳して見られる．運動状態にあるLi+イオンの割合がミリング時間の増加にしたがい大きく増大することが分かった．ニオブ酸リチウムでは最大で10%程度のLi+イオンが運動状態に移るが，LTOでは10hミリングで20%程度のLi+イオンが運動状態にあると考えられる．","ja":"リチウムイオン2次電池の負極材料としてのスピネル型チタン酸リチウム(LTO)はLiの挿入脱離反応において体積膨張率が小さいことからひずみの影響を受けにくくサイクル特性が良いとされるが，電子伝導性は高くなく伝導性向上のための取り組みが進められている．LTOにおける電気伝導挙動を明らかにするために，メカニカルミリング法を用いて結晶構造中に構造擾乱を誘起することで局所的に格子ひずみを導入し，局所構造の変化に対する伝導挙動の変化を電気伝導度測定と7Li-NMR測定の結果を議論した．ミリング処理によりXRDパターンは拡がり，回折強度の大きく減少したことからミリングにより結晶構造内にひずみなど擾乱が導入されたことが分かった．ミリングされた試料のstatic NMRスペクトルにはLi+イオンの運動状態を反映した2つのスペクトルが重畳して見られる．運動状態にあるLi+イオンの割合がミリング時間の増加にしたがい大きく増大することが分かった．ニオブ酸リチウムでは最大で10%程度のLi+イオンが運動状態に移るが，LTOでは10hミリングで20%程度のLi+イオンが運動状態にあると考えられる．"},"is_international_presentation":false},"priority":"input_data"}
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line:310, {"insert":{"user_id":"1000038966","type":"presentations","id":"30376729"},"force":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=341697","label":"url"}],"presentation_title":{"en":"Na系遷移金属酸化物における局所構造とNa+イオンの運動状態","ja":"Na系遷移金属酸化物における局所構造とNa+イオンの運動状態"},"presenters":{"en":[{"name":"Nakamura Koichi"},{"name":"Takeuchi Satoshi"},{"name":"Inukai Munehiro"},{"name":"Kawasaki Yu"},{"name":"Moriga Toshihiro"}],"ja":[{"name":"中村 浩一"},{"name":"竹内 智史"},{"name":"犬飼 宗弘"},{"name":"川崎 祐"},{"name":"森賀 俊広"}]},"event":{"en":"日本物理学会2017年秋季大会 講演概要集","ja":"日本物理学会2017年秋季大会 講演概要集"},"publication_date":"2017-09-21","languages":["jpn"],"promoter":{"en":"The Physical Society of Japan","ja":"日本物理学会"},"location":{"en":"岩手","ja":"岩手"},"description":{"en":"NaxCoO2をはじめとする層状酸化物は，リチウムイオン二次電池に代わる次世代型二次電池の正極材料として注目され，近年活発に研究されている．NaxCoO2におけるイオンの運動状態に着目し，電気伝導度測定やNMR(核磁気共鳴)法を用いた23Naにおけるスピン-格子緩和時間T1の結果から，Na+イオンの運動状態や局所構造について議論した．250K以下での23Na-NMR スペクトルは1本の中心線を示すが，室温以上ではCo副格子の局所的な変化にともなう電場勾配の変化の影響で四重極相互作用の2次の粉末図形スペクトルを示したが，700Kまでの高温度域でもスペクトルの先鋭化は見られなかった．NaxCrO2の電気伝導度における活性化エネルギーはNa組成に依存し0.7∼1eVと見積もられ，NaxCoO2(∼0.4eV)に比べ大きい．NaxCrO2の四重極相互作用はNaxCoO2より小さく，四重極相互作用の1次の粉末図形が観測された．","ja":"NaxCoO2をはじめとする層状酸化物は，リチウムイオン二次電池に代わる次世代型二次電池の正極材料として注目され，近年活発に研究されている．NaxCoO2におけるイオンの運動状態に着目し，電気伝導度測定やNMR(核磁気共鳴)法を用いた23Naにおけるスピン-格子緩和時間T1の結果から，Na+イオンの運動状態や局所構造について議論した．250K以下での23Na-NMR スペクトルは1本の中心線を示すが，室温以上ではCo副格子の局所的な変化にともなう電場勾配の変化の影響で四重極相互作用の2次の粉末図形スペクトルを示したが，700Kまでの高温度域でもスペクトルの先鋭化は見られなかった．NaxCrO2の電気伝導度における活性化エネルギーはNa組成に依存し0.7∼1eVと見積もられ，NaxCoO2(∼0.4eV)に比べ大きい．NaxCrO2の四重極相互作用はNaxCoO2より小さく，四重極相互作用の1次の粉末図形が観測された．"},"is_international_presentation":false},"priority":"input_data"}
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line:327, {"insert":{"user_id":"1000038966","type":"presentations","id":"30376746"},"force":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=324864","label":"url"}],"presentation_title":{"en":"LiMPO4(M=Fe, Mn, Co)における高温でのイオン運動と局所構造の変化","ja":"LiMPO4(M=Fe, Mn, Co)における高温でのイオン運動と局所構造の変化"},"presenters":{"en":[{"name":"Ito Hiroaki"},{"name":"Inukai Munehiro"},{"name":"Moriga Toshihiro"},{"name":"岩井 良樹"},{"name":"桑田 直明"},{"name":"河村 純一"},{"name":"Nakamura Koichi"}],"ja":[{"name":"井藤 弘章"},{"name":"犬飼 宗弘"},{"name":"森賀 俊広"},{"name":"岩井 良樹"},{"name":"桑田 直明"},{"name":"河村 純一"},{"name":"中村 浩一"}]},"event":{"en":"第42回固体イオニクス討論会","ja":"第42回固体イオニクス討論会"},"publication_date":"2016-12-06","languages":["jpn"],"promoter":{"en":"固体イオニクス学会","ja":"固体イオニクス学会"},"location":{"en":"Nagoya","ja":"名古屋"},"description":{"en":"Olivine type lithium iron phosphates have been studied as a cathode material for lithium ion secondary batteries. The NMR line widths and spin-lattice relaxation time T1 of 7Li nucleus in LiFePO4 changed from 550K to 700K, while those of LiMnPO4 and LiCoPO4 did not show the remarkable temperature dependence. The peak broadening of XRD pattern of LiFePO4 at high temperatures suggests that the crystal structure around Li sites becomes locally disordered. It is considered that these situations would stimulate Li+ ion dynamics related to changes of the NMR line width and T1 at high temperatures.","ja":"現在までコバルト酸リチウム(LiCoO2)が主に正極材料として用いられてきたが，価格，安全性，コバルトの安定供給などの面から，様々な代替材料の開発が進められている．共有結合に基づくPO4四面体を母構造に持つオリビン型リン酸鉄リチウム(LiFePO4)などは，車載用の大容量・高電圧のリチウムイオン2次電池の電極材料として精力的に研究されている．本研究では，LiFePO4，LiMnPO4，LiCoPO4の3つのオリビン型遷移金属リン酸リチウムに着目し，核磁気共鳴によるスペクトルおよび緩和時間測定の結果から，これらの局所的な構造とLi+イオンの運動状態について議論した．室温以上では，LiMnPO4は700Kまで大きな変化は見られずほぼ一定のT1を示すが，LiFePO4では線幅の温度変化と同様に550K以上で変化が見られることから，このT1の増大はLi+イオンの運動状態に関係していると考えられた．"},"is_international_presentation":false},"priority":"input_data"}
line:328, {"insert":{"user_id":"1000038966","type":"presentations","id":"30376747"},"force":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=324861","label":"url"}],"presentation_title":{"en":"NaCoO2のNa組成とNaサイト周辺の局所構造","ja":"NaCoO2のNa組成とNaサイト周辺の局所構造"},"presenters":{"en":[{"name":"Nakamura Koichi"},{"name":"Takeuchi Satoshi"},{"name":"Inukai Munehiro"},{"name":"Moriga Toshihiro"}],"ja":[{"name":"中村 浩一"},{"name":"竹内 智史"},{"name":"犬飼 宗弘"},{"name":"森賀 俊広"}]},"event":{"en":"日本物理学会2016年秋季大会 講演概要集","ja":"日本物理学会2016年秋季大会 講演概要集"},"publication_date":"2016-09-13","languages":["jpn"],"promoter":{"en":"The Physical Society of Japan","ja":"日本物理学会"},"location":{"en":"Kanazawa","ja":"金沢"},"description":{"en":"NaxCoO2をはじめとする層状酸化物は，リチウムイオン二次電池に代わる次世代型二次電池の正極材料として注目され，近年活発に研究されている．NaxCoO2におけるイオンの運動状態に着目し，電気伝導度測定やNMR(核磁気共鳴)法を用いた23Naにおけるスピン-格子緩和時間T1の結果から，Na+イオンの運動状態や局所構造について議論した．250K以下での23Na-NMR スペクトルは1本の中心線を示すが，室温以上ではCo副格子の局所的な変化にともなう電場勾配の変化の影響で四重極相互作用の2次の粉末図形スペクトルを示した．室温以上700Kまでの高温度域でもスペクトルの先鋭化は見られず，四重極周波数は温度の上昇にともなって徐々に増大した．","ja":"NaxCoO2をはじめとする層状酸化物は，リチウムイオン二次電池に代わる次世代型二次電池の正極材料として注目され，近年活発に研究されている．NaxCoO2におけるイオンの運動状態に着目し，電気伝導度測定やNMR(核磁気共鳴)法を用いた23Naにおけるスピン-格子緩和時間T1の結果から，Na+イオンの運動状態や局所構造について議論した．250K以下での23Na-NMR スペクトルは1本の中心線を示すが，室温以上ではCo副格子の局所的な変化にともなう電場勾配の変化の影響で四重極相互作用の2次の粉末図形スペクトルを示した．室温以上700Kまでの高温度域でもスペクトルの先鋭化は見られず，四重極周波数は温度の上昇にともなって徐々に増大した．"},"is_international_presentation":false},"priority":"input_data"}
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