=== Generating (published_papers) ===
=== Generating (research_interests) ===
=== Generating (education) ===
=== Generating (research_experience) ===
=== Generating (misc) ===
=== Generating (research_projects) ===
=== Generating (books_etc) ===
=== Generating (industrial_property_rights) ===
=== Generating (awards) ===
EID=318377 is rejected. (Reason: 賞名が登録されていません．)
EID=318377 is rejected. (Reason: 賞名が登録されていません．)
=== Generating (association_memberships) ===
=== Generating (teaching_experience) ===
=== Generating (committee_memberships) ===
=== Generating (presentations) ===
EID=339998 is rejected. (Reason: タイトルが登録されていません．)
EID=339998 is rejected. (Reason: タイトルが登録されていません．)
==== begin registerFile(/WWW/pub2/data/ERD/person/262684/researchmap/published_papers.jsonl) ====
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line:2, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=407537","label":"url"}],"paper_title":{"en":"Development of 1,3a,6a-triazapentalene derivatives as practical erasable fluorescent cell staining reagents.","ja":"Development of 1,3a,6a-triazapentalene derivatives as practical erasable fluorescent cell staining reagents."},"authors":{"en":[{"name":"Yuna Kondo"},{"name":"Tenta Nakamura"},{"name":"Daisuke Tsuji"},{"name":"Sato Ryota"},{"name":"Karanjit Sangita"},{"name":"Reiko Akagi"},{"name":"Namba Kosuke"}],"ja":[{"name":"近藤 優奈"},{"name":"中村 天太"},{"name":"Daisuke Tsuji"},{"name":"佐藤 亮太"},{"name":"カランジット サンギータ"},{"name":"Reiko Akagi"},{"name":"難波 康祐"}]},"publication_date":"2024-02-28","publication_name":{"en":"Tetrahedron Letters","ja":"Tetrahedron Letters"},"volume":"Vol.138","starting_page":"154986","ending_page":"154986","languages":["eng"],"referee":true,"identifiers":{"issn":["0040-4039"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:3, {"insert":{"user_id":"5000093573","type":"published_papers","id":"46285541"},"force":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=407535","label":"url"}],"paper_title":{"en":"Inactivation of siderophore iron-chelating moieties by the fungal wheat root symbiont Pyrenophore biseptata","ja":"Inactivation of siderophore iron-chelating moieties by the fungal wheat root symbiont Pyrenophore biseptata"},"authors":{"en":[{"name":"K. S. French"},{"name":"E. Chukwuma"},{"name":"I. Linshitz"},{"name":"Namba Kosuke"},{"name":"O. W. Duckworth"},{"name":"M. A. Cubeta"},{"name":"O. Baars"}],"ja":[{"name":"K. S. French"},{"name":"E. Chukwuma"},{"name":"I. Linshitz"},{"name":"難波 康祐"},{"name":"O. W. Duckworth"},{"name":"M. A. Cubeta"},{"name":"O. Baars"}]},"publication_date":"2024-01-19","publication_name":{"en":"Environmental Microbiology Reports","ja":"Environmental Microbiology Reports"},"starting_page":"e13234","ending_page":"e13234","languages":["eng"],"referee":true,"identifiers":{"issn":["1758-2229"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:4, {"insert":{"user_id":"5000093573","type":"published_papers","id":"46285542"},"force":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=407531","label":"url"}],"paper_title":{"en":"A Simple and Powerful tert-Butylation of Carboxylic Acids and Alcohols","ja":"A Simple and Powerful tert-Butylation of Carboxylic Acids and Alcohols"},"authors":{"en":[{"name":"Chie Ogasa"},{"name":"Kimika Kayano"},{"name":"Namba Kosuke"}],"ja":[{"name":"小笠千恵"},{"name":"茅野 公佳"},{"name":"難波 康祐"}]},"publication_date":"2024","publication_name":{"en":"Synlett","ja":"Synlett"},"volume":"Vol.35","starting_page":"235","ending_page":"239","languages":["eng"],"referee":true,"identifiers":{"issn":["0936-5214"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:5, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://repo.lib.tokushima-u.ac.jp/ja/118228","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=396502","label":"url"}],"paper_title":{"en":"A suitable stereoisomer of vibrioferrin probes for iron uptake of Vibrio parahaemolyticus","ja":"A suitable stereoisomer of vibrioferrin probes for iron uptake of Vibrio parahaemolyticus"},"authors":{"en":[{"name":"Sumida Ryuichi"},{"name":"Okuda Misa"},{"name":"Mera Akane"},{"name":"Inoue Masaki"},{"name":"Karanjit Sangita"},{"name":"Niwa Kanji"},{"name":"Tsutsumi Tomohiro"},{"name":"Sato Ryota"},{"name":"Nakayama Atsushi"},{"name":"Tanaka Naonobu"},{"name":"Oda Masataka"},{"name":"Namba Kosuke"}],"ja":[{"name":"住田 龍一"},{"name":"奥田 実沙"},{"name":"米良 茜"},{"name":"井上 雅貴"},{"name":"カランジット サンギータ"},{"name":"丹羽 莞慈"},{"name":"堤 大洋"},{"name":"佐藤 亮太"},{"name":"中山 淳"},{"name":"田中 直伸"},{"name":"Oda Masataka"},{"name":"難波 康祐"}]},"publication_date":"2023-05-08","publication_name":{"en":"Chemistry Letters","ja":"Chemistry Letters"},"languages":["eng"],"referee":true,"identifiers":{"doi":["10.1246/cl.230166"],"issn":["1348-0715"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:6, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://repo.lib.tokushima-u.ac.jp/ja/118227","label":"url"},{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/36813913","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=396501","label":"url"}],"paper_title":{"en":"1,3a,6a-Triazapentalene derivatives as photo-induced cytotoxic small fluorescent dyes","ja":"1,3a,6a-Triazapentalene derivatives as photo-induced cytotoxic small fluorescent dyes"},"authors":{"en":[{"name":"Tsuji Daisuke"},{"name":"Nakayama Atsushi"},{"name":"Yamamoto RIko"},{"name":"Nagano Shuji"},{"name":"Taniguchi Takashi"},{"name":"Sato Ryota"},{"name":"Karanjit Sangita"},{"name":"Muguruma Naoki"},{"name":"Takayama Tetsuji"},{"name":"Itoh Kohji"},{"name":"Namba Kosuke"}],"ja":[{"name":"Tsuji Daisuke"},{"name":"中山 淳"},{"name":"山本 璃子"},{"name":"長野 秀嗣"},{"name":"谷口 喬"},{"name":"佐藤 亮太"},{"name":"カランジット サンギータ"},{"name":"六車 直樹"},{"name":"高山 哲治"},{"name":"Itoh Kohji"},{"name":"難波 康祐"}]},"description":{"en":"1,3a,6a-Triazapentalene (TAP) is a compact fluorescent chromophore whose fluorescence properties vary greatly depending on the substituents on the TAP ring. This study investigated the photo-induced cytotoxicities of various TAP derivatives. Among the derivatives, 2-p-nitrophenyl-TAP showed significant cytotoxicity to HeLa cells under UV irradiation but no cytotoxicity without UV. In addition, the photo-induced cytotoxicity of 2-p-nitirophenyl-TAP was found to be cancer cell selective and effective against HeLa cells and HCT 116 cells. Under UV irradiation, 2-p-nitrophenyl-TAP generated reactive oxygen species (ROS) that induced an apoptosis and ferroptosis in cancer cells. Therefore, it was revealed that 2-p-nitrophenyl-TAP is the most compact dye that can generate ROS by photoirradiation.","ja":"1,3a,6a-Triazapentalene (TAP) is a compact fluorescent chromophore whose fluorescence properties vary greatly depending on the substituents on the TAP ring. This study investigated the photo-induced cytotoxicities of various TAP derivatives. Among the derivatives, 2-p-nitrophenyl-TAP showed significant cytotoxicity to HeLa cells under UV irradiation but no cytotoxicity without UV. In addition, the photo-induced cytotoxicity of 2-p-nitirophenyl-TAP was found to be cancer cell selective and effective against HeLa cells and HCT 116 cells. Under UV irradiation, 2-p-nitrophenyl-TAP generated reactive oxygen species (ROS) that induced an apoptosis and ferroptosis in cancer cells. Therefore, it was revealed that 2-p-nitrophenyl-TAP is the most compact dye that can generate ROS by photoirradiation."},"publication_date":"2023-02-22","publication_name":{"en":"Communications Chemistry","ja":"Communications Chemistry"},"volume":"Vol.6","number":"No.1","starting_page":"37","ending_page":"37","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1038/s42004-023-00838-0"],"issn":["2399-3669"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:7, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://repo.lib.tokushima-u.ac.jp/ja/118226","label":"url"},{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/36424382","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=396500","label":"url"}],"paper_title":{"en":"Uptake mechanism of iron-phytosiderophore from the soil based on the structure of yellow stripe transporter","ja":"Uptake mechanism of iron-phytosiderophore from the soil based on the structure of yellow stripe transporter"},"authors":{"en":[{"name":"Yamagata Atsushi"},{"name":"Murata Yoshiko"},{"name":"Namba Kosuke"},{"name":"Terada Tohru"},{"name":"Fukai Shuya"},{"name":"Shirouzu Mikako"}],"ja":[{"name":"Yamagata Atsushi"},{"name":"Murata Yoshiko"},{"name":"難波 康祐"},{"name":"Terada Tohru"},{"name":"Fukai Shuya"},{"name":"Shirouzu Mikako"}]},"description":{"en":"Calcareous soils cover one-third of all land and cause severe growth defects in plants due to the poor water solubility of iron at high pH. Poaceae species use a unique chelation strategy, whereby plants secrete a high-affinity metal chelator, known as phytosiderophores (mugineic acids), and reabsorb the iron-phytosiderophore complex by the yellow stripe 1/yellow stripe 1-like (YS1/YSL) transporter for efficient uptake of iron from the soil. Here, we present three cryo-electron microscopy structures of barley YS1 (HvYS1) in the apo state, in complex with an iron-phytosiderophore complex, Fe(III)-deoxymugineic acid (Fe(III)-DMA), and in complex with the iron-bound synthetic DMA analog (Fe(III)-PDMA). The structures reveal a homodimeric assembly mediated through an anti-parallel β-sheet interaction with cholesterol hemisuccinate. Each protomer adopts an outward open conformation, and Fe(III)-DMA is bound near the extracellular space in the central cavity. Fe(III)-PDMA occupies the same binding site as Fe(III)-DMA, demonstrating that PDMA can function as a potent fertilizer in an essentially identical manner to DMA. Our results provide a structural framework for iron-phytosiderophore recognition and transport by YS1/YSL transporters, which will enable the rational design of new, high-potency fertilizers.","ja":"Calcareous soils cover one-third of all land and cause severe growth defects in plants due to the poor water solubility of iron at high pH. Poaceae species use a unique chelation strategy, whereby plants secrete a high-affinity metal chelator, known as phytosiderophores (mugineic acids), and reabsorb the iron-phytosiderophore complex by the yellow stripe 1/yellow stripe 1-like (YS1/YSL) transporter for efficient uptake of iron from the soil. Here, we present three cryo-electron microscopy structures of barley YS1 (HvYS1) in the apo state, in complex with an iron-phytosiderophore complex, Fe(III)-deoxymugineic acid (Fe(III)-DMA), and in complex with the iron-bound synthetic DMA analog (Fe(III)-PDMA). The structures reveal a homodimeric assembly mediated through an anti-parallel β-sheet interaction with cholesterol hemisuccinate. Each protomer adopts an outward open conformation, and Fe(III)-DMA is bound near the extracellular space in the central cavity. Fe(III)-PDMA occupies the same binding site as Fe(III)-DMA, demonstrating that PDMA can function as a potent fertilizer in an essentially identical manner to DMA. Our results provide a structural framework for iron-phytosiderophore recognition and transport by YS1/YSL transporters, which will enable the rational design of new, high-potency fertilizers."},"publication_date":"2022-11-23","publication_name":{"en":"Nature Communications","ja":"Nature Communications"},"volume":"Vol.13","number":"No.1","starting_page":"7180","ending_page":"7180","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1038/s41467-022-34930-1"],"issn":["2041-1723"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:8, {"insert":{"user_id":"5000093573","type":"published_papers","id":"39594898"},"force":{"see_also":[{"@id":"https://repo.lib.tokushima-u.ac.jp/ja/117329","label":"url"},{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/35446586","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=388689","label":"url"}],"paper_title":{"en":"Total synthesis of proposed structures of 4,10-dihydroxy 8,12-guaianolides","ja":"Total synthesis of proposed structures of 4,10-dihydroxy 8,12-guaianolides"},"authors":{"en":[{"name":"Kimura Yuki"},{"name":"Ohashi Eisaku"},{"name":"Karanjit Sangita"},{"name":"Taniguchi Takashi"},{"name":"Nakayama Atsushi"},{"name":"Imagawa Hiroshi"},{"name":"Sato Ryota"},{"name":"Namba Kosuke"}],"ja":[{"name":"木村 有希"},{"name":"Ohashi Eisaku"},{"name":"カランジット サンギータ"},{"name":"谷口 喬"},{"name":"中山 淳"},{"name":"Imagawa Hiroshi"},{"name":"佐藤 亮太"},{"name":"難波 康祐"}]},"description":{"en":"The first total syntheses of two 4,10-dihydroxy-8,12-guaianolides that were reported to be natural products were achieved. Toward the syntheses of a collection of related guaianolides, the typical 5,7-fused system of 8,12-guaianolides was constructed by a ring expansion reaction of a hydroxylated coronafacic acid analogue that can be practically synthesized and optically resolved. The total syntheses of these compounds revealed that the previously reported structures of both natural products were incorrect.","ja":"The first total syntheses of two 4,10-dihydroxy-8,12-guaianolides that were reported to be natural products were achieved. Toward the syntheses of a collection of related guaianolides, the typical 5,7-fused system of 8,12-guaianolides was constructed by a ring expansion reaction of a hydroxylated coronafacic acid analogue that can be practically synthesized and optically resolved. The total syntheses of these compounds revealed that the previously reported structures of both natural products were incorrect."},"publication_date":"2022-04-22","publication_name":{"en":"Organic Letters","ja":"Organic Letters"},"volume":"Vol.24","number":"No.17","starting_page":"3297","ending_page":"3301","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1021/acs.orglett.2c01215"],"issn":["1523-7052"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:9, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=388688","label":"url"}],"paper_title":{"en":"A heterogeneous bifunctional silica-supported Ag2O/Im+Cl- catalyst for efficient CO2 conversion","ja":"A heterogeneous bifunctional silica-supported Ag2O/Im+Cl- catalyst for efficient CO2 conversion"},"authors":{"en":[{"name":"Karanjit Sangita"},{"name":"Tanaka Emiko"},{"name":"Shrestha K. L."},{"name":"Nakayama Atsushi"},{"name":"Ariga Katsuhiko"},{"name":"Namba Kosuke"}],"ja":[{"name":"カランジット サンギータ"},{"name":"田中 瑛実子"},{"name":"Shrestha K. L."},{"name":"中山 淳"},{"name":"Ariga Katsuhiko"},{"name":"難波 康祐"}]},"publication_date":"2022-03-08","publication_name":{"en":"Catalysis Science & Technology","ja":"Catalysis Science & Technology"},"volume":"Vol.12","starting_page":"3297","ending_page":"3301","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1039/D2CY00194B"],"issn":["2044-4761"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:10, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://repo.lib.tokushima-u.ac.jp/ja/116279","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=381696","label":"url"}],"paper_title":{"en":"Efficient construction of the hexacyclic ring core of palau'amine: the pKa concept for proceeding with unfavorable equilibrium reactions","ja":"Efficient construction of the hexacyclic ring core of palau'amine: the pKa concept for proceeding with unfavorable equilibrium reactions"},"authors":{"en":[{"name":"Ohashi Eisaku"},{"name":"Karanjit Sangita"},{"name":"Nakayama Atsushi"},{"name":"Takeuchi Kohei"},{"name":"Emam E Sherif"},{"name":"ANDO Hidenori"},{"name":"Ishida Tatsuhiro"},{"name":"Namba Kosuke"}],"ja":[{"name":"大橋 栄作"},{"name":"カランジット サンギータ"},{"name":"中山 淳"},{"name":"竹内 公平"},{"name":"Sherif Emam Abdallah Emam"},{"name":"安藤 英紀"},{"name":"石田 竜弘"},{"name":"難波 康祐"}]},"publication_date":"2021-08-11","publication_name":{"en":"Chemical Science","ja":"Chemical Science"},"volume":"Vol.12","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1039/D1SC03260G"],"issn":["2041-6539"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:11, {"insert":{"user_id":"5000093573","type":"published_papers","id":"33172809"},"force":{"see_also":[{"@id":"https://repo.lib.tokushima-u.ac.jp/ja/116179","label":"url"},{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-85107022552&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=377108","label":"url"}],"paper_title":{"en":"Development of a novel antioxidant based on a dimeric dihydroisocoumarin derivative","ja":"Development of a novel antioxidant based on a dimeric dihydroisocoumarin derivative"},"authors":{"en":[{"name":"Nakayama Atsushi"},{"name":"Nakamura Tenta"},{"name":"Ara Tabassum"},{"name":"fukuta tatsuya"},{"name":"Karanjit Sangita"},{"name":"Harada Takeshi"},{"name":"Oda Asuka"},{"name":"Sato Hideo"},{"name":"Abe Masahiro"},{"name":"Kogure Kentaro"},{"name":"Namba Kosuke"}],"ja":[{"name":"中山 淳"},{"name":"中村 天太"},{"name":"Tabassum Ara"},{"name":"fukuta tatsuya"},{"name":"カランジット サンギータ"},{"name":"原田 武志"},{"name":"小田 明日香"},{"name":"佐藤 次朗"},{"name":"安倍 正博"},{"name":"小暮 健太朗"},{"name":"難波 康祐"}]},"publication_date":"2021-06-22","publication_name":{"en":"Tetrahedron Letters","ja":"Tetrahedron Letters"},"volume":"Vol.74","starting_page":"153176","ending_page":"153176","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1016/j.tetlet.2021.153176"],"issn":["0040-4039"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:12, {"insert":{"user_id":"5000093573","type":"published_papers","id":"33397488"},"force":{"see_also":[{"@id":"https://repo.lib.tokushima-u.ac.jp/ja/116178","label":"url"},{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/33692352","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=380093","label":"url"}],"paper_title":{"en":"Development of a mugineic acid family phytosiderophore analog as an iron fertilizer","ja":"Development of a mugineic acid family phytosiderophore analog as an iron fertilizer"},"authors":{"en":[{"name":"Suzuki Motofumi"},{"name":"Urabe Atsumi"},{"name":"Sasaki Sayaka"},{"name":"Tsugawa Ryo"},{"name":"Nishio Satoshi"},{"name":"Mukaiyama Haruka"},{"name":"Murata Yoshiko"},{"name":"Masuda Hiroshi"},{"name":"Aung Sann M."},{"name":"Mera Akane"},{"name":"Takeuchi Masaki"},{"name":"Fukushima Keijo"},{"name":"Kanaki Michika"},{"name":"Kobayashi Kaori"},{"name":"Chiba Yudai"},{"name":"Shrestha Babu Binod"},{"name":"Nakanishi Hiromi"},{"name":"Watanabe T."},{"name":"Nakayama Atsushi"},{"name":"Fujino Hiromichi"},{"name":"Kobayashi Takanori"},{"name":"Tanino Keiji"},{"name":"Nishizawa Naoko"},{"name":"Namba Kosuke"}],"ja":[{"name":"Suzuki Motofumi"},{"name":"占部 敦美"},{"name":"笹木 清加"},{"name":"津川 稜"},{"name":"西尾 賢"},{"name":"向山 はるか"},{"name":"Murata Yoshiko"},{"name":"Masuda Hiroshi"},{"name":"Aung Sann M."},{"name":"米良 茜"},{"name":"竹内 政樹"},{"name":"福島 圭穣"},{"name":"Kanaki Michika"},{"name":"Kobayashi Kaori"},{"name":"Chiba Yudai"},{"name":"Shrestha Babu Binod"},{"name":"Nakanishi Hiromi"},{"name":"Watanabe T."},{"name":"中山 淳"},{"name":"藤野 裕道"},{"name":"Kobayashi Takanori"},{"name":"Tanino Keiji"},{"name":"Nishizawa Naoko"},{"name":"難波 康祐"}]},"description":{"en":"Iron (Fe) is an essential nutrient, but is poorly bioavailable because of its low solubility in alkaline soils; this leads to reduced agricultural productivity. To overcome this problem, we first showed that the soil application of synthetic 2'-deoxymugineic acid, a natural phytosiderophore from the Poaceae, can recover Fe deficiency in rice grown in calcareous soil. However, the high cost and poor stability of synthetic 2'-deoxymugineic acid preclude its agricultural use. In this work, we develop a more stable and less expensive analog, proline-2'-deoxymugineic acid, and demonstrate its practical synthesis and transport of its Fe-chelated form across the plasma membrane by Fe(III)·2'-deoxymugineic acid transporters. Possibility of its use as an iron fertilizer on alkaline soils is supported by promotion of rice growth in a calcareous soil by soil application of metal free proline-2'-deoxymugineic acid.","ja":"Iron (Fe) is an essential nutrient, but is poorly bioavailable because of its low solubility in alkaline soils; this leads to reduced agricultural productivity. To overcome this problem, we first showed that the soil application of synthetic 2'-deoxymugineic acid, a natural phytosiderophore from the Poaceae, can recover Fe deficiency in rice grown in calcareous soil. However, the high cost and poor stability of synthetic 2'-deoxymugineic acid preclude its agricultural use. In this work, we develop a more stable and less expensive analog, proline-2'-deoxymugineic acid, and demonstrate its practical synthesis and transport of its Fe-chelated form across the plasma membrane by Fe(III)·2'-deoxymugineic acid transporters. Possibility of its use as an iron fertilizer on alkaline soils is supported by promotion of rice growth in a calcareous soil by soil application of metal free proline-2'-deoxymugineic acid."},"publication_date":"2021-03-10","publication_name":{"en":"Nature Communications","ja":"Nature Communications"},"volume":"Vol.12","number":"No.1","starting_page":"1558","ending_page":"1558","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1038/s41467-021-21837-6"],"issn":["2041-1723"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:13, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://repo.lib.tokushima-u.ac.jp/ja/116742","label":"url"},{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/33334885","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=381727","label":"url"}],"paper_title":{"en":"Iron uptake mediated by the plant-derived chelator nicotianamine in the small intestine","ja":"Iron uptake mediated by the plant-derived chelator nicotianamine in the small intestine"},"authors":{"en":[{"name":"Murata Yoshiko"},{"name":"Yoshida Masami"},{"name":"Sakamoto Naho"},{"name":"Morimoto Shiho"},{"name":"Watanabe Takehiro"},{"name":"Namba Kosuke"}],"ja":[{"name":"Murata Yoshiko"},{"name":"Yoshida Masami"},{"name":"Sakamoto Naho"},{"name":"Morimoto Shiho"},{"name":"Watanabe Takehiro"},{"name":"難波 康祐"}]},"description":{"en":"Iron is an essential metal for all living organisms that is absorbed in the intestinal cells as a heme-chelated or free form. It is unclear how important plant-derived chelators, such as nicotianamine (NA), an organic small molecule that is ubiquitous in crops, vegetables, and various other foods, contribute to iron bioavailability in mammals. We performed electrophysiological assays with Xenopus laevis oocytes and radioactive tracer experiments with Caco-2 cells. The findings revealed that the proton-coupled amino acid transporter SLC36A1 (PAT1) transports iron in the form of NA-Fe (II) complex in vitro. Decreased expression of hPAT1 by RNA interference in Caco-2 cells reduced the uptake of NA-Fe (II) complex. The uptake of inorganic Fe (II) was relatively unaffected. These results imply that PAT1 transports iron as a NA-Fe (II) complex. The rate of Fe absorption in the spleen, liver, and kidney was higher when mice were orally administered NA-Fe (II) compared with free Fe (II). The profile of site-specific PAT1 expression in the mouse intestine coincided with those of NA and iron contents, which were the highest in the proximal jejunum. Orally administered NA-Fe (II) complex in mice was detected in the proximal jejunum by thin layer chromatography. In contrast, much less Fe (or NA) was detected in the duodenum, where the divalent metal transporter SLC11A2 (DMT1) absorbs free Fe (II). The collective results revealed the role of PAT1 in NA-Fe (II) absorption in the intestine and potential implication of NA in iron uptake in mammals.","ja":"Iron is an essential metal for all living organisms that is absorbed in the intestinal cells as a heme-chelated or free form. It is unclear how important plant-derived chelators, such as nicotianamine (NA), an organic small molecule that is ubiquitous in crops, vegetables, and various other foods, contribute to iron bioavailability in mammals. We performed electrophysiological assays with Xenopus laevis oocytes and radioactive tracer experiments with Caco-2 cells. The findings revealed that the proton-coupled amino acid transporter SLC36A1 (PAT1) transports iron in the form of NA-Fe (II) complex in vitro. Decreased expression of hPAT1 by RNA interference in Caco-2 cells reduced the uptake of NA-Fe (II) complex. The uptake of inorganic Fe (II) was relatively unaffected. These results imply that PAT1 transports iron as a NA-Fe (II) complex. The rate of Fe absorption in the spleen, liver, and kidney was higher when mice were orally administered NA-Fe (II) compared with free Fe (II). The profile of site-specific PAT1 expression in the mouse intestine coincided with those of NA and iron contents, which were the highest in the proximal jejunum. Orally administered NA-Fe (II) complex in mice was detected in the proximal jejunum by thin layer chromatography. In contrast, much less Fe (or NA) was detected in the duodenum, where the divalent metal transporter SLC11A2 (DMT1) absorbs free Fe (II). The collective results revealed the role of PAT1 in NA-Fe (II) absorption in the intestine and potential implication of NA in iron uptake in mammals."},"publication_date":"2021-01","publication_name":{"en":"The Journal of Biological Chemistry","ja":"The Journal of Biological Chemistry"},"volume":"Vol.296","starting_page":"100195","ending_page":"100195","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1074/jbc.RA120.015861"],"issn":["1083-351X"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:14, {"insert":{"user_id":"5000093573","type":"published_papers","id":"33397489"},"force":{"see_also":[{"@id":"https://repo.lib.tokushima-u.ac.jp/ja/116176","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=379996","label":"url"}],"paper_title":{"en":"Hydrotalcite-Supported Ag/Pd Bimetallic Nanoclusters Catalyzed Oxidation and One-Pot Aldol Reaction in Water","ja":"Hydrotalcite-Supported Ag/Pd Bimetallic Nanoclusters Catalyzed Oxidation and One-Pot Aldol Reaction in Water"},"authors":{"en":[{"name":"Karanjit Sangita"},{"name":"Tamura Ayumu"},{"name":"Kashihara Masaya"},{"name":"Ushiyama Kazuki"},{"name":"Shreshta K. L."},{"name":"Ariga Katsuhiko"},{"name":"Namba Kosuke"}],"ja":[{"name":"カランジット サンギータ"},{"name":"田村 歩"},{"name":"柏原 雅也"},{"name":"牛山 和輝"},{"name":"Shreshta K. L."},{"name":"Ariga Katsuhiko"},{"name":"難波 康祐"}]},"publication_date":"2020-09-29","publication_name":{"en":"Catalysts","ja":"Catalysts"},"volume":"Vol.10","number":"No.10","starting_page":"1120","ending_page":"1120","languages":["eng"],"referee":true,"identifiers":{"doi":["10.3390/catal10101120"],"issn":["2073-4344"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:15, {"insert":{"user_id":"5000093573","type":"published_papers","id":"33397490"},"force":{"see_also":[{"@id":"https://repo.lib.tokushima-u.ac.jp/ja/116180","label":"url"},{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/32969565","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=380069","label":"url"}],"paper_title":{"en":"Concise Total Synthesis of Tronocarpine","ja":"Concise Total Synthesis of Tronocarpine"},"authors":{"en":[{"name":"Nakayama Atsushi"},{"name":"Nakamura Tenta"},{"name":"Zaima Toshihiro"},{"name":"Fujimoto Saho"},{"name":"Karanjit Sangita"},{"name":"Namba Kosuke"}],"ja":[{"name":"中山 淳"},{"name":"中村 天太"},{"name":"財間 俊宏"},{"name":"藤本 沙帆"},{"name":"カランジット サンギータ"},{"name":"難波 康祐"}]},"description":{"en":"A concise total synthesis of tronocarpine, a chippiine-type indole alkaloid, was accomplished. The key feature of this total synthesis is a one-pot construction of the pentacyclic skeleton containing an azabicyclo[3.3.1]nonane core by tandem cyclization from an indole derivative with all carbon side chains and functional groups. This tandem cyclization consists of α,β-unsaturated aldehyde formation, intramolecular aldol reaction, six-membered lactamization, azide reduction, and seven-membered lactamization. The stereochemical outcome in this tandem cyclization is controlled by the stereocenter at the C14 position. This strategy can be utilized to synthesize other chippiine-type alkaloids with azabicyclo[3.3.1]nonane skeletons.","ja":"A concise total synthesis of tronocarpine, a chippiine-type indole alkaloid, was accomplished. The key feature of this total synthesis is a one-pot construction of the pentacyclic skeleton containing an azabicyclo[3.3.1]nonane core by tandem cyclization from an indole derivative with all carbon side chains and functional groups. This tandem cyclization consists of α,β-unsaturated aldehyde formation, intramolecular aldol reaction, six-membered lactamization, azide reduction, and seven-membered lactamization. The stereochemical outcome in this tandem cyclization is controlled by the stereocenter at the C14 position. This strategy can be utilized to synthesize other chippiine-type alkaloids with azabicyclo[3.3.1]nonane skeletons."},"publication_date":"2020-09-24","publication_name":{"en":"Angewandte Chemie International Edition","ja":"Angewandte Chemie International Edition"},"volume":"Vol.60","number":"No.2","starting_page":"635","ending_page":"639","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1002/anie.202009966"],"issn":["1521-3773"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:16, {"insert":{"user_id":"5000093573","type":"published_papers","id":"30458577"},"force":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=368062","label":"url"}],"paper_title":{"en":"Total Synthesis of Epilupinine: Synthetic Strategy of Fused Bicyclic Skeleton Containing Nitrogen","ja":"Total Synthesis of Epilupinine: Synthetic Strategy of Fused Bicyclic Skeleton Containing Nitrogen"},"authors":{"en":[{"name":"Tomohiro Tsutsumi"},{"name":"Namba Kosuke"}],"ja":[{"name":"堤 大洋"},{"name":"難波 康祐"}]},"publication_date":"2020-05-22","publication_name":{"en":"Chemistry Letters","ja":"Chemistry Letters"},"volume":"Vol.49","starting_page":"963","ending_page":"969","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1246/cl.200340"],"issn":["1348-0715"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:17, {"insert":{"user_id":"5000093573","type":"published_papers","id":"30458578"},"force":{"see_also":[{"@id":"https://repo.lib.tokushima-u.ac.jp/ja/115070","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=368053","label":"url"}],"paper_title":{"en":"Synthesis and evaluation of 1,1,7,7-tetramethyl-9-azajulolidine (TMAJ) as a highly active derivative of N,N-dimethylaminopyridine","ja":"Synthesis and evaluation of 1,1,7,7-tetramethyl-9-azajulolidine (TMAJ) as a highly active derivative of N,N-dimethylaminopyridine"},"authors":{"en":[{"name":"Tomohiro Tsutsumi"},{"name":"Arisa Saitoh"},{"name":"Tomoyo Kasai"},{"name":"MengYue Chu"},{"name":"Karanjit Sangita"},{"name":"Nakayama Atsushi"},{"name":"Namba Kosuke"}],"ja":[{"name":"堤 大洋"},{"name":"斎藤 亜梨紗"},{"name":"笠井 知世"},{"name":"初 もんゆえ"},{"name":"カランジット サンギータ"},{"name":"中山 淳"},{"name":"難波 康祐"}]},"publication_date":"2020-05-17","publication_name":{"en":"Tetrahedron Letters","ja":"Tetrahedron Letters"},"volume":"Vol.61","number":"No.26","starting_page":"152047","ending_page":"152047","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1016/j.tetlet.2020.152047"],"issn":["0040-4039"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:18, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://repo.lib.tokushima-u.ac.jp/ja/115071","label":"url"},{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-85077692885&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=362825","label":"url"}],"paper_title":{"en":"Development of a 1,3a,6a-triazapentalene derivatives as a compact and thiol-specific fluorescent labeling reagent","ja":"Development of a 1,3a,6a-triazapentalene derivatives as a compact and thiol-specific fluorescent labeling reagent"},"authors":{"en":[{"name":"Nakayama Atsushi"},{"name":"Ohtani Akira"},{"name":"Inokuma Tsubasa"},{"name":"Tsuji Daisuke"},{"name":"Mukaiyama Haruka"},{"name":"Akira Nakayama"},{"name":"Itou Kouji"},{"name":"Otaka Akira"},{"name":"Keiji Tanino"},{"name":"Namba Kosuke"}],"ja":[{"name":"中山 淳"},{"name":"大谷 彬"},{"name":"猪熊 翼"},{"name":"辻 大輔"},{"name":"向山 はるか"},{"name":"Akira Nakayama"},{"name":"伊藤 孝司"},{"name":"大髙 章"},{"name":"Keiji Tanino"},{"name":"難波 康祐"}]},"publication_date":"2020-01-09","publication_name":{"en":"Communications Chemistry","ja":"Communications Chemistry"},"volume":"Vol.3","starting_page":"6","ending_page":"6","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1038/s42004-019-0250-0"],"issn":["2399-3669"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:19, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://repo.lib.tokushima-u.ac.jp/ja/115585","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=362831","label":"url"}],"paper_title":{"en":"Synthesis and Antimicrobial Evaluation of Side-Chain Derivatives based on Eurotiumide A","ja":"Synthesis and Antimicrobial Evaluation of Side-Chain Derivatives based on Eurotiumide A"},"authors":{"en":[{"name":"Nakayama Atsushi"},{"name":"Satoh Hideo"},{"name":"Nakamura Tenta"},{"name":"Mai Hamada"},{"name":"Shuji Nagano"},{"name":"Kameyama Shuhei"},{"name":"Yui Furue"},{"name":"Naoki Hayashi"},{"name":"Go Kamoshida"},{"name":"Karanjit Sangita"},{"name":"Masataka Oda"},{"name":"Namba Kosuke"}],"ja":[{"name":"中山 淳"},{"name":"佐藤 次朗"},{"name":"中村 天太"},{"name":"濱田 麻衣"},{"name":"長野 秀嗣"},{"name":"亀山 周平"},{"name":"Yui Furue"},{"name":"Naoki Hayashi"},{"name":"Go Kamoshida"},{"name":"カランジット サンギータ"},{"name":"Masataka Oda"},{"name":"難波 康祐"}]},"publication_date":"2020-01","publication_name":{"en":"Marine Drugs","ja":"Marine Drugs"},"volume":"Vol.18","number":"No.2","starting_page":"92","ending_page":"92","languages":["eng"],"referee":true,"identifiers":{"doi":["10.3390/md18020092"],"issn":["1660-3397"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:20, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://repo.lib.tokushima-u.ac.jp/ja/113683","label":"url"},{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/31474735","label":"url"},{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-85071659929&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=353834","label":"url"}],"paper_title":{"en":"Asymmetric Total Syntheses and Structure Elucidations of (+)-Eurotiumide F and (+)-Eurotiumide G","ja":"Asymmetric Total Syntheses and Structure Elucidations of (+)-Eurotiumide F and (+)-Eurotiumide G"},"authors":{"en":[{"name":"Nakayama Atsushi"},{"name":"Satoh Hideo"},{"name":"Nagano Shuji"},{"name":"Karanjit Sangita"},{"name":"Imagawa Hiroshi"},{"name":"Namba Kosuke"}],"ja":[{"name":"中山 淳"},{"name":"佐藤 次朗"},{"name":"長野 秀嗣"},{"name":"カランジット サンギータ"},{"name":"今川 洋"},{"name":"難波 康祐"}]},"description":{"en":"Asymmetric total syntheses of dihydropyran containing natural products, (+)-eurotiumide F and (+)-eurotiumide G have been described. These total syntheses revealed the absolute configuration of eurotiumide F and G, and confirmed the reported structure of eurotiumide F and revised the reported structure of eurotiumide G. Highlight of these syntheses is thermal rearrangement with 4-methoxyisochroman-1-one derivative having propargyl ether on phenolic ether under thermal condition to construct dihydropyran ring. X-Ray crystallographic analysis of (+)-eurotiumide G clarified the stereochemistry at the C1-position.","ja":"Asymmetric total syntheses of dihydropyran containing natural products, (+)-eurotiumide F and (+)-eurotiumide G have been described. These total syntheses revealed the absolute configuration of eurotiumide F and G, and confirmed the reported structure of eurotiumide F and revised the reported structure of eurotiumide G. Highlight of these syntheses is thermal rearrangement with 4-methoxyisochroman-1-one derivative having propargyl ether on phenolic ether under thermal condition to construct dihydropyran ring. X-Ray crystallographic analysis of (+)-eurotiumide G clarified the stereochemistry at the C1-position."},"publication_date":"2019-07-16","publication_name":{"en":"Chemical & Pharmaceutical Bulletin","ja":"Chemical & Pharmaceutical Bulletin"},"volume":"Vol.67","number":"No.9","starting_page":"953","ending_page":"958","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1248/cpb.c18-00948"],"issn":["1347-5223"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:21, {"insert":{"user_id":"5000093573","type":"published_papers","id":"30458579"},"force":{"see_also":[{"@id":"https://repo.lib.tokushima-u.ac.jp/ja/113631","label":"url"},{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/30963767","label":"url"},{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-85064687055&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=353833","label":"url"}],"paper_title":{"en":"A Concise Asymmetric Total Synthesis of (+)-Epilupinine","ja":"A Concise Asymmetric Total Synthesis of (+)-Epilupinine"},"authors":{"en":[{"name":"Tsutsumi Tomohiro"},{"name":"Karanjit Sangita"},{"name":"Nakayama Atsushi"},{"name":"Namba Kosuke"}],"ja":[{"name":"堤 大洋"},{"name":"カランジット サンギータ"},{"name":"中山 淳"},{"name":"難波 康祐"}]},"description":{"en":"Asymmetric total synthesis of (+)-epilupinine was achieved in just three steps using only commercially available common reagents. The total synthesis involved alkylations of N-nosylamide, ozone oxidation, and sequential reactions of the removal of the nosyl group, intramolecular dehydrative condensation, intramolecular Mannich reaction catalyzed by l-proline, and a reduction.","ja":"Asymmetric total synthesis of (+)-epilupinine was achieved in just three steps using only commercially available common reagents. The total synthesis involved alkylations of N-nosylamide, ozone oxidation, and sequential reactions of the removal of the nosyl group, intramolecular dehydrative condensation, intramolecular Mannich reaction catalyzed by l-proline, and a reduction."},"publication_date":"2019-04-09","publication_name":{"en":"Organic Letters","ja":"Organic Letters"},"volume":"Vol.21","number":"No.8","starting_page":"2620","ending_page":"2624","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1021/acs.orglett.9b00607"],"issn":["1523-7052"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:22, {"insert":{"user_id":"5000093573","type":"published_papers","id":"30458580"},"force":{"see_also":[{"@id":"https://repo.lib.tokushima-u.ac.jp/ja/113632","label":"url"},{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-85066142615&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=351723","label":"url"}],"paper_title":{"en":"Microwave-assisted Tertiary Carbon Radical Reaction for Construction of Quaternary Carbon Center","ja":"Microwave-assisted Tertiary Carbon Radical Reaction for Construction of Quaternary Carbon Center"},"authors":{"en":[{"name":"Sato Ryota"},{"name":"Okamoto Ryuji"},{"name":"Ishizuka Takumi"},{"name":"Nakayama Atsushi"},{"name":"Karanjit Sangita"},{"name":"Namba Kosuke"}],"ja":[{"name":"佐藤 亮太"},{"name":"岡本 龍治"},{"name":"石塚 匠"},{"name":"中山 淳"},{"name":"カランジット サンギータ"},{"name":"難波 康祐"}]},"publication_date":"2019-02","publication_name":{"en":"Chemistry Letters","ja":"Chemistry Letters"},"volume":"Vol.48","number":"No.5","starting_page":"414","ending_page":"417","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1246/cl.190040"],"issn":["1348-0715"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:23, {"insert":{"user_id":"5000093573","type":"published_papers","id":"30458581"},"force":{"see_also":[{"@id":"https://repo.lib.tokushima-u.ac.jp/ja/113635","label":"url"},{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/30270318","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=356296","label":"url"}],"paper_title":{"en":"Organic Chemistry Research on the Mechanistic Elucidation of Iron Acquisition in Barley","ja":"Organic Chemistry Research on the Mechanistic Elucidation of Iron Acquisition in Barley"},"authors":{"en":[{"name":"Namba Kosuke"},{"name":"Yoshiko Murata"}],"ja":[{"name":"難波 康祐"},{"name":"村田 佳子"}]},"description":{"en":"An organic chemistry approach to the mechanistic elucidation of iron acquisition in graminaceous plants is introduced here. To elucidate this detailed mechanism using phytosiderophores, the efficient synthesis of 2'-deoxymugineic acid (DMA), a phytosiderophore of rice, was established. The synthetic DMA was confirmed to have similar iron transport activity to that of natural mugineic acid (MA). It was also revealed that the addition of synthetic DMA, along with iron, to a rice hydroponic solution enabled the rice to grow well even under an alkaline condition, and DMA clearly showed its high potential as a fertilizer to improve food production. On the other hand, the 2'-hydroxy group of MA was confirmed to serve as a point of introduction for labeling, allowing the synthesis of various mugineic acid derivatives as molecular probes. The incorporation of fluorescent mugineic acid into cells allowed them to be clearly observed by fluorescence confocal analysis, and this provided the first direct experimental evidence of transporter-mediated internalization of mugineic acid into cells.","ja":"An organic chemistry approach to the mechanistic elucidation of iron acquisition in graminaceous plants is introduced here. To elucidate this detailed mechanism using phytosiderophores, the efficient synthesis of 2'-deoxymugineic acid (DMA), a phytosiderophore of rice, was established. The synthetic DMA was confirmed to have similar iron transport activity to that of natural mugineic acid (MA). It was also revealed that the addition of synthetic DMA, along with iron, to a rice hydroponic solution enabled the rice to grow well even under an alkaline condition, and DMA clearly showed its high potential as a fertilizer to improve food production. On the other hand, the 2'-hydroxy group of MA was confirmed to serve as a point of introduction for labeling, allowing the synthesis of various mugineic acid derivatives as molecular probes. The incorporation of fluorescent mugineic acid into cells allowed them to be clearly observed by fluorescence confocal analysis, and this provided the first direct experimental evidence of transporter-mediated internalization of mugineic acid into cells."},"publication_date":"2018-10-01","publication_name":{"en":"Biological & Pharmaceutical Bulletin","ja":"Biological & Pharmaceutical Bulletin"},"volume":"Vol.41","number":"No.10","starting_page":"1502","ending_page":"1507","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1248/bpb.b18-00070"],"issn":["1347-5215"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
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line:25, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=342435","label":"url"}],"paper_title":{"en":"Quantitation of sevourane in whole blood and aqueous solutions byvolatile organic compound sensing","ja":"Quantitation of sevourane in whole blood and aqueous solutions byvolatile organic compound sensing"},"authors":{"en":[{"name":"Yuri Hase"},{"name":"Kuniaki Suzuki"},{"name":"Nobuhito Kamekura"},{"name":"Yu Takahashi"},{"name":"Namba Kosuke"},{"name":"Toshiaki Fujiwara"}],"ja":[{"name":"Yuri Hase"},{"name":"Kuniaki Suzuki"},{"name":"Nobuhito Kamekura"},{"name":"Yu Takahashi"},{"name":"難波 康祐"},{"name":"Toshiaki Fujiwara"}]},"publication_date":"2018-06-01","publication_name":{"en":"Journal of Pharmacological and Toxicological Methods","ja":"Journal of Pharmacological and Toxicological Methods"},"volume":"Vol.94","starting_page":"71","ending_page":"76","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1016/j.vascn.2018.05.005"],"issn":["1056-8719"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:26, {"insert":{"user_id":"5000093573","type":"published_papers","id":"30458582"},"force":{"see_also":[{"@id":"https://repo.lib.tokushima-u.ac.jp/ja/113634","label":"url"},{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/29701268","label":"url"},{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-85049583439&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=342430","label":"url"}],"paper_title":{"en":"Direct Synthesis of Polycyclic Tropinones by a Condensation-[4+3]-Cycloaddition Cascade Reaction.","ja":"Direct Synthesis of Polycyclic Tropinones by a Condensation-[4+3]-Cycloaddition Cascade Reaction."},"authors":{"en":[{"name":"Okamoto Tsubasa"},{"name":"Shibata Miki"},{"name":"Karanjit Sangita"},{"name":"Nakayama Atsushi"},{"name":"Yoshida Masahiro"},{"name":"Namba Kosuke"}],"ja":[{"name":"岡本 翼"},{"name":"柴田 弥希"},{"name":"カランジット サンギータ"},{"name":"中山 淳"},{"name":"吉田 昌裕"},{"name":"難波 康祐"}]},"description":{"en":"A concise method of constructing polycyclic tropinone frameworks was developed. The single-step synthesis of polycyclic tropinone consists of an intramolecular [4+3] cycloaddition reaction of N-nosyl-pyrrole with oxyallyl cation that was generated in situ by an intermolecular condensation reaction of the nucleophilic functional groups on a tethered pyrrole with the aldehyde of 2-(silyloxy)-acrolein. This cascade reaction afforded various polycyclic tropinones including tri-, tetra-, and pentacyclic systems in high yields as single diastereomers.","ja":"A concise method of constructing polycyclic tropinone frameworks was developed. The single-step synthesis of polycyclic tropinone consists of an intramolecular [4+3] cycloaddition reaction of N-nosyl-pyrrole with oxyallyl cation that was generated in situ by an intermolecular condensation reaction of the nucleophilic functional groups on a tethered pyrrole with the aldehyde of 2-(silyloxy)-acrolein. This cascade reaction afforded various polycyclic tropinones including tri-, tetra-, and pentacyclic systems in high yields as single diastereomers."},"publication_date":"2018-04-27","publication_name":{"en":"Chemistry - A European Journal","ja":"Chemistry - A European Journal"},"volume":"Vol.24","number":"No.38","starting_page":"9508","ending_page":"9513","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1002/chem.201802011"],"issn":["1521-3765"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
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line:33, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://repo.lib.tokushima-u.ac.jp/ja/114563","label":"url"},{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/27861811","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=329625","label":"url"}],"paper_title":{"en":"The helical propensity of the extracellular loop is responsible for the substrate specificity of Fe(III)-phytosiderophore transporters.","ja":"The helical propensity of the extracellular loop is responsible for the substrate specificity of Fe(III)-phytosiderophore transporters."},"authors":{"en":[{"name":"Harada Erisa"},{"name":"Sugase Kenji"},{"name":"Namba Kosuke"},{"name":"Murata Yoshiko"}],"ja":[{"name":"Harada Erisa"},{"name":"Sugase Kenji"},{"name":"難波 康祐"},{"name":"Murata Yoshiko"}]},"description":{"en":"Hordeum vulgare L. yellow stripe 1 (HvYS1) is a selective transporter of Fe(III)-phytosiderophores in barley that is responsible for iron acquisition from the soil. In contrast, maize Zea mays, yellow stripe 1 (ZmYS1) possesses broad substrate specificity. In this study, a quantitative evaluation of the transport activities of HvYS1 and ZmYS1 chimera proteins revealed that the seventh extracellular membrane loop is essential for substrate specificity. The loop peptides of both transporters were prepared and analysed by circular dichroism and NMR. The spectra revealed a higher propensity for α-helical conformation of the HvYS1 loop peptide and a largely disordered structure for that of ZmYS1. These structural differences are potentially responsible for the substrate specificities of the transporters.","ja":"Hordeum vulgare L. yellow stripe 1 (HvYS1) is a selective transporter of Fe(III)-phytosiderophores in barley that is responsible for iron acquisition from the soil. In contrast, maize Zea mays, yellow stripe 1 (ZmYS1) possesses broad substrate specificity. In this study, a quantitative evaluation of the transport activities of HvYS1 and ZmYS1 chimera proteins revealed that the seventh extracellular membrane loop is essential for substrate specificity. The loop peptides of both transporters were prepared and analysed by circular dichroism and NMR. The spectra revealed a higher propensity for α-helical conformation of the HvYS1 loop peptide and a largely disordered structure for that of ZmYS1. These structural differences are potentially responsible for the substrate specificities of the transporters."},"publication_date":"2016-11-23","publication_name":{"en":"FEBS Letters","ja":"FEBS Letters"},"volume":"Vol.590","number":"No.24","starting_page":"4617","ending_page":"4627","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1002/1873-3468.12482"],"issn":["1873-3468"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:34, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://repo.lib.tokushima-u.ac.jp/ja/111875","label":"url"},{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/27793568","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=329632","label":"url"}],"paper_title":{"en":"Functional 1,3a,6a-triazapentalene scaffold: Design of fluorescent probes for kinesin spindle protein (KSP)","ja":"Functional 1,3a,6a-triazapentalene scaffold: Design of fluorescent probes for kinesin spindle protein (KSP)"},"authors":{"en":[{"name":"Sawada Jun-ichi"},{"name":"Osawa Ayumi"},{"name":"Takeuchi Tomoki"},{"name":"Kaneda Masato"},{"name":"Oishi Shinya"},{"name":"Fujii Nobutaka"},{"name":"Asai Akira"},{"name":"Tanino keiji"},{"name":"Namba Kosuke"}],"ja":[{"name":"Sawada Jun-ichi"},{"name":"Osawa Ayumi"},{"name":"Takeuchi Tomoki"},{"name":"Kaneda Masato"},{"name":"Oishi Shinya"},{"name":"Fujii Nobutaka"},{"name":"Asai Akira"},{"name":"Tanino keiji"},{"name":"難波 康祐"}]},"description":{"en":"1,3a,6a-Triazapentalene is a compact fluorescent chromophore. In this study, triazapentalene was used to modify a series of biphenyl-type inhibitors of kinesin spindle protein (KSP) to develop fluorescent probes for the intracellular visualization of this protein. Microscopic studies demonstrated that these novel triazapentalene-labeled compounds exhibited inhibitory activity towards KSP in cultured cells and provided important information concerning the intracellular distribution.","ja":"1,3a,6a-Triazapentalene is a compact fluorescent chromophore. In this study, triazapentalene was used to modify a series of biphenyl-type inhibitors of kinesin spindle protein (KSP) to develop fluorescent probes for the intracellular visualization of this protein. Microscopic studies demonstrated that these novel triazapentalene-labeled compounds exhibited inhibitory activity towards KSP in cultured cells and provided important information concerning the intracellular distribution."},"publication_date":"2016-10-15","publication_name":{"en":"Bioorganic & Medicinal Chemistry Letters","ja":"Bioorganic & Medicinal Chemistry Letters"},"volume":"Vol.26","number":"No.23","starting_page":"5765","ending_page":"5769","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1016/j.bmcl.2016.10.047"],"issn":["1464-3405"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:35, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://repo.lib.tokushima-u.ac.jp/ja/112331","label":"url"},{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/27490470","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=329637","label":"url"}],"paper_title":{"en":"Effective Cellular Morphology Analysis for Differentiation Processes by a Fluorescent 1,3a,6a-Triazapentalene Derivative Probe in Live Cells","ja":"Effective Cellular Morphology Analysis for Differentiation Processes by a Fluorescent 1,3a,6a-Triazapentalene Derivative Probe in Live Cells"},"authors":{"en":[{"name":"Kamada Rui"},{"name":"Tano Fumi"},{"name":"Kudoh Fuki"},{"name":"Kimura Nozomi"},{"name":"Chuman Yoshiro"},{"name":"Osawa Ayumi"},{"name":"Namba Kosuke"},{"name":"Tanino Keiji"},{"name":"Sakaguchi Kazuyasu"}],"ja":[{"name":"Kamada Rui"},{"name":"Tano Fumi"},{"name":"Kudoh Fuki"},{"name":"Kimura Nozomi"},{"name":"Chuman Yoshiro"},{"name":"Osawa Ayumi"},{"name":"難波 康祐"},{"name":"Tanino Keiji"},{"name":"Sakaguchi Kazuyasu"}]},"description":{"en":"Nuclear and cytoplasmic morphological changes provide important information about cell differentiation processes, cell functions, and signal responses. There is a strong desire to develop a rapid and simple method for visualizing cytoplasmic and nuclear morphology. Here, we developed a novel and rapid method for probing cellular morphological changes of live cell differentiation process by a fluorescent probe, TAP-4PH, a 1,3a,6a-triazapentalene derivative. TAP-4PH showed high fluorescence in cytoplasmic area, and visualized cytoplasmic and nuclear morphological changes of live cells during differentiation. We demonstrated that TAP-4PH visualized dendritic axon and spine formation in neuronal differentiation, and nuclear structural changes during neutrophilic differentiation. We also showed that the utility of TAP-4PH for visualization of cytoplasmic and nuclear morphologies of various type of live cells. Our visualizing method has no toxicity and no influence on the cellular differentiation and function. The cell morphology can be rapidly observed after addition of TAP-4PH and can continue to be observed in the presence of TAP-4PH in cell culture medium. Moreover, TAP-4PH can be easily removed after observation by washing for subsequent biological assay. Taken together, these results demonstrate that our visualization method is a powerful tool to probe differentiation processes before subsequent biological assay in live cells.","ja":"Nuclear and cytoplasmic morphological changes provide important information about cell differentiation processes, cell functions, and signal responses. There is a strong desire to develop a rapid and simple method for visualizing cytoplasmic and nuclear morphology. Here, we developed a novel and rapid method for probing cellular morphological changes of live cell differentiation process by a fluorescent probe, TAP-4PH, a 1,3a,6a-triazapentalene derivative. TAP-4PH showed high fluorescence in cytoplasmic area, and visualized cytoplasmic and nuclear morphological changes of live cells during differentiation. We demonstrated that TAP-4PH visualized dendritic axon and spine formation in neuronal differentiation, and nuclear structural changes during neutrophilic differentiation. We also showed that the utility of TAP-4PH for visualization of cytoplasmic and nuclear morphologies of various type of live cells. Our visualizing method has no toxicity and no influence on the cellular differentiation and function. The cell morphology can be rapidly observed after addition of TAP-4PH and can continue to be observed in the presence of TAP-4PH in cell culture medium. Moreover, TAP-4PH can be easily removed after observation by washing for subsequent biological assay. Taken together, these results demonstrate that our visualization method is a powerful tool to probe differentiation processes before subsequent biological assay in live cells."},"publication_date":"2016-08-04","publication_name":{"en":"PLoS ONE","ja":"PLoS ONE"},"volume":"Vol.11","number":"No.8","starting_page":"e0160625","ending_page":"e0160625","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1371/journal.pone.0160625"],"issn":["1932-6203"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:36, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=329641","label":"url"}],"paper_title":{"en":"Direct cyclization of 1,3-diaryl propargylic alcohols with dicarbonyl compounds by palladium-boric acid dual-catalyst system","ja":"Direct cyclization of 1,3-diaryl propargylic alcohols with dicarbonyl compounds by palladium-boric acid dual-catalyst system"},"authors":{"en":[{"name":"Yoshida Masahiro"},{"name":"Ohno Shoko"},{"name":"Eguchi Sayaka"},{"name":"Mizuguchi Tomotaka"},{"name":"Namba Kosuke"}],"ja":[{"name":"吉田 昌裕"},{"name":"Ohno Shoko"},{"name":"Eguchi Sayaka"},{"name":"Mizuguchi Tomotaka"},{"name":"難波 康祐"}]},"publication_date":"2016-07-26","publication_name":{"en":"Tetrahedron","ja":"Tetrahedron"},"volume":"Vol.72","number":"No.36","starting_page":"5633","ending_page":"5639","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1016/j.tet.2016.07.055"],"issn":["0040-4020"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:37, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://repo.lib.tokushima-u.ac.jp/ja/111876","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=329992","label":"url"}],"paper_title":{"en":"Facile Guanidine Formation under Mild Acidic Conditions","ja":"Facile Guanidine Formation under Mild Acidic Conditions"},"authors":{"en":[{"name":"Kohei Takeuchi"},{"name":"Nakayama Atsushi"},{"name":"Keiji Tanino"},{"name":"Namba Kosuke"}],"ja":[{"name":"竹内 公平"},{"name":"中山 淳"},{"name":"Keiji Tanino"},{"name":"難波 康祐"}]},"publication_date":"2016-06-23","publication_name":{"en":"Synlett","ja":"Synlett"},"volume":"Vol.27","number":"No.18","starting_page":"2591","ending_page":"2596","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1055/s-0035-1562478"],"issn":["0936-5214"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:38, {"insert":{"user_id":"5000093573","type":"published_papers","id":"33590265"},"force":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/27373639","label":"url"},{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-84977588368&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=316489","label":"url"}],"paper_title":{"en":"Substituent Effect at C4-Position of 1,3a,6a-Triazapentalene","ja":"Substituent Effect at C4-Position of 1,3a,6a-Triazapentalene"},"authors":{"en":[{"name":"Nakayama Atsushi"},{"name":"Satoshi Nishio"},{"name":"Akira Otani"},{"name":"Akane Mera"},{"name":"Ayumi Osawa"},{"name":"keiji Tanino"},{"name":"Namba Kosuke"}],"ja":[{"name":"中山 淳"},{"name":"西尾 賢"},{"name":"大谷 彬"},{"name":"米良 茜"},{"name":"大澤 歩"},{"name":"谷野 圭持"},{"name":"難波 康祐"}]},"description":{"en":"Various 2,4-disubstituted-1,3a,6a-triazapentalenes possessing methyl and phenyl groups at the C4-position were synthesized. Fluorescence observation of the synthetic 4-methyl- and 4-phenyl-1,3a,6a-triazapentalenes revealed that the introduction of a substituent at the C4-position allowed a long-wavelength shift of the fluorescence maximum. Furthermore, the phenyl group at the C4-position was found to induce a substantial increase in the extinction coefficient value.","ja":"Various 2,4-disubstituted-1,3a,6a-triazapentalenes possessing methyl and phenyl groups at the C4-position were synthesized. Fluorescence observation of the synthetic 4-methyl- and 4-phenyl-1,3a,6a-triazapentalenes revealed that the introduction of a substituent at the C4-position allowed a long-wavelength shift of the fluorescence maximum. Furthermore, the phenyl group at the C4-position was found to induce a substantial increase in the extinction coefficient value."},"publication_date":"2016-04-12","publication_name":{"en":"Chemical & Pharmaceutical Bulletin","ja":"Chemical & Pharmaceutical Bulletin"},"volume":"Vol.64","number":"No.7","starting_page":"830","ending_page":"837","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1248/cpb.c16-00196"],"issn":["1347-5223"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:39, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-84963522445&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=310598","label":"url"}],"paper_title":{"en":"Synthesis of functionalized 2,3-dihydropyrroles by oxidative radical cyclization of N-Sulfonyl β-enamino esters with alkenes","ja":"Synthesis of functionalized 2,3-dihydropyrroles by oxidative radical cyclization of N-Sulfonyl β-enamino esters with alkenes"},"authors":{"en":[{"name":"Yoshida Masahiro"},{"name":"Kobayashi Asuka"},{"name":"Nakayama Atsushi"},{"name":"Namba Kosuke"}],"ja":[{"name":"吉田 昌裕"},{"name":"小林 明日香"},{"name":"中山 淳"},{"name":"難波 康祐"}]},"publication_date":"2016-03-16","publication_name":{"en":"Tetrahedron","ja":"Tetrahedron"},"volume":"Vol.72","number":"No.20","starting_page":"2544","ending_page":"2551","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1016/j.tet.2016.03.055"],"issn":["0040-4020"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:40, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://repo.lib.tokushima-u.ac.jp/ja/115641","label":"url"},{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/26530707","label":"url"},{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-84946600416&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=305950","label":"url"}],"paper_title":{"en":"Total synthesis of palau'amine","ja":"Total synthesis of palau'amine"},"authors":{"en":[{"name":"Namba Kosuke"},{"name":"Takeuchi Kohei"},{"name":"Kaihara Yukari"},{"name":"Oda Masataka"},{"name":"Nakayama Akira"},{"name":"Nakayama Atsushi"},{"name":"Yoshida Masahiro"},{"name":"Tanino Keiji"}],"ja":[{"name":"難波 康祐"},{"name":"竹内 公平"},{"name":"Kaihara Yukari"},{"name":"Oda Masataka"},{"name":"Nakayama Akira"},{"name":"中山 淳"},{"name":"吉田 昌裕"},{"name":"Tanino Keiji"}]},"description":{"en":"Palau'amine has received a great deal of attention in the past two decades as an attractive synthetic target by virtue of its intriguing molecular architecture and significant immunosuppressive activity. Here we report the total synthesis of palau'amine characterized by the construction of an ABDE tetracyclic ring core including a trans-bicylo[3.3.0]octane skeleton at a middle stage of total synthesis. The ABDE tetracyclic ring core is constructed by a cascade reaction of a cleavage of the N-N bond, including simultaneous formation of imine, the addition of amide anion to the resulting imine (D-ring formation) and the condensation of pyrrole with methyl ester (B-ring formation) in a single step. The synthetic palau'amine is confirmed to exhibit excellent immunosuppressive activity. The present synthetic route has the potential to help elucidate a pharmacophore as well as the mechanistic details of immunosuppressive activity.","ja":"Palau'amine has received a great deal of attention in the past two decades as an attractive synthetic target by virtue of its intriguing molecular architecture and significant immunosuppressive activity. Here we report the total synthesis of palau'amine characterized by the construction of an ABDE tetracyclic ring core including a trans-bicylo[3.3.0]octane skeleton at a middle stage of total synthesis. The ABDE tetracyclic ring core is constructed by a cascade reaction of a cleavage of the N-N bond, including simultaneous formation of imine, the addition of amide anion to the resulting imine (D-ring formation) and the condensation of pyrrole with methyl ester (B-ring formation) in a single step. The synthetic palau'amine is confirmed to exhibit excellent immunosuppressive activity. The present synthetic route has the potential to help elucidate a pharmacophore as well as the mechanistic details of immunosuppressive activity."},"publication_date":"2015-11-04","publication_name":{"en":"Nature Communications","ja":"Nature Communications"},"volume":"Vol.6","starting_page":"8731","ending_page":"8731","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1038/ncomms9731"],"issn":["2041-1723"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:41, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-84930088524&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=299049","label":"url"}],"paper_title":{"en":"Acid-catalyzed [4+3] cycloaddition reaction of N-nosyl pyrroles","ja":"Acid-catalyzed [4+3] cycloaddition reaction of N-nosyl pyrroles"},"authors":{"en":[{"name":"Shibata Miki"},{"name":"Fuchigami Ryuichi"},{"name":"Kotaka Ryota"},{"name":"Tanino Keiji"},{"name":"Namba Kosuke"}],"ja":[{"name":"柴田 弥希"},{"name":"淵上 龍一"},{"name":"古高 涼太"},{"name":"谷野 圭持"},{"name":"難波 康祐"}]},"publication_date":"2015-07-01","publication_name":{"en":"Tetrahedron","ja":"Tetrahedron"},"volume":"Vol.71","number":"No.26-27","starting_page":"4495","ending_page":"4499","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1016/j.tet.2015.02.071"],"issn":["0040-4020"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:42, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://repo.lib.tokushima-u.ac.jp/ja/114927","label":"url"},{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/25781941","label":"url"},{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-84925003396&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=316551","label":"url"}],"paper_title":{"en":"Transgenic Petunia with the Iron(III)-Phytosiderophore Transporter Gene Acquires Tolerance to Iron Deficiency in Alkaline Environments","ja":"Transgenic Petunia with the Iron(III)-Phytosiderophore Transporter Gene Acquires Tolerance to Iron Deficiency in Alkaline Environments"},"authors":{"en":[{"name":"Murata Yoshiko"},{"name":"Ito Yoshiyuki"},{"name":"Iwashita Takashi"},{"name":"Namba Kosuke"}],"ja":[{"name":"Murata Yoshiko"},{"name":"Ito Yoshiyuki"},{"name":"Iwashita Takashi"},{"name":"難波 康祐"}]},"description":{"en":"Iron is an essential nutrient for all plants. However, terrestrial plants often suffer from iron deficiency in alkaline soil due to its extremely low solubility. Alkaline soil accounts for about 30% of all cultivated ground in the world. Plants have evolved two distinct strategies, I and II, for iron uptake from the soil. Dicots and non-graminaceous monocots use Strategy I, which is primarily based on the reduction of iron(III) to iron(II) and the uptake of iron(II) by the iron-regulated transporter, IRT1. In contrast, graminaceous plants use Strategy II to efficiently acquire insoluble iron(III). Strategy II comprises the synthesis and secretion of iron-chelating phytosiderophores, such as mugineic acids and the Yellow Stripe 1 transporter proteins of the iron(III)-phytosiderophore complex. Barley, which exhibits the highest tolerance to iron deficiency in alkaline soil among graminaceous plants, utilizes mugineic acids and the specific iron(III)-mugineic acids transporter, HvYS1. In this study, we established the transgenic plant Petunia hybrida, which originally had only Strategy I, by introducing the HvYS1 transporter gene derived from barley. When the transgenic plants were grown hydroponically in media containing the iron(III)-2'-deoxymugineic acid complex, free 2'-deoxymugineic acid and its iron(III) complex were detected in the root extract of the transgenic plant by electrospray ionization-Fourier transform-ion cyclotron resonance mass spectrometry. The growth of the transgenic petunia was significantly better than that of the control host in alkaline conditions. Consequently, the transgenic plant acquired a significantly enhanced tolerance to alkaline hydroponic media in the presence of the iron(III)-2'-deoxymugineic acid complex. Furthermore, the flower color of the transgenic plant deepened. The results showed that iron-phytosiderophore complexes and their transporters can potentially be utilized to overcome the worldwide iron uptake problems to diverse plant species that are found in areas with alkaline conditions.","ja":"Iron is an essential nutrient for all plants. However, terrestrial plants often suffer from iron deficiency in alkaline soil due to its extremely low solubility. Alkaline soil accounts for about 30% of all cultivated ground in the world. Plants have evolved two distinct strategies, I and II, for iron uptake from the soil. Dicots and non-graminaceous monocots use Strategy I, which is primarily based on the reduction of iron(III) to iron(II) and the uptake of iron(II) by the iron-regulated transporter, IRT1. In contrast, graminaceous plants use Strategy II to efficiently acquire insoluble iron(III). Strategy II comprises the synthesis and secretion of iron-chelating phytosiderophores, such as mugineic acids and the Yellow Stripe 1 transporter proteins of the iron(III)-phytosiderophore complex. Barley, which exhibits the highest tolerance to iron deficiency in alkaline soil among graminaceous plants, utilizes mugineic acids and the specific iron(III)-mugineic acids transporter, HvYS1. In this study, we established the transgenic plant Petunia hybrida, which originally had only Strategy I, by introducing the HvYS1 transporter gene derived from barley. When the transgenic plants were grown hydroponically in media containing the iron(III)-2'-deoxymugineic acid complex, free 2'-deoxymugineic acid and its iron(III) complex were detected in the root extract of the transgenic plant by electrospray ionization-Fourier transform-ion cyclotron resonance mass spectrometry. The growth of the transgenic petunia was significantly better than that of the control host in alkaline conditions. Consequently, the transgenic plant acquired a significantly enhanced tolerance to alkaline hydroponic media in the presence of the iron(III)-2'-deoxymugineic acid complex. Furthermore, the flower color of the transgenic plant deepened. The results showed that iron-phytosiderophore complexes and their transporters can potentially be utilized to overcome the worldwide iron uptake problems to diverse plant species that are found in areas with alkaline conditions."},"publication_date":"2015-03-17","publication_name":{"en":"PLoS ONE","ja":"PLoS ONE"},"volume":"Vol.10","number":"No.3","starting_page":"e0120227","ending_page":"e0120227","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1371/journal.pone.0120227"],"issn":["1932-6203"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:43, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://repo.lib.tokushima-u.ac.jp/ja/115060","label":"url"},{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-84922311525&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=289916","label":"url"}],"paper_title":{"en":"Synthesis of Yellow and Red Fluorescent 1,3a,6a-Triazapentalenes and the Theoretical Investigation of Their Optical Properties.","ja":"Synthesis of Yellow and Red Fluorescent 1,3a,6a-Triazapentalenes and the Theoretical Investigation of Their Optical Properties."},"authors":{"en":[{"name":"Namba Kosuke"},{"name":"Osawa Ayumi"},{"name":"Nakayama Akira"},{"name":"Mera Akane"},{"name":"Tano Fumi"},{"name":"Chuman Yoshiro"},{"name":"Sakuda Eri"},{"name":"Taketsugu Tetsuya"},{"name":"Sakaguchi Kazuyasu"},{"name":"Kitamura Noboru"},{"name":"Tanino Keiji"}],"ja":[{"name":"難波 康祐"},{"name":"Osawa Ayumi"},{"name":"Nakayama Akira"},{"name":"Mera Akane"},{"name":"Tano Fumi"},{"name":"Chuman Yoshiro"},{"name":"Sakuda Eri"},{"name":"Taketsugu Tetsuya"},{"name":"Sakaguchi Kazuyasu"},{"name":"Kitamura Noboru"},{"name":"Tanino Keiji"}]},"publication_date":"2015-01-23","publication_name":{"en":"Chemical Science","ja":"Chemical Science"},"volume":"Vol.6","number":"No.2","starting_page":"1083","ending_page":"1093","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1039/C4SC02780A"],"issn":["2041-6539"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:44, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/25393516","label":"url"},{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-84920744808&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=289917","label":"url"}],"paper_title":{"en":"2'-Deoxymugineic acid promotes growth of rice (Oryza sativa L.) by orchestrating iron and nitrate uptake processes under high pH conditions","ja":"2'-Deoxymugineic acid promotes growth of rice (Oryza sativa L.) by orchestrating iron and nitrate uptake processes under high pH conditions"},"authors":{"en":[{"name":"Araki Ryoichi"},{"name":"Kousaka Kayoko"},{"name":"Namba Kosuke"},{"name":"Murata Yoshiko"},{"name":"Murata Jun"}],"ja":[{"name":"Araki Ryoichi"},{"name":"Kousaka Kayoko"},{"name":"難波 康祐"},{"name":"Murata Yoshiko"},{"name":"Murata Jun"}]},"description":{"en":"Poaceae plants release 2'-deoxymugineic acid (DMA) and related phytosiderophores to chelate iron (Fe), which often exists as insoluble Fe(III) in the rhizosphere, especially under high pH conditions. Although the molecular mechanisms behind the biosynthesis and secretion of DMA have been studied extensively, little information is known about whether DMA has biological roles other than chelating Fe in vivo. Here, we demonstrate that hydroponic cultures of rice (Oryza sativa) seedlings show almost complete restoration in shoot height and soil-plant analysis development (SPAD) values after treatment with 3-30 μm DMA at high pH (pH 8.0), compared with untreated control seedlings at normal pH (pH 5.8). These changes were accompanied by selective accumulation of Fe over other metals. While this enhanced growth was evident under high pH conditions, DMA application also enhanced seedling growth under normal pH conditions in which Fe was fairly accessible. Microarray and qRT-PCR analyses revealed that exogenous DMA application attenuated the increased expression levels of various genes related to Fe transport and accumulation. Surprisingly, despite the preferential utilization of ammonium over nitrate as a nitrogen source by rice, DMA application also increased nitrate reductase activity and the expression of genes encoding high-affinity nitrate transporters and nitrate reductases, all of which were otherwise considerably lower under high pH conditions. These data suggest that exogenous DMA not only plays an important role in facilitating the uptake of environmental Fe, but also orchestrates Fe and nitrate assimilation for optimal growth under high pH conditions.","ja":"Poaceae plants release 2'-deoxymugineic acid (DMA) and related phytosiderophores to chelate iron (Fe), which often exists as insoluble Fe(III) in the rhizosphere, especially under high pH conditions. Although the molecular mechanisms behind the biosynthesis and secretion of DMA have been studied extensively, little information is known about whether DMA has biological roles other than chelating Fe in vivo. Here, we demonstrate that hydroponic cultures of rice (Oryza sativa) seedlings show almost complete restoration in shoot height and soil-plant analysis development (SPAD) values after treatment with 3-30 μm DMA at high pH (pH 8.0), compared with untreated control seedlings at normal pH (pH 5.8). These changes were accompanied by selective accumulation of Fe over other metals. While this enhanced growth was evident under high pH conditions, DMA application also enhanced seedling growth under normal pH conditions in which Fe was fairly accessible. Microarray and qRT-PCR analyses revealed that exogenous DMA application attenuated the increased expression levels of various genes related to Fe transport and accumulation. Surprisingly, despite the preferential utilization of ammonium over nitrate as a nitrogen source by rice, DMA application also increased nitrate reductase activity and the expression of genes encoding high-affinity nitrate transporters and nitrate reductases, all of which were otherwise considerably lower under high pH conditions. These data suggest that exogenous DMA not only plays an important role in facilitating the uptake of environmental Fe, but also orchestrates Fe and nitrate assimilation for optimal growth under high pH conditions."},"publication_date":"2015-01-16","publication_name":{"en":"The Plant Journal : for Cell and Molecular Biology","ja":"The Plant Journal : for Cell and Molecular Biology"},"volume":"Vol.81","number":"No.2","starting_page":"233","ending_page":"246","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1111/tpj.12722"],"issn":["1365-313X"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:45, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/25353377","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=286528","label":"url"}],"paper_title":{"en":"One-pot synthesis of tri- and tetrasubstituted pyridines by sequential ring-opening-cyclization-oxidation reaction of N-arylmethyl 3-aziridinylpropiolate esters","ja":"One-pot synthesis of tri- and tetrasubstituted pyridines by sequential ring-opening-cyclization-oxidation reaction of N-arylmethyl 3-aziridinylpropiolate esters"},"authors":{"en":[{"name":"Yoshida Masahiro"},{"name":"Mizuguchi Tomotaka"},{"name":"Namba Kosuke"}],"ja":[{"name":"吉田 昌裕"},{"name":"Mizuguchi Tomotaka"},{"name":"難波 康祐"}]},"description":{"en":"A novel strategy for the one-pot synthesis of substituted pyridines from N-arylmethyl 3-aziridinylpropiolate esters is described. The method employs a three-step procedure including the formation of allenyl imines, phosphine-catalyzed cyclization, and subsequent oxidation of the dihydropyridines. Depending on the reaction conditions of the final oxidation step, tri- and tetrasubstituted pyridines can be selectively produced.","ja":"A novel strategy for the one-pot synthesis of substituted pyridines from N-arylmethyl 3-aziridinylpropiolate esters is described. The method employs a three-step procedure including the formation of allenyl imines, phosphine-catalyzed cyclization, and subsequent oxidation of the dihydropyridines. Depending on the reaction conditions of the final oxidation step, tri- and tetrasubstituted pyridines can be selectively produced."},"publication_date":"2014-10-29","publication_name":{"en":"Angewandte Chemie International Edition","ja":"Angewandte Chemie International Edition"},"volume":"Vol.53","number":"No.52","starting_page":"14550","ending_page":"14554","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1002/anie.201409015"],"issn":["1521-3773"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:46, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-84905977663&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=281028","label":"url"}],"paper_title":{"en":"N-Acyl-N-tosylhydrazine as a Synthon To Construct Tetrasubstituted Carbon Centers Possessing a Nitrogen Group","ja":"N-Acyl-N-tosylhydrazine as a Synthon To Construct Tetrasubstituted Carbon Centers Possessing a Nitrogen Group"},"authors":{"en":[{"name":"Namba Kosuke"},{"name":"Shobo Yoshihiro"},{"name":"Fujimoto Kazuki"},{"name":"Shoji Isamu"},{"name":"Yoshida Masahiro"},{"name":"Tanino Keiji"}],"ja":[{"name":"難波 康祐"},{"name":"正保 好啓"},{"name":"藤本 夏月"},{"name":"東海林 勇"},{"name":"吉田 昌裕"},{"name":"谷野 圭持"}]},"publication_date":"2014-08","publication_name":{"en":"European Journal of Organic Chemistry","ja":"European Journal of Organic Chemistry"},"volume":"Vol.2014","number":"No.24","starting_page":"5196","ending_page":"5203","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1002/ejoc.201402650"],"issn":["1099-0690"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:47, {"insert":{"user_id":"5000093573","type":"published_papers","id":"33590266"},"force":{"see_also":[{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-84899921459&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=276104","label":"url"}],"paper_title":{"en":"Total synthesis of (-)-HM-3 and (-)-HM-4 utilizing a palladium-catalyzed addition of an arylboronic acid to an allenic alcohol-Eschenmoser-Claisen rearrangement","ja":"Total synthesis of (-)-HM-3 and (-)-HM-4 utilizing a palladium-catalyzed addition of an arylboronic acid to an allenic alcohol-Eschenmoser-Claisen rearrangement"},"authors":{"en":[{"name":"Yoshida Masahiro"},{"name":"Kasai Tomoyo"},{"name":"Mizuguti Tomotaka"},{"name":"Namba Kosuke"}],"ja":[{"name":"吉田 昌裕"},{"name":"笠井 知世"},{"name":"水口 智貴"},{"name":"難波 康祐"}]},"publication_date":"2014-03","publication_name":{"en":"Synlett","ja":"Synlett"},"volume":"Vol.25","number":"No.8","starting_page":"1160","ending_page":"1162","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1055/s-0033-1341059"],"issn":["1437-2096"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:48, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/24595409","label":"url"},{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-84896474986&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=275036","label":"url"}],"paper_title":{"en":"Synthesis of functionalized 2-vinyl-2,3-dihydropyrroles and 3-methylene-1,2,3,4-tetrahydropyridines by palladium-catalyzed cyclization of ß-enaminocarbonyl compounds with allylic bisacetates","ja":"Synthesis of functionalized 2-vinyl-2,3-dihydropyrroles and 3-methylene-1,2,3,4-tetrahydropyridines by palladium-catalyzed cyclization of ß-enaminocarbonyl compounds with allylic bisacetates"},"authors":{"en":[{"name":"Yoshida Masahiro"},{"name":"Kinoshita Kouki"},{"name":"Namba Kosuke"}],"ja":[{"name":"吉田 昌裕"},{"name":"木下 航輝"},{"name":"難波 康祐"}]},"description":{"en":"The N-Heterocyclic carbene-catalysed oxidative carboxylation of arylaldehydes with water successfully proceeded when a sulfoxylalkyl-substituted imidazolium salt was used as the catalyst. The reactions can be run in the absence of oxidant, and a variety of arylaldehydes having an electron-withdrawing group were converted to the corresponding carboxylic acids.","ja":"The N-Heterocyclic carbene-catalysed oxidative carboxylation of arylaldehydes with water successfully proceeded when a sulfoxylalkyl-substituted imidazolium salt was used as the catalyst. The reactions can be run in the absence of oxidant, and a variety of arylaldehydes having an electron-withdrawing group were converted to the corresponding carboxylic acids."},"publication_date":"2014-02-12","publication_name":{"en":"Organic & Biomolecular Chemistry","ja":"Organic & Biomolecular Chemistry"},"volume":"Vol.12","number":"No.15","starting_page":"2394","ending_page":"2403","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1039/C3OB42510J"],"issn":["1477-0539"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:49, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/24174159","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=272607","label":"url"}],"paper_title":{"en":"Synthesis of substituted tetrahydrocyclobuta[b]benzofurans by palladium-catalyzed domino substitution-[2+2] cycloaddition of propargylic carbonates with 2-vinylphenols","ja":"Synthesis of substituted tetrahydrocyclobuta[b]benzofurans by palladium-catalyzed domino substitution-[2+2] cycloaddition of propargylic carbonates with 2-vinylphenols"},"authors":{"en":[{"name":"Yoshida Masahiro"},{"name":"Ohno Shoko"},{"name":"Namba Kosuke"}],"ja":[{"name":"吉田 昌裕"},{"name":"Ohno Shoko"},{"name":"難波 康祐"}]},"description":{"en":"Radical methods: The title reaction proceeds in the presence of a palladium catalyst to deliver substituted tetrahydrocyclobuta[b]benzofurans in a stereoselective manner. A radical mechanism is discussed.","ja":"Radical methods: The title reaction proceeds in the presence of a palladium catalyst to deliver substituted tetrahydrocyclobuta[b]benzofurans in a stereoselective manner. A radical mechanism is discussed."},"publication_date":"2013-10","publication_name":{"en":"Angewandte Chemie International Edition","ja":"Angewandte Chemie International Edition"},"volume":"Vol.52","number":"No.51","starting_page":"13597","ending_page":"13600","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1002/anie.201306903"],"issn":["1521-3773"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:50, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-84872356621&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263633","label":"url"}],"paper_title":{"en":"Transformations of 1-(Oxiranylmethyl)-1,2,3-triazoles into 2-(Oxiranylmethyl)-1,2,3-triazoles and Alkanenitriles.","ja":"Transformations of 1-(Oxiranylmethyl)-1,2,3-triazoles into 2-(Oxiranylmethyl)-1,2,3-triazoles and Alkanenitriles."},"authors":{"en":[{"name":"Osawa Ayumi"},{"name":"Mera Akane"},{"name":"Namba Kosuke"},{"name":"Tanino Keiji"}],"ja":[{"name":"Osawa Ayumi"},{"name":"Mera Akane"},{"name":"難波 康祐"},{"name":"Tanino Keiji"}]},"publication_date":"2013","publication_name":{"en":"Synlett","ja":"Synlett"},"volume":"Vol.24","number":"No.2","starting_page":"207","ending_page":"210","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1055/s-0032-1317937"],"issn":["0936-5214"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:51, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"http://ci.nii.ac.jp/naid/40019465282/","label":"url"},{"@id":"https://cir.nii.ac.jp/crid/1523951030331176960/","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263634","label":"url"}],"paper_title":{"en":"Total Synthesis of Manzacidins. An Overview and Perspective","ja":"Total Synthesis of Manzacidins. An Overview and Perspective"},"authors":{"en":[{"name":"Ohfune Yasufumi"},{"name":"Oe Kentaro"},{"name":"Namba Kosuke"},{"name":"Shinada Tetsuro"}],"ja":[{"name":"Ohfune Yasufumi"},{"name":"Oe Kentaro"},{"name":"難波 康祐"},{"name":"Shinada Tetsuro"}]},"publication_date":"2012-11-01","publication_name":{"en":"Heterocycles","ja":"Heterocycles"},"volume":"Vol.85","number":"No.11","starting_page":"2617","ending_page":"2649","languages":["eng"],"referee":true,"identifiers":{"doi":["10.3987/REV-12-746"],"issn":["0385-5414"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:52, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"http://ci.nii.ac.jp/naid/120004883875/","label":"url"},{"@id":"https://cir.nii.ac.jp/crid/1050282813988714368/","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263631","label":"url"}],"paper_title":{"en":"Concise [4+3] cycloaddition reaction of pyrroles leading to tropinone derivatives","ja":"Concise [4+3] cycloaddition reaction of pyrroles leading to tropinone derivatives"},"authors":{"en":[{"name":"Fuchigami Ryuichi"},{"name":"Namba Kosuke"},{"name":"Tanino Keiji"}],"ja":[{"name":"Fuchigami Ryuichi"},{"name":"難波 康祐"},{"name":"Tanino Keiji"}]},"description":{"en":"A concise [4+3] cycloaddition reaction of pyrroles with 2-(silyloxy)allyl cations has been developed. The oxyallyl cations stabilized with a methylthio group or geminal methyl groups were generated from the corresponding allylic alcohols under the influence of a Brönsted acid (Tf2NH), respectively. The use of N-nosyl-protected pyrroles as the four-carbon unit was found to give tropinone derivatives in high yield.","ja":"A concise [4+3] cycloaddition reaction of pyrroles with 2-(silyloxy)allyl cations has been developed. The oxyallyl cations stabilized with a methylthio group or geminal methyl groups were generated from the corresponding allylic alcohols under the influence of a Brönsted acid (Tf2NH), respectively. The use of N-nosyl-protected pyrroles as the four-carbon unit was found to give tropinone derivatives in high yield."},"publication_date":"2012-10-24","publication_name":{"en":"Tetrahedron Letters","ja":"Tetrahedron Letters"},"volume":"Vol.53","number":"No.43","starting_page":"5725","ending_page":"5728","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1016/j.tetlet.2012.07.130"],"issn":["0040-4039"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:53, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/23072579","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263632","label":"url"}],"paper_title":{"en":"One-pot Synthesis of Highly Fluorescent 2,5-Disubstituted-1,3a,6a-triazapentalene.","ja":"One-pot Synthesis of Highly Fluorescent 2,5-Disubstituted-1,3a,6a-triazapentalene."},"authors":{"en":[{"name":"Namba Kosuke"},{"name":"Mera Akane"},{"name":"Osawa Ayumi"},{"name":"Sakuda Eri"},{"name":"Kitamura Noboru"},{"name":"Tanino Keiji"}],"ja":[{"name":"難波 康祐"},{"name":"Mera Akane"},{"name":"Osawa Ayumi"},{"name":"Sakuda Eri"},{"name":"Kitamura Noboru"},{"name":"Tanino Keiji"}]},"description":{"en":"A one-pot synthetic method was established for the preparation of 2,5-disubstituted-1,3a,6a-triazapentalenes. The fluorescence observation of the synthetic 2,5-disubstituted-1,3a,6a-triazapentalenes revealed that the introduction of a substituent at the C5 position allowed a substantial change in the fluorescence quantum yield with little effect on the fluorescence wavelength.","ja":"A one-pot synthetic method was established for the preparation of 2,5-disubstituted-1,3a,6a-triazapentalenes. The fluorescence observation of the synthetic 2,5-disubstituted-1,3a,6a-triazapentalenes revealed that the introduction of a substituent at the C5 position allowed a substantial change in the fluorescence quantum yield with little effect on the fluorescence wavelength."},"publication_date":"2012-10-16","publication_name":{"en":"Organic Letters","ja":"Organic Letters"},"volume":"Vol.14","number":"No.21","starting_page":"5554","ending_page":"5557","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1021/ol302668y"],"issn":["1523-7052"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:54, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/22339178","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263629","label":"url"}],"paper_title":{"en":"Hg(OTf)2-Catalyzed Vinylogous Semi-Pinacol Rearrangement Leading to 1,4-Dihydroquinolines.","ja":"Hg(OTf)2-Catalyzed Vinylogous Semi-Pinacol Rearrangement Leading to 1,4-Dihydroquinolines."},"authors":{"en":[{"name":"Namba Kosuke"},{"name":"Kanaki Michika"},{"name":"Suto Hiroki"},{"name":"Nishizawa Mugio"},{"name":"Tanino Keiji"}],"ja":[{"name":"難波 康祐"},{"name":"Kanaki Michika"},{"name":"Suto Hiroki"},{"name":"Nishizawa Mugio"},{"name":"Tanino Keiji"}]},"description":{"en":"An efficient method for the construction of dihydroquinoline derivatives possessing a quaternary carbon center is developed by an application of Hg(OTf)(2)-catalyzed vinylogous semi-pinacol-type rearrangement. The reaction was found to be specifically catalyzed by mercury salt and to proceed via a bicyclic aminal.","ja":"An efficient method for the construction of dihydroquinoline derivatives possessing a quaternary carbon center is developed by an application of Hg(OTf)(2)-catalyzed vinylogous semi-pinacol-type rearrangement. The reaction was found to be specifically catalyzed by mercury salt and to proceed via a bicyclic aminal."},"publication_date":"2012-02-16","publication_name":{"en":"Organic Letters","ja":"Organic Letters"},"volume":"Vol.14","number":"No.5","starting_page":"1222","ending_page":"1225","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1021/ol2034492"],"issn":["1523-7052"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:55, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263630","label":"url"}],"paper_title":{"en":"Carbon-Nitrogen Bond Formation Between Allyl Silyl Ether and Hydrazide Promoted by Mercuric Triflate Catalyst.","ja":"Carbon-Nitrogen Bond Formation Between Allyl Silyl Ether and Hydrazide Promoted by Mercuric Triflate Catalyst."},"authors":{"en":[{"name":"Yamamoto Hirofumi"},{"name":"Yamasaki N."},{"name":"Yoshidome S."},{"name":"Sasaki Ikuo"},{"name":"Namba Kosuke"},{"name":"Imagawa Hiroshi"},{"name":"Nishizawa Mugio"}],"ja":[{"name":"Yamamoto Hirofumi"},{"name":"Yamasaki N."},{"name":"Yoshidome S."},{"name":"Sasaki Ikuo"},{"name":"難波 康祐"},{"name":"Imagawa Hiroshi"},{"name":"Nishizawa Mugio"}]},"publication_date":"2012","publication_name":{"en":"Synlett","ja":"Synlett"},"volume":"Vol.23","number":"No.7","starting_page":"1069","ending_page":"1073","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1055/s-0031-1290758"],"issn":["0936-5214"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:56, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/21736311","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263628","label":"url"}],"paper_title":{"en":"Direct Synthesis of Fluorescent 1,3a,6a-Triazazapentalene Derivatives via Click-Cyclization-Aromatization Cascade Reaction.","ja":"Direct Synthesis of Fluorescent 1,3a,6a-Triazazapentalene Derivatives via Click-Cyclization-Aromatization Cascade Reaction."},"authors":{"en":[{"name":"Namba Kosuke"},{"name":"Osawa Ayumi"},{"name":"Ishizaka Shoji"},{"name":"Kitamura Noboru"},{"name":"Tanino Keiji"}],"ja":[{"name":"難波 康祐"},{"name":"Osawa Ayumi"},{"name":"Ishizaka Shoji"},{"name":"Kitamura Noboru"},{"name":"Tanino Keiji"}]},"description":{"en":"An efficient and versatile method was established for the preparation of 1,3a,6a-triazapentalenes. The 1,3a,6a-triazapentalene skeleton without an additional fused ring system was discovered to be a compact and highly fluorescent chromophore, which exhibited various interesting fluorescent properties such as a noteworthy correlation of luminescent wavelength with the Hammett ς(p) value and a strongly positive solvatofluorochromism.","ja":"An efficient and versatile method was established for the preparation of 1,3a,6a-triazapentalenes. The 1,3a,6a-triazapentalene skeleton without an additional fused ring system was discovered to be a compact and highly fluorescent chromophore, which exhibited various interesting fluorescent properties such as a noteworthy correlation of luminescent wavelength with the Hammett ς(p) value and a strongly positive solvatofluorochromism."},"publication_date":"2011-07-13","publication_name":{"en":"Journal of the American Chemical Society","ja":"Journal of the American Chemical Society"},"volume":"Vol.133","number":"No.30","starting_page":"11466","ending_page":"11469","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1021/ja203917r"],"issn":["1520-5126"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:57, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/21108292","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263626","label":"url"}],"paper_title":{"en":"Mugineic acid derivatives as molecular probes for the mechanistic elucidation of iron acquisition in barley.","ja":"Mugineic acid derivatives as molecular probes for the mechanistic elucidation of iron acquisition in barley."},"authors":{"en":[{"name":"Namba Kosuke"},{"name":"Kobayashi Kaori"},{"name":"Murata Yoshiko"},{"name":"Hirakawa Hiroko"},{"name":"Yamagaki T."},{"name":"Iwashita Takashi"},{"name":"Nishizawa Mugio"},{"name":"Kusumoto Shoichi"},{"name":"Tanino Keiji"}],"ja":[{"name":"難波 康祐"},{"name":"Kobayashi Kaori"},{"name":"Murata Yoshiko"},{"name":"Hirakawa Hiroko"},{"name":"Yamagaki T."},{"name":"Iwashita Takashi"},{"name":"Nishizawa Mugio"},{"name":"Kusumoto Shoichi"},{"name":"Tanino Keiji"}]},"publication_date":"2010-12-17","publication_name":{"en":"Angewandte Chemie International Edition","ja":"Angewandte Chemie International Edition"},"volume":"Vol.49","number":"No.51","starting_page":"9956","ending_page":"9959","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1002/anie.201004853"],"issn":["1521-3773"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:58, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/21286237","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263627","label":"url"}],"paper_title":{"en":"Synthetic Studies on Palauamine. Construction of the Cyclopentane Core via an Asymmetric [1,3]-Dipolar Cycloaddition.","ja":"Synthetic Studies on Palauamine. Construction of the Cyclopentane Core via an Asymmetric [1,3]-Dipolar Cycloaddition."},"authors":{"en":[{"name":"Namba Kosuke"},{"name":"Inai Makoto"},{"name":"Sundermeier Uta"},{"name":"Williams M. Robert"}],"ja":[{"name":"難波 康祐"},{"name":"Inai Makoto"},{"name":"Sundermeier Uta"},{"name":"Williams M. Robert"}]},"description":{"en":"The cyclopentane core of palau'amine has been constructed in optically pure form through the use of an asymmetric azomethine ylid [1,3]-dipolar cycloaddition reaction.","ja":"The cyclopentane core of palau'amine has been constructed in optically pure form through the use of an asymmetric azomethine ylid [1,3]-dipolar cycloaddition reaction."},"publication_date":"2010-12-15","publication_name":{"en":"Tetrahedron Letters","ja":"Tetrahedron Letters"},"volume":"Vol.51","starting_page":"6557","ending_page":"6559","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1016/j.tetlet.2010.10.037"],"issn":["0040-4039"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:59, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"http://ci.nii.ac.jp/naid/10027409394/","label":"url"},{"@id":"https://cir.nii.ac.jp/crid/1390001205312278400/","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263635","label":"url"}],"paper_title":{"en":"Development of Practical Synthetic Method toward Mechanistic Elucidation of Biologically Active Natural Products","ja":"生物活性天然有機化合物の機能解明を指向した実践的合成手法の開発"},"authors":{"en":[{"name":"Namba Kosuke"}],"ja":[{"name":"難波 康祐"}]},"description":{"en":"The limited supplies of biologically active natural products from natural source have been a severe bottleneck for their application to medical care or mechanistic study of their functions. Synthetic organic chemistry may become a best possible solution of this supply problem by the development of practical synthetic methods suited to the intended molecules. For right-half of halichondrin B, we established a new catalytic cycle of Cr-mediated coupling reaction, new asymmetric Ni/Cr-mediated coupling reaction, surprisingly efficient catalytic Cr-mediated coupling reaction, catalytic Ni/Cr-mediated macrocyclization without use of high-dilution techniques, and effective device for forming polycyclic ring system of halichondrin B. For mugineic acid, we established the practical synthesis of 2'-deoxy mugineic acid with minimal requirements for workup and purification procedure, efficient synthesis of mugineic acid, and synthesis of mugineic acid derivatives as molecular probes. For E-ring of palau'amine, we established Hg(OTf)2-catalyzed olefin cyclization reactions, and its application to the construction of tetra-substituted carbon center possessing nitrogen that corresponds to C16 position of palau'amine.","ja":"The limited supplies of biologically active natural products from natural source have been a severe bottleneck for their application to medical care or mechanistic study of their functions. Synthetic organic chemistry may become a best possible solution of this supply problem by the development of practical synthetic methods suited to the intended molecules. For right-half of halichondrin B, we established a new catalytic cycle of Cr-mediated coupling reaction, new asymmetric Ni/Cr-mediated coupling reaction, surprisingly efficient catalytic Cr-mediated coupling reaction, catalytic Ni/Cr-mediated macrocyclization without use of high-dilution techniques, and effective device for forming polycyclic ring system of halichondrin B. For mugineic acid, we established the practical synthesis of 2'-deoxy mugineic acid with minimal requirements for workup and purification procedure, efficient synthesis of mugineic acid, and synthesis of mugineic acid derivatives as molecular probes. For E-ring of palau'amine, we established Hg(OTf)2-catalyzed olefin cyclization reactions, and its application to the construction of tetra-substituted carbon center possessing nitrogen that corresponds to C16 position of palau'amine."},"publication_date":"2010-12-01","publication_name":{"en":"Journal of Synthetic Organic Chemistry, Japan","ja":"有機合成化学協会誌"},"volume":"Vol.68","starting_page":"1249","ending_page":"1260","languages":["jpn"],"referee":true,"invited":true,"identifiers":{"doi":["10.5059/yukigoseikyokaishi.68.1249"],"issn":["0037-9980"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:60, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/20730843","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263622","label":"url"}],"paper_title":{"en":"Hg(OTf)2-BINAPHANE-Catalyzed Enantioselective Anilino Sulfonamide Allyl Alcohol Cyclization.","ja":"Hg(OTf)2-BINAPHANE-Catalyzed Enantioselective Anilino Sulfonamide Allyl Alcohol Cyclization."},"authors":{"en":[{"name":"Yamamoto Hirofumi"},{"name":"Ho Elizabeth"},{"name":"Namba Kosuke"},{"name":"Imagawa Hiroshi"},{"name":"Nishizawa Mugio"}],"ja":[{"name":"Yamamoto Hirofumi"},{"name":"Ho Elizabeth"},{"name":"難波 康祐"},{"name":"Imagawa Hiroshi"},{"name":"Nishizawa Mugio"}]},"publication_date":"2010-10-04","publication_name":{"en":"Chemistry - A European Journal","ja":"Chemistry - A European Journal"},"volume":"Vol.16","number":"No.37","starting_page":"11271","ending_page":"11274","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1002/chem.201001656"],"issn":["1521-3765"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:61, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"http://ci.nii.ac.jp/naid/10027183656/","label":"url"},{"@id":"https://cir.nii.ac.jp/crid/1390001204584263040/","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263624","label":"url"}],"paper_title":{"en":"Hg(OTf)2-Catalyzed Cycloisomerization of Aryl- and Hetero- Substituted 1,3-Dienes.","ja":"Hg(OTf)2-Catalyzed Cycloisomerization of Aryl- and Hetero- Substituted 1,3-Dienes."},"authors":{"en":[{"name":"Nishizawa Mugio"},{"name":"Shiomi Shinya"},{"name":"Odate Daiki"},{"name":"Sasaki Ikuo"},{"name":"Namba Kosuke"},{"name":"Yamamoto Hirofumi"},{"name":"Imagawa Hiroshi"}],"ja":[{"name":"Nishizawa Mugio"},{"name":"Shiomi Shinya"},{"name":"Odate Daiki"},{"name":"Sasaki Ikuo"},{"name":"難波 康祐"},{"name":"Yamamoto Hirofumi"},{"name":"Imagawa Hiroshi"}]},"publication_date":"2010-08-05","publication_name":{"en":"Chemistry Letters","ja":"Chemistry Letters"},"volume":"Vol.39","number":"No.8","starting_page":"830","ending_page":"831","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1246/cl.2010.830"],"issn":["0366-7022"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:62, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/20354995","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263621","label":"url"}],"paper_title":{"en":"Toward Mechanistic Elucidation of Iron Acquisition in Barley: Efficient Synthesis of Mugineic Acids and Their Transport Activities.","ja":"Toward Mechanistic Elucidation of Iron Acquisition in Barley: Efficient Synthesis of Mugineic Acids and Their Transport Activities."},"authors":{"en":[{"name":"Namba Kosuke"},{"name":"Murata Yoshiko"}],"ja":[{"name":"難波 康祐"},{"name":"Murata Yoshiko"}]},"description":{"en":"Iron acquisition of graminaceous plants is characterized by the synthesis and secretion of iron-chelating compounds, mugineic acids (MAs), and by a specific uptake system for MAs-iron(III) complexes. We identified a transporter, HvYS1 (Hordeum vulgare L. yellow stripe 1), that is highly specific for MAs-iron(III) in barley roots. In this article we outline the characterization of HvYS1, and our recent work on the practical syntheses of MAs and investigations into the molecular basis of the specific transport of their iron(III) complexes by HvYS1. 2'-Deoxymugineic acid (DMA) was synthesized in a good overall yield from commercially available Boc-l-allylglycine using a minimal number of short simple operations with minimal protecting groups and work-up/purification procedures. The same strategy was also successfully applied to beta-hydroxy-l-allylglycine, which was obtained by an allylic oxidation of l-allylglycine derivatives, to give MA and 2'-epi-MA efficiently. HvYS1 transported the iron(III) complexes of all three synthetic specimens with efficiency similar to that of a natural mugineic acid complex. With sufficient quantities of MAs in hand, we analyzed the function of HvYS1 and revealed by preparing chimeric transporters that the sixth outer membrane loop of the transporter plays a vital role in substrate specificity.","ja":"Iron acquisition of graminaceous plants is characterized by the synthesis and secretion of iron-chelating compounds, mugineic acids (MAs), and by a specific uptake system for MAs-iron(III) complexes. We identified a transporter, HvYS1 (Hordeum vulgare L. yellow stripe 1), that is highly specific for MAs-iron(III) in barley roots. In this article we outline the characterization of HvYS1, and our recent work on the practical syntheses of MAs and investigations into the molecular basis of the specific transport of their iron(III) complexes by HvYS1. 2'-Deoxymugineic acid (DMA) was synthesized in a good overall yield from commercially available Boc-l-allylglycine using a minimal number of short simple operations with minimal protecting groups and work-up/purification procedures. The same strategy was also successfully applied to beta-hydroxy-l-allylglycine, which was obtained by an allylic oxidation of l-allylglycine derivatives, to give MA and 2'-epi-MA efficiently. HvYS1 transported the iron(III) complexes of all three synthetic specimens with efficiency similar to that of a natural mugineic acid complex. With sufficient quantities of MAs in hand, we analyzed the function of HvYS1 and revealed by preparing chimeric transporters that the sixth outer membrane loop of the transporter plays a vital role in substrate specificity."},"publication_date":"2010-04","publication_name":{"en":"Chemical Record","ja":"Chemical Record"},"volume":"Vol.10","number":"No.2","starting_page":"140","ending_page":"150","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1002/tcr.200900028"],"issn":["1528-0691"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:63, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/19795873","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263620","label":"url"}],"paper_title":{"en":"4-Aminopyridines-Catalyzed Direct and Regioselective Acylation of N-Tosylhydrazide","ja":"4-Aminopyridines-Catalyzed Direct and Regioselective Acylation of N-Tosylhydrazide"},"authors":{"en":[{"name":"Namba Kosuke"},{"name":"Shoji Isamu"},{"name":"Nishizawa Mugio"},{"name":"Tanino Keiji"}],"ja":[{"name":"難波 康祐"},{"name":"Shoji Isamu"},{"name":"Nishizawa Mugio"},{"name":"Tanino Keiji"}]},"description":{"en":"An efficient and simple method for selective acylation of either one of two nitrogen atoms of tosylhydrazide was developed. The selectivity was drastically controlled by a catalytic amount of 4-aminopyridine or 4-(dimethylamino)pyridine with common acylating agents. The nitrogen atom masked with a tosyl group was acylated in the presence of 4-aminopyridine, whereas the primary nitrogen atom was acylated in the absence of 4-aminopyridine.","ja":"An efficient and simple method for selective acylation of either one of two nitrogen atoms of tosylhydrazide was developed. The selectivity was drastically controlled by a catalytic amount of 4-aminopyridine or 4-(dimethylamino)pyridine with common acylating agents. The nitrogen atom masked with a tosyl group was acylated in the presence of 4-aminopyridine, whereas the primary nitrogen atom was acylated in the absence of 4-aminopyridine."},"publication_date":"2009-11-05","publication_name":{"en":"Organic Letters","ja":"Organic Letters"},"volume":"Vol.11","number":"No.21","starting_page":"4970","ending_page":"4973","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1021/ol9021194"],"issn":["1523-7052"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:64, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/19492366","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263618","label":"url"}],"paper_title":{"en":"Toward Palauamine; Hg(OTf)2-Catalyzed Synthesis of Cyclopentane Core.","ja":"Toward Palauamine; Hg(OTf)2-Catalyzed Synthesis of Cyclopentane Core."},"authors":{"en":[{"name":"Namba Kosuke"},{"name":"Kaihara Yukari"},{"name":"Yamamoto Hirofumi"},{"name":"Imagawa Hiroshi"},{"name":"Tanino Keiji"},{"name":"Williams M. Robert"},{"name":"Nishizawa Mugio"}],"ja":[{"name":"難波 康祐"},{"name":"Kaihara Yukari"},{"name":"Yamamoto Hirofumi"},{"name":"Imagawa Hiroshi"},{"name":"Tanino Keiji"},{"name":"Williams M. Robert"},{"name":"Nishizawa Mugio"}]},"publication_date":"2009-07-06","publication_name":{"en":"Chemistry - A European Journal","ja":"Chemistry - A European Journal"},"volume":"Vol.15","number":"No.27","starting_page":"6560","ending_page":"6563","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1002/chem.200900622"],"issn":["1521-3765"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:65, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/19128191","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263612","label":"url"}],"paper_title":{"en":"Attempts to Improve the Overall Stereoselectivity of Ireland-Claisen Rearrangement","ja":"Attempts to Improve the Overall Stereoselectivity of Ireland-Claisen Rearrangement"},"authors":{"en":[{"name":"Chen C-L."},{"name":"Namba Kosuke"},{"name":"Kishi Yoshito"}],"ja":[{"name":"Chen C-L."},{"name":"難波 康祐"},{"name":"Kishi Yoshito"}]},"description":{"en":"With focus on the steric effects present in the transition states for the [3,3]-sigmatropic rearrangement, the substrate 5 has been designed to improve the overall stereoselectivity of the Ireland-Claisen rearrangement. Experimentally, it has been found that (1) only Z-6 rearranges to 7 at 80 degrees C and (2) E-6 isomerizes to Z-6 at 80 degrees C, thereby allowing the transformation of 5 into 7 in an almost quantitative yield. To illustrate the usefulness of this approach, two additional examples are given.","ja":"With focus on the steric effects present in the transition states for the [3,3]-sigmatropic rearrangement, the substrate 5 has been designed to improve the overall stereoselectivity of the Ireland-Claisen rearrangement. Experimentally, it has been found that (1) only Z-6 rearranges to 7 at 80 degrees C and (2) E-6 isomerizes to Z-6 at 80 degrees C, thereby allowing the transformation of 5 into 7 in an almost quantitative yield. To illustrate the usefulness of this approach, two additional examples are given."},"publication_date":"2009-01-15","publication_name":{"en":"Organic Letters","ja":"Organic Letters"},"volume":"Vol.11","number":"No.2","starting_page":"409","ending_page":"412","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1021/ol8027225"],"issn":["1523-7052"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:66, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263616","label":"url"}],"paper_title":{"en":"Hg(OTf)2-Catalyzed Instantaneous Hydration of β- and δ-Hydroxy Internal Alkynes with Complete Regioselectivity","ja":"Hg(OTf)2-Catalyzed Instantaneous Hydration of β- and δ-Hydroxy Internal Alkynes with Complete Regioselectivity"},"authors":{"en":[{"name":"Nishizawa Mugio"},{"name":"Takemoto T."},{"name":"Sasaki Ikuo"},{"name":"Nakano Mayo"},{"name":"Ho Elizabeth"},{"name":"Namba Kosuke"},{"name":"Yamamoto Hirofumi"},{"name":"Imagawa Hiroshi"}],"ja":[{"name":"Nishizawa Mugio"},{"name":"Takemoto T."},{"name":"Sasaki Ikuo"},{"name":"Nakano Mayo"},{"name":"Ho Elizabeth"},{"name":"難波 康祐"},{"name":"Yamamoto Hirofumi"},{"name":"Imagawa Hiroshi"}]},"publication_date":"2009","publication_name":{"en":"Synlett","ja":"Synlett"},"starting_page":"1175","ending_page":"1179","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1055/s-0028-1088153"],"issn":["0936-5214"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:67, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/19137523","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263614","label":"url"}],"paper_title":{"en":"Silaphenylmercuric Triflate-Catalyzed Reactions: The First Solid Supported Mercuric Salt Catalyst.","ja":"Silaphenylmercuric Triflate-Catalyzed Reactions: The First Solid Supported Mercuric Salt Catalyst."},"authors":{"en":[{"name":"Yamamoto Hirofumi"},{"name":"Sasaki Ikuo"},{"name":"Hirai Y"},{"name":"Namba Kosuke"},{"name":"Imagawa Hiroshi"},{"name":"Nishizawa Mugio"}],"ja":[{"name":"Yamamoto Hirofumi"},{"name":"Sasaki Ikuo"},{"name":"Hirai Y"},{"name":"難波 康祐"},{"name":"Imagawa Hiroshi"},{"name":"Nishizawa Mugio"}]},"description":{"en":"Let it flow, let it flow: A procedure to generate the first solid-supported mercuric salt, silaphenylmercuric triflate, is described. Silaphenylmercuric triflate showed remarkable catalytic activity for an indole synthesis, furanoyne cyclization, arylyne cyclization, and tandem carbocyclizations. An efficient flow reaction system for indole synthesis and arylyne cyclization is also described (see figure).","ja":"Let it flow, let it flow: A procedure to generate the first solid-supported mercuric salt, silaphenylmercuric triflate, is described. Silaphenylmercuric triflate showed remarkable catalytic activity for an indole synthesis, furanoyne cyclization, arylyne cyclization, and tandem carbocyclizations. An efficient flow reaction system for indole synthesis and arylyne cyclization is also described (see figure)."},"publication_date":"2009","publication_name":{"en":"Angewandte Chemie International Edition","ja":"Angewandte Chemie International Edition"},"volume":"Vol.48","starting_page":"1244","ending_page":"1247","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1002/anie.200804641"],"issn":["1521-3773"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:68, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/18396886","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263599","label":"url"}],"paper_title":{"en":"Hg(OTf)2-Catalyzed Arylene Cyclization.","ja":"Hg(OTf)2-Catalyzed Arylene Cyclization."},"authors":{"en":[{"name":"Namba Kosuke"},{"name":"Yamamoto Hirofumi"},{"name":"Sasaki Ikuo"},{"name":"Mori Kumiko"},{"name":"Imagawa Hiroshi"},{"name":"Nishizawa Mugio"}],"ja":[{"name":"難波 康祐"},{"name":"Yamamoto Hirofumi"},{"name":"Sasaki Ikuo"},{"name":"Mori Kumiko"},{"name":"Imagawa Hiroshi"},{"name":"Nishizawa Mugio"}]},"description":{"en":"Novel Hg(OTf) 2-catalyzed arylene cyclization was achieved with highly efficient catalytic turnover (up to 200 times). The reaction takes place via protonation of allylic hydroxyl group by in situ formed TfOH of an organomercuric intermediate to generate a cationic species. Subsequent smooth demercuration regenerates the catalyst.","ja":"Novel Hg(OTf) 2-catalyzed arylene cyclization was achieved with highly efficient catalytic turnover (up to 200 times). The reaction takes place via protonation of allylic hydroxyl group by in situ formed TfOH of an organomercuric intermediate to generate a cationic species. Subsequent smooth demercuration regenerates the catalyst."},"publication_date":"2008-04-09","publication_name":{"en":"Organic Letters","ja":"Organic Letters"},"volume":"Vol.10","number":"No.9","starting_page":"1767","ending_page":"1770","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1021/ol800450x"],"issn":["1523-7060"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:69, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263603","label":"url"}],"paper_title":{"en":"Efficient Glycosylation Using ODS Adsorption Method Based on the Affinity of Long Alkoxybenzyl Glycoside.","ja":"Efficient Glycosylation Using ODS Adsorption Method Based on the Affinity of Long Alkoxybenzyl Glycoside."},"authors":{"en":[{"name":"Imagawa Hiroshi"},{"name":"Kinoshita Atsushi"},{"name":"Yamamoto Hirofumi"},{"name":"Namba Kosuke"},{"name":"Nishizawa Mugio"}],"ja":[{"name":"Imagawa Hiroshi"},{"name":"Kinoshita Atsushi"},{"name":"Yamamoto Hirofumi"},{"name":"難波 康祐"},{"name":"Nishizawa Mugio"}]},"publication_date":"2008","publication_name":{"en":"Synlett","ja":"Synlett"},"starting_page":"1981","ending_page":"1984","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1055/s-2008-1077948"],"issn":["0936-5214"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:70, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263602","label":"url"}],"paper_title":{"en":"Hg(OTf)2-Catalyzed Cyclization of N-Tosylanilinoallylic Alcohols to 2-Vinylindolines","ja":"Hg(OTf)2-Catalyzed Cyclization of N-Tosylanilinoallylic Alcohols to 2-Vinylindolines"},"authors":{"en":[{"name":"Namba Kosuke"},{"name":"Nakagawa Yuki"},{"name":"Yamamoto Hirofumi"},{"name":"Imagawa Hiroshi"},{"name":"Nishizawa Mugio"}],"ja":[{"name":"難波 康祐"},{"name":"Nakagawa Yuki"},{"name":"Yamamoto Hirofumi"},{"name":"Imagawa Hiroshi"},{"name":"Nishizawa Mugio"}]},"publication_date":"2008","publication_name":{"en":"Synlett","ja":"Synlett"},"volume":"Vol.11","starting_page":"1719","ending_page":"1723","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1055/s-2008-1077881"],"issn":["0936-5214"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:71, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263597","label":"url"}],"paper_title":{"en":"A specific transporter for iron (III)-phytosiderophore complex involved iron acquisition by bareley roots.","ja":"A specific transporter for iron (III)-phytosiderophore complex involved iron acquisition by bareley roots."},"authors":{"en":[{"name":"Murata Yoshiko"},{"name":"Harada Emiko"},{"name":"Sugase Kenji"},{"name":"Namba Kosuke"},{"name":"Horikawa Manabu"},{"name":"Ma J.-F."},{"name":"Yamaji Nahoko"},{"name":"Ueno D."},{"name":"Nomoko Kyosuke"},{"name":"Iwashita Takashi"},{"name":"Kusumoto Shoichi"}],"ja":[{"name":"Murata Yoshiko"},{"name":"Harada Emiko"},{"name":"Sugase Kenji"},{"name":"難波 康祐"},{"name":"Horikawa Manabu"},{"name":"Ma J.-F."},{"name":"Yamaji Nahoko"},{"name":"Ueno D."},{"name":"Nomoko Kyosuke"},{"name":"Iwashita Takashi"},{"name":"Kusumoto Shoichi"}]},"publication_date":"2008","publication_name":{"en":"Pure and Applied Chemistry","ja":"Pure and Applied Chemistry"},"volume":"Vol.80","number":"No.12","starting_page":"2689","ending_page":"2697","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1351/pac200880122689"],"issn":["0033-4545"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:72, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/18041847","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263595","label":"url"}],"paper_title":{"en":"Virtually Complete E-Selective -Unsaturated Ester Synthesis by Hg(OTf)2-Catalyzed Hydration of sec-Ethoxyalkynyl Acetate.","ja":"Virtually Complete E-Selective -Unsaturated Ester Synthesis by Hg(OTf)2-Catalyzed Hydration of sec-Ethoxyalkynyl Acetate."},"authors":{"en":[{"name":"Nishizawa Mugio"},{"name":"Hirakawa Hiroko"},{"name":"Nakagawa Yuki"},{"name":"Yamamoto Hirofumi"},{"name":"Namba Kosuke"},{"name":"Imagawa Hiroshi"}],"ja":[{"name":"Nishizawa Mugio"},{"name":"Hirakawa Hiroko"},{"name":"Nakagawa Yuki"},{"name":"Yamamoto Hirofumi"},{"name":"難波 康祐"},{"name":"Imagawa Hiroshi"}]},"description":{"en":"The reaction of alkyl-substituted sec-ethoxyalkynyl acetates with water catalyzed by Hg(OTf)2 afforded alpha,beta-unsaturated esters in excellent yield with high catalytic turnover up to 1000 times under very mild reaction conditions with virtually complete E-selectivity, superior even to that of the HWE reaction.","ja":"The reaction of alkyl-substituted sec-ethoxyalkynyl acetates with water catalyzed by Hg(OTf)2 afforded alpha,beta-unsaturated esters in excellent yield with high catalytic turnover up to 1000 times under very mild reaction conditions with virtually complete E-selectivity, superior even to that of the HWE reaction."},"publication_date":"2007-11-28","publication_name":{"en":"Organic Letters","ja":"Organic Letters"},"volume":"Vol.9","number":"No.26","starting_page":"5577","ending_page":"5580","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1021/ol702548r"],"issn":["1523-7060"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:73, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/17764194","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263592","label":"url"}],"paper_title":{"en":"Catalytic Activation of the Leaving Group in the SN2 Reaction.","ja":"Catalytic Activation of the Leaving Group in the SN2 Reaction."},"authors":{"en":[{"name":"Yamamoto Hirofumi"},{"name":"Pandey G."},{"name":"Asai Yumiko"},{"name":"Nakano Mayo"},{"name":"Kinoshita Atsushi"},{"name":"Namba Kosuke"},{"name":"Imagawa Hiroshi"},{"name":"Nishizawa Mugio"}],"ja":[{"name":"Yamamoto Hirofumi"},{"name":"Pandey G."},{"name":"Asai Yumiko"},{"name":"Nakano Mayo"},{"name":"Kinoshita Atsushi"},{"name":"難波 康祐"},{"name":"Imagawa Hiroshi"},{"name":"Nishizawa Mugio"}]},"description":{"en":"A novel catalytic activation of the leaving group in the S(N)2 reaction is achieved as an extension of our mercuric triflate-catalyzed reactions. Derivatives of anilinoethyl 4-pentynoate reacted smoothly with catalytic amounts of Hg(OTf)(2) to give indoline derivatives in excellent yield with efficient catalytic turnovers under very mild conditions. The reaction of optically pure secondary alcohol derivatives resulted in inversion of stereochemistry, which is a definitive feature of the S(N)2 reaction. The procedure is applicable for benzoazepine synthesis.","ja":"A novel catalytic activation of the leaving group in the S(N)2 reaction is achieved as an extension of our mercuric triflate-catalyzed reactions. Derivatives of anilinoethyl 4-pentynoate reacted smoothly with catalytic amounts of Hg(OTf)(2) to give indoline derivatives in excellent yield with efficient catalytic turnovers under very mild conditions. The reaction of optically pure secondary alcohol derivatives resulted in inversion of stereochemistry, which is a definitive feature of the S(N)2 reaction. The procedure is applicable for benzoazepine synthesis."},"publication_date":"2007-09-01","publication_name":{"en":"Organic Letters","ja":"Organic Letters"},"volume":"Vol.9","number":"No.20","starting_page":"4029","ending_page":"4032","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1021/ol701737x"],"issn":["1523-7060"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:74, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/17707820","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263590","label":"url"}],"paper_title":{"en":"Structural element responsible for the Fe(III)-specific transport as phytosiderophore complex by HvYS1 transporter of barley.","ja":"Structural element responsible for the Fe(III)-specific transport as phytosiderophore complex by HvYS1 transporter of barley."},"authors":{"en":[{"name":"Harada Emiko"},{"name":"Sugase Kenji"},{"name":"Namba Kosuke"},{"name":"Iwashita Takashi"},{"name":"Yoshiko Murata"}],"ja":[{"name":"Harada Emiko"},{"name":"Sugase Kenji"},{"name":"難波 康祐"},{"name":"Iwashita Takashi"},{"name":"Yoshiko Murata"}]},"description":{"en":"Hordeum vulgare L. yellow stripe 1 (HvYS1) is a selective transporter for Fe(III)-phytosiderophores, involved in primary iron acquisition from soils in barley roots. In contrast, Zea mays yellow stripe 1 (ZmYS1) in maize possesses broad substrate specificity, despite a high homology with HvYS1. Here we revealed, by assessing the transport activity of a series of HvYS1-ZmYS1 chimeras, that the outer membrane loop between the sixth and seventh transmembrane regions is essential for substrate specificity. Circular dichroism spectra indicated that a synthetic peptide corresponding to the loop of HvYS1 forms an alpha-helix in solution, whereas that of ZmYS1 is flexible. We propose that the structural difference at this particular loop determines the substrate specificity of the HvYS1 transporter.","ja":"Hordeum vulgare L. yellow stripe 1 (HvYS1) is a selective transporter for Fe(III)-phytosiderophores, involved in primary iron acquisition from soils in barley roots. In contrast, Zea mays yellow stripe 1 (ZmYS1) in maize possesses broad substrate specificity, despite a high homology with HvYS1. Here we revealed, by assessing the transport activity of a series of HvYS1-ZmYS1 chimeras, that the outer membrane loop between the sixth and seventh transmembrane regions is essential for substrate specificity. Circular dichroism spectra indicated that a synthetic peptide corresponding to the loop of HvYS1 forms an alpha-helix in solution, whereas that of ZmYS1 is flexible. We propose that the structural difference at this particular loop determines the substrate specificity of the HvYS1 transporter."},"publication_date":"2007-08-13","publication_name":{"en":"FEBS Letters","ja":"FEBS Letters"},"volume":"Vol.581","number":"No.22","starting_page":"4298","ending_page":"4302","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1016/j.febslet.2007.08.011"],"issn":["0014-5793"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:75, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/17411060","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263564","label":"url"}],"paper_title":{"en":"Synthesis and Absolute Structure of Manzacidin B","ja":"Synthesis and Absolute Structure of Manzacidin B"},"authors":{"en":[{"name":"Shinada Tetsuro"},{"name":"Ikebe Eijiro"},{"name":"Oe Kentaro"},{"name":"Namba Kosuke"},{"name":"Kawasaki Masanori"},{"name":"Ohfune Yasufumi"}],"ja":[{"name":"Shinada Tetsuro"},{"name":"Ikebe Eijiro"},{"name":"Oe Kentaro"},{"name":"難波 康祐"},{"name":"Kawasaki Masanori"},{"name":"Ohfune Yasufumi"}]},"description":{"en":"[reaction: see text] Four possible stereoisomers of manzacidin B were synthesized using stereochemically defined synthetic routes via the azide 7 and oxazoline 11 starting with the (R)-alpha-methyl Garner aldehyde 5. Comparisons of the spectroscopic data of the synthetic isomers 4a-d with those of the natural manzacidin B revised the proposed structure 3 to (4S,5S,6R)-4d.","ja":"[reaction: see text] Four possible stereoisomers of manzacidin B were synthesized using stereochemically defined synthetic routes via the azide 7 and oxazoline 11 starting with the (R)-alpha-methyl Garner aldehyde 5. Comparisons of the spectroscopic data of the synthetic isomers 4a-d with those of the natural manzacidin B revised the proposed structure 3 to (4S,5S,6R)-4d."},"publication_date":"2007-04-06","publication_name":{"en":"Organic Letters","ja":"Organic Letters"},"volume":"Vol.9","number":"No.9","starting_page":"1765","ending_page":"1767","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1021/ol0704789"],"issn":["1523-7060"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:76, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/17691091","label":"url"},{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-34848928102&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263588","label":"url"}],"paper_title":{"en":"A Practical Synthesis of a Phytosiderophore 2-Deoxymugineic Acid. A Key to the Mechanistic Study of Iron Acquisition by Graminaceous Plants","ja":"A Practical Synthesis of a Phytosiderophore 2-Deoxymugineic Acid. A Key to the Mechanistic Study of Iron Acquisition by Graminaceous Plants"},"authors":{"en":[{"name":"Namba Kosuke"},{"name":"Murata Yoshiko"},{"name":"Horikawa Manabu"},{"name":"Iwashita Takashi"},{"name":"Kusumoto Shoichi"}],"ja":[{"name":"難波 康祐"},{"name":"Murata Yoshiko"},{"name":"Horikawa Manabu"},{"name":"Iwashita Takashi"},{"name":"Kusumoto Shoichi"}]},"publication_date":"2007","publication_name":{"en":"Angewandte Chemie International Edition","ja":"Angewandte Chemie International Edition"},"volume":"Vol.46","number":"No.37","starting_page":"7060","ending_page":"7063","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1002/anie.200702403"],"issn":["1433-7851"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:77, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263565","label":"url"}],"paper_title":{"en":"Total synthesis and morphogenesis-inducing activity of (±)-thallusin and its analogues.","ja":"Total synthesis and morphogenesis-inducing activity of (±)-thallusin and its analogues."},"authors":{"en":[{"name":"Nishizawa Mugio"},{"name":"Iyenaga Tomoaki"},{"name":"Kurisaki Takahiro"},{"name":"Sharfuddin M."},{"name":"Namba Kosuke"},{"name":"Imagawa Hiroshi"},{"name":"Shizuri Y."},{"name":"Matsuo Y."}],"ja":[{"name":"Nishizawa Mugio"},{"name":"Iyenaga Tomoaki"},{"name":"Kurisaki Takahiro"},{"name":"Sharfuddin M."},{"name":"難波 康祐"},{"name":"Imagawa Hiroshi"},{"name":"Shizuri Y."},{"name":"Matsuo Y."}]},"publication_date":"2007","publication_name":{"en":"Tetrahedron Letters","ja":"Tetrahedron Letters"},"volume":"Vol.48","number":"No.24","starting_page":"4229","ending_page":"4233","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1016/j.tetlet.2007.04.075"],"issn":["0040-4039"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:78, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"http://ci.nii.ac.jp/naid/10017499016/","label":"url"},{"@id":"https://cir.nii.ac.jp/crid/1360846644035282304/","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263563","label":"url"}],"paper_title":{"en":"On the Stereoselectivity of Asymmetric Strecker Synthesis in a Cyclohexane System: Synthesis of Optically Active Cis- and Trans-1-amino-2-hydroxycyclohexane-1-carboxylic Acids.","ja":"On the Stereoselectivity of Asymmetric Strecker Synthesis in a Cyclohexane System: Synthesis of Optically Active Cis- and Trans-1-amino-2-hydroxycyclohexane-1-carboxylic Acids."},"authors":{"en":[{"name":"Shinada Tetsuro"},{"name":"Kawakami Tadashi"},{"name":"Sakai Hiroshi"},{"name":"Matsuda Hiromi"},{"name":"Umezawa Taiki"},{"name":"Kawasaki Masanori"},{"name":"Namba Kosuke"},{"name":"Ohfune Yasufumi"}],"ja":[{"name":"Shinada Tetsuro"},{"name":"Kawakami Tadashi"},{"name":"Sakai Hiroshi"},{"name":"Matsuda Hiromi"},{"name":"Umezawa Taiki"},{"name":"Kawasaki Masanori"},{"name":"難波 康祐"},{"name":"Ohfune Yasufumi"}]},"publication_date":"2006-05-15","publication_name":{"en":"Bulletin of the Chemical Society of Japan","ja":"Bulletin of the Chemical Society of Japan"},"volume":"Vol.79","number":"No.5","starting_page":"768","ending_page":"774","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1246/bcsj.79.768"],"issn":["0009-2673"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:79, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/16288521","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263562","label":"url"}],"paper_title":{"en":"Surprisingly Efficient Catalytic Cr-Mediated Coupling Reactions.","ja":"Surprisingly Efficient Catalytic Cr-Mediated Coupling Reactions."},"authors":{"en":[{"name":"Namba Kosuke"},{"name":"Wang J."},{"name":"Cui S."},{"name":"Kishi Yoshito"}],"ja":[{"name":"難波 康祐"},{"name":"Wang J."},{"name":"Cui S."},{"name":"Kishi Yoshito"}]},"description":{"en":"[reaction: see text] With use of 1 mol % of Cr catalyst 5, surprisingly efficient Cr-mediated couplings of aldehydes with various types of nucleophiles have been realized. The catalyst set of Cr catalyst 5 and Ni catalyst 4 is used for alkenylation, alkynylation, and arylation, whereas the catalyst set of Cr catalyst 5 and CoPc (cobalt phthalocyanine) is used for 2-haloallylation, alkylation, and propargylation. Only the Cr catalyst 5 is required for allylation. The reaction rates in DME and THF have been found significantly faster than that in MeCN.","ja":"[reaction: see text] With use of 1 mol % of Cr catalyst 5, surprisingly efficient Cr-mediated couplings of aldehydes with various types of nucleophiles have been realized. The catalyst set of Cr catalyst 5 and Ni catalyst 4 is used for alkenylation, alkynylation, and arylation, whereas the catalyst set of Cr catalyst 5 and CoPc (cobalt phthalocyanine) is used for 2-haloallylation, alkylation, and propargylation. Only the Cr catalyst 5 is required for allylation. The reaction rates in DME and THF have been found significantly faster than that in MeCN."},"publication_date":"2005-11-24","publication_name":{"en":"Organic Letters","ja":"Organic Letters"},"volume":"Vol.7","number":"No.24","starting_page":"5421","ending_page":"5425","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1021/ol052085k"],"issn":["1523-7060"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:80, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/16288520","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263561","label":"url"}],"paper_title":{"en":"A New Method for Translating the Asymmetric Ni/Cr-Mediated Coupling Reactions from Stoichiometric to Catalytic.","ja":"A New Method for Translating the Asymmetric Ni/Cr-Mediated Coupling Reactions from Stoichiometric to Catalytic."},"authors":{"en":[{"name":"Namba Kosuke"},{"name":"Cui S."},{"name":"Wang J."},{"name":"Kishi Yoshito"}],"ja":[{"name":"難波 康祐"},{"name":"Cui S."},{"name":"Wang J."},{"name":"Kishi Yoshito"}]},"description":{"en":"[reaction: see text] A new method has been developed for effectively translating the degree of asymmetric induction and the chemical yield achieved in the stoichiometric asymmetric Ni/Cr-mediated coupling to a catalytic asymmetric process via a chiral sulfonamide ligand. It has also been shown that the Ni catalyst plays a central role. Among a number of the Ni catalysts, the 2,9-dimethylphenanthroline/NiCl(2) complex (7) has been found to be the most effective.","ja":"[reaction: see text] A new method has been developed for effectively translating the degree of asymmetric induction and the chemical yield achieved in the stoichiometric asymmetric Ni/Cr-mediated coupling to a catalytic asymmetric process via a chiral sulfonamide ligand. It has also been shown that the Ni catalyst plays a central role. Among a number of the Ni catalysts, the 2,9-dimethylphenanthroline/NiCl(2) complex (7) has been found to be the most effective."},"publication_date":"2005-11-24","publication_name":{"en":"Organic Letters","ja":"Organic Letters"},"volume":"Vol.7","number":"No.24","starting_page":"5417","ending_page":"5419","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1021/ol052084s"],"issn":["1523-7060"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:81, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/16262397","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263560","label":"url"}],"paper_title":{"en":"Catalytic Ni/Cr-Mediated Macrocyclization without Use of High-Dilution Techniques.","ja":"Catalytic Ni/Cr-Mediated Macrocyclization without Use of High-Dilution Techniques."},"authors":{"en":[{"name":"Namba Kosuke"},{"name":"Kishi Yoshito"}],"ja":[{"name":"難波 康祐"},{"name":"Kishi Yoshito"}]},"description":{"en":"The feasibility of catalytic Ni/Cr-mediated macrocyclization was demonstrated for the two substrates chosen from the halichondrin area. With 5 mol % of Ni and Cr catalysts, the macrocyclization was realized without use of high-dilution techniques. The reported method has a number of appealing features, including user-friendliness, easy workup, apparent scalability, and cost-effectiveness. In addition, all the required reagents are commercially available or obtainable in one or two steps from commercially available chemicals.","ja":"The feasibility of catalytic Ni/Cr-mediated macrocyclization was demonstrated for the two substrates chosen from the halichondrin area. With 5 mol % of Ni and Cr catalysts, the macrocyclization was realized without use of high-dilution techniques. The reported method has a number of appealing features, including user-friendliness, easy workup, apparent scalability, and cost-effectiveness. In addition, all the required reagents are commercially available or obtainable in one or two steps from commercially available chemicals."},"publication_date":"2005-11-09","publication_name":{"en":"Journal of the American Chemical Society","ja":"Journal of the American Chemical Society"},"volume":"Vol.127","starting_page":"15382","ending_page":"15383","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1021/ja055966v"],"issn":["0002-7863"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:82, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/15606128","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263559","label":"url"}],"paper_title":{"en":"New Catalytic Cycle for Couplings of Aldehydes with Organochromium Reagents.","ja":"New Catalytic Cycle for Couplings of Aldehydes with Organochromium Reagents."},"authors":{"en":[{"name":"Namba Kosuke"},{"name":"Kishi Yoshito"}],"ja":[{"name":"難波 康祐"},{"name":"Kishi Yoshito"}]},"description":{"en":"[reaction: see text] A new catalytic cycle has been developed to effect all three subgroups of Cr-mediated couplings, i.e., (1) Ni/Cr-mediated alkenylation, alkynylation, and arylation, (2) Co/Cr-mediated 2-haloallylation, alkylation, and propargylation, and (3) Cr-mediated allylation. In the presence of chiral sulfonamide ligands, good asymmetric inductions can be achieved for some of the Ni/Cr-mediated alkenylation, Co/Cr-mediated 2-haloallylation and propargylation, and Cr-mediated allylation.","ja":"[reaction: see text] A new catalytic cycle has been developed to effect all three subgroups of Cr-mediated couplings, i.e., (1) Ni/Cr-mediated alkenylation, alkynylation, and arylation, (2) Co/Cr-mediated 2-haloallylation, alkylation, and propargylation, and (3) Cr-mediated allylation. In the presence of chiral sulfonamide ligands, good asymmetric inductions can be achieved for some of the Ni/Cr-mediated alkenylation, Co/Cr-mediated 2-haloallylation and propargylation, and Cr-mediated allylation."},"publication_date":"2004-12-23","publication_name":{"en":"Organic Letters","ja":"Organic Letters"},"volume":"Vol.6","number":"No.26","starting_page":"5031","ending_page":"5033","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1021/ol047661b"],"issn":["1523-7060"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:83, {"insert":{"user_id":"5000093573","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/15212512","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=263558","label":"url"}],"paper_title":{"en":"A Simple but Remarkably Effective Device for Forming the C8-C14 Polycyclic Ring System of Halichondrin B.","ja":"A Simple but Remarkably Effective Device for Forming the C8-C14 Polycyclic Ring System of Halichondrin B."},"authors":{"en":[{"name":"Namba Kosuke"},{"name":"Jun H.-S."},{"name":"Kishi Yoshito"}],"ja":[{"name":"難波 康祐"},{"name":"Jun H.-S."},{"name":"Kishi Yoshito"}]},"description":{"en":"A simple device consisting of two ion-exchange columns, two alumina-based filters, and a pump (Figure 1) was assembled to form the C8-C14 polycyclic ring system present in the halichondrin B class of marine natural products. The effectiveness of this device was tested for three substrates. In each case, the desired polycyclic ketal 3, 5, or 7 was obtained almost quantitatively in a single operation.","ja":"A simple device consisting of two ion-exchange columns, two alumina-based filters, and a pump (Figure 1) was assembled to form the C8-C14 polycyclic ring system present in the halichondrin B class of marine natural products. The effectiveness of this device was tested for three substrates. In each case, the desired polycyclic ketal 3, 5, or 7 was obtained almost quantitatively in a single operation."},"publication_date":"2004-06-30","publication_name":{"en":"Journal of the American Chemical Society","ja":"Journal of the American Chemical Society"},"volume":"Vol.126","number":"No.25","starting_page":"7770","ending_page":"7771","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1021/ja047826b"],"issn":["0002-7863"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
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