=== Generating (published_papers) ===
=== Generating (teaching_experience) ===
=== Generating (education) ===
=== Generating (research_experience) ===
=== Generating (misc) ===
=== Generating (research_projects) ===
=== Generating (books_etc) ===
=== Generating (industrial_property_rights) ===
=== Generating (awards) ===
=== Generating (association_memberships) ===
=== Generating (presentations) ===
==== begin registerFile(/WWW/pub2/data/ERD/person/309265/researchmap/published_papers.jsonl) ====
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line:3, {"insert":{"user_id":"7000009000","type":"published_papers","id":"45669457"},"force":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/38502523","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=405226","label":"url"}],"paper_title":{"en":"Variable Photoluminescence Intensity Ratio with the Excitation Wavelength in Eu3+-Doped Perovskite-Type Alkaline Earth ZirconatesPossibility of a Unique Visualization of Ultraviolet Light","ja":"Variable Photoluminescence Intensity Ratio with the Excitation Wavelength in Eu3+-Doped Perovskite-Type Alkaline Earth ZirconatesPossibility of a Unique Visualization of Ultraviolet Light"},"authors":{"en":[{"name":"Fujishiro Fumito"},{"name":"Yamamoto Suzuka"},{"name":"Yahata Tomoki"},{"name":"Oishi Masatsugu"}],"ja":[{"name":"Fujishiro Fumito"},{"name":"Yamamoto Suzuka"},{"name":"矢羽田 友樹"},{"name":"大石 昌嗣"}]},"description":{"en":"Photoluminescence (PL) spectra arising from 4f-4f dipole transitions of Eu doped at both the and sites of perovskite-type alkaline earth zirconates obtained at various excitation wavelengths were evaluated. Changes in the excitation wavelength caused obvious differences in the PL intensity ratio of the induced electric dipole (ED) D → F transition to the magnetic dipole (MD) D → F transition for Eu-doped SrZrO and CaZrO, in which only the B site had a center of symmetry. Two charge transfer (CT) bands associated with the excitation of Eu were observed in the spectra of these oxide samples, which arose from the difference in the electronic structure of the Eu-O coordination at the A and B sites. We conclude that simultaneous Eu substitution at sites with and without a center of symmetry, which have different charge transfer energies, induced the observed novel PL changes with a changing excitation wavelength. Our results may enable the development of a new type of ultraviolet light detector.","ja":"Photoluminescence (PL) spectra arising from 4f-4f dipole transitions of Eu doped at both the and sites of perovskite-type alkaline earth zirconates obtained at various excitation wavelengths were evaluated. Changes in the excitation wavelength caused obvious differences in the PL intensity ratio of the induced electric dipole (ED) D → F transition to the magnetic dipole (MD) D → F transition for Eu-doped SrZrO and CaZrO, in which only the B site had a center of symmetry. Two charge transfer (CT) bands associated with the excitation of Eu were observed in the spectra of these oxide samples, which arose from the difference in the electronic structure of the Eu-O coordination at the A and B sites. We conclude that simultaneous Eu substitution at sites with and without a center of symmetry, which have different charge transfer energies, induced the observed novel PL changes with a changing excitation wavelength. Our results may enable the development of a new type of ultraviolet light detector."},"publication_date":"2024-02-27","publication_name":{"en":"Inorganic Chemistry","ja":"Inorganic Chemistry"},"volume":"Vol.63","number":"No.13","starting_page":"5865","ending_page":"5871","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1021/acs.inorgchem.3c04327"],"issn":["1520-510X"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
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line:10, {"insert":{"user_id":"7000009000","type":"published_papers","id":"39828905"},"force":{"see_also":[{"@id":"https://repo.lib.tokushima-u.ac.jp/ja/117904","label":"url"},{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/36052573","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=391701","label":"url"}],"paper_title":{"en":"Adaptive Cation Pillar Effects Achieving High Capacity in Li-Rich Layered Oxide, Li2MnO3-LiMeO2 (Me = Ni, Co, Mn)","ja":"Adaptive Cation Pillar Effects Achieving High Capacity in Li-Rich Layered Oxide, Li2MnO3-LiMeO2 (Me = Ni, Co, Mn)"},"authors":{"en":[{"name":"Hiroi Satoshi"},{"name":"Oishi Masatsugu"},{"name":"Ohara Koji"},{"name":"Shimoda Keiji"},{"name":"Kabutan Daiki"},{"name":"Uchimoto Yoshiharu"}],"ja":[{"name":"Hiroi Satoshi"},{"name":"大石 昌嗣"},{"name":"Ohara Koji"},{"name":"Shimoda Keiji"},{"name":"株丹 大輝"},{"name":"Uchimoto Yoshiharu"}]},"description":{"en":"Intensive research is underway to further enhance the performance of lithium-ion batteries (LIBs). To increase the capacity of positive electrode materials, Li-rich layered oxides (LLO) are attracting attention but have not yet been put to practical use. The structural mechanisms through which LLO materials exhibit higher capacity than conventional materials remain unclear because their disordered phases make it difficult to obtain structural information by conventional analysis. The X-ray total scattering analysis reveals a disordered structure consisting of metal ions in octahedral and tetrahedral sites of Li layers as a result of cation mixing after the extraction of Li ions. Metal ions in octahedral sites act as rigid pillars. The metal ions move to the tetrahedral site of the Li layer, which functions as a Li-layer pillar during Li extraction, and returns to the metal site during Li insertion, facilitating Li diffusion as an adaptive pillar. Adaptive pillars are the specific structural features that differ from those of the conventional layered materials, and their effects are responsible for the high capacity of LLO materials. An essential understanding of the pillar effects will contribute to design guidelines for intercalation-type positive electrodes for next-generation LIBs.","ja":"Intensive research is underway to further enhance the performance of lithium-ion batteries (LIBs). To increase the capacity of positive electrode materials, Li-rich layered oxides (LLO) are attracting attention but have not yet been put to practical use. The structural mechanisms through which LLO materials exhibit higher capacity than conventional materials remain unclear because their disordered phases make it difficult to obtain structural information by conventional analysis. The X-ray total scattering analysis reveals a disordered structure consisting of metal ions in octahedral and tetrahedral sites of Li layers as a result of cation mixing after the extraction of Li ions. Metal ions in octahedral sites act as rigid pillars. The metal ions move to the tetrahedral site of the Li layer, which functions as a Li-layer pillar during Li extraction, and returns to the metal site during Li insertion, facilitating Li diffusion as an adaptive pillar. Adaptive pillars are the specific structural features that differ from those of the conventional layered materials, and their effects are responsible for the high capacity of LLO materials. An essential understanding of the pillar effects will contribute to design guidelines for intercalation-type positive electrodes for next-generation LIBs."},"publication_date":"2022-09-02","publication_name":{"en":"Small","ja":"Small"},"number":"No.2203412","starting_page":"1","ending_page":"11","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1002/smll.202203412"],"issn":["1613-6829"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
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We site-selectively investigated the valence states and local structures of Ni in Li0.89Ni1.11O2, where Ni atoms occupy mainly the NiO2 host-layer sites and partially the interlayer Li sites in-between the host layers, during electrochemical Li insertion/extraction in a lithium-ion battery (LIB). The site-selective X-ray near edge structure evaluated via the P-DAFS method revealed that the interlayer Ni atoms exhibited much lower electrochemical activity as compared to those at the host-layer site. Furthermore, the present analyses of site-selective extended X-ray absorption fine structure performed using the P-DAFS method indicates local structural changes around the residual Ni atoms at the interlayer space during the initial charge; it tends to gather to form rock-salt NiO-like domains around the interlayer Ni. The presence of the NiO-like domains in the interlayer space locally diminishes the interlayer distance and would yield strain energy because of the lattice mismatch, which retards the subsequent Li insertion both thermodynamically and kinetically. Such restrictions on the Li insertion inevitably make the NiO-like domains electrochemically inactive, resulting in an appreciable irreversible capacity after the initial charge but an achievement of robust linkage of neighboring NiO2 layers that tend to be dissociated without the Li occupation. The P-DAFS characterization of antisite transition metals interchanging with Li atoms complements the understanding of the detailed charge-compensation and degradation mechanisms in the electrode materials.","ja":"Roles of antisite transition metals interchanging with Li atoms in electrode materials of Li transition-metal complex oxides were clarified using a newly developed direct labeling method, termed powder diffraction anomalous fine structure (P-DAFS) near the Ni K-edge. We site-selectively investigated the valence states and local structures of Ni in Li0.89Ni1.11O2, where Ni atoms occupy mainly the NiO2 host-layer sites and partially the interlayer Li sites in-between the host layers, during electrochemical Li insertion/extraction in a lithium-ion battery (LIB). The site-selective X-ray near edge structure evaluated via the P-DAFS method revealed that the interlayer Ni atoms exhibited much lower electrochemical activity as compared to those at the host-layer site. Furthermore, the present analyses of site-selective extended X-ray absorption fine structure performed using the P-DAFS method indicates local structural changes around the residual Ni atoms at the interlayer space during the initial charge; it tends to gather to form rock-salt NiO-like domains around the interlayer Ni. The presence of the NiO-like domains in the interlayer space locally diminishes the interlayer distance and would yield strain energy because of the lattice mismatch, which retards the subsequent Li insertion both thermodynamically and kinetically. Such restrictions on the Li insertion inevitably make the NiO-like domains electrochemically inactive, resulting in an appreciable irreversible capacity after the initial charge but an achievement of robust linkage of neighboring NiO2 layers that tend to be dissociated without the Li occupation. The P-DAFS characterization of antisite transition metals interchanging with Li atoms complements the understanding of the detailed charge-compensation and degradation mechanisms in the electrode materials."},"publication_date":"2015-06","publication_name":{"en":"Physical Chemistry Chemical Physics","ja":"Physical Chemistry Chemical Physics"},"volume":"Vol.17","number":"No.21","starting_page":"14064","ending_page":"14070","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1039/c5cp00940e"],"issn":["1463-9084"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:32, {"insert":{"user_id":"7000009000","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-84916912213&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=312555","label":"url"}],"paper_title":{"en":"Structural modification by adding Li cations into Mg/Cs-TFSA molten salt facilitating Mg electrodeposition","ja":"Structural modification by adding Li cations into Mg/Cs-TFSA molten salt facilitating Mg electrodeposition"},"authors":{"en":[{"name":"Ohara Koji"},{"name":"Umebayashi Yasuhiro"},{"name":"Ichitsubo Tetsu"},{"name":"Matsumoto Kazuhiko"},{"name":"Hagiwara Rika"},{"name":"Arai Hajime"},{"name":"Mori Masahiro"},{"name":"Orikasa Yuki"},{"name":"Okamoto Shinya"},{"name":"Oishi Masatsugu"},{"name":"Aiso Yuka"},{"name":"Nohira Toshiyuki"},{"name":"Uchimoto Yoshiharu"},{"name":"Ogumi Zempachi"},{"name":"Matsubara Eiichiro"}],"ja":[{"name":"Ohara Koji"},{"name":"Umebayashi Yasuhiro"},{"name":"Ichitsubo Tetsu"},{"name":"Matsumoto Kazuhiko"},{"name":"Hagiwara Rika"},{"name":"Arai Hajime"},{"name":"Mori Masahiro"},{"name":"Orikasa Yuki"},{"name":"Okamoto Shinya"},{"name":"大石 昌嗣"},{"name":"Aiso Yuka"},{"name":"Nohira Toshiyuki"},{"name":"Uchimoto Yoshiharu"},{"name":"Ogumi Zempachi"},{"name":"Matsubara Eiichiro"}]},"publication_date":"2015","publication_name":{"en":"RSC Advances","ja":"RSC Advances"},"volume":"Vol.5","starting_page":"3063","ending_page":"3069","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1039/c4ra13244k"],"issn":["2046-2069"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:33, {"insert":{"user_id":"7000009000","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-84912569269&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=312554","label":"url"}],"paper_title":{"en":"Direct observation of reversible charge compensation by oxygen ion in Li-rich manganese layered oxide positive electrode material, Li1.16Ni0.15Co0.19Mn0.50O2","ja":"Direct observation of reversible charge compensation by oxygen ion in Li-rich manganese layered oxide positive electrode material, Li1.16Ni0.15Co0.19Mn0.50O2"},"authors":{"en":[{"name":"Oishi Masatsugu"},{"name":"Yogi Chihiro"},{"name":"Watanabe Iwao"},{"name":"Ohta Toshiaki"},{"name":"Orikasa Yuki"},{"name":"Uchimoto Yoshiharu"},{"name":"Ogumi Zempachi"}],"ja":[{"name":"大石 昌嗣"},{"name":"Yogi Chihiro"},{"name":"Watanabe Iwao"},{"name":"Ohta Toshiaki"},{"name":"Orikasa Yuki"},{"name":"Uchimoto Yoshiharu"},{"name":"Ogumi Zempachi"}]},"publication_date":"2015","publication_name":{"en":"Journal of Power Sources","ja":"Journal of Power Sources"},"volume":"Vol.276","starting_page":"89","ending_page":"94","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1016/j.jpowsour.2014.11.104"],"issn":["0378-7753"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:34, {"insert":{"user_id":"7000009000","type":"published_papers","id":"31347501"},"force":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/25343791","label":"url"},{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-84930194058&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=312556","label":"url"}],"paper_title":{"en":"Revisit to Diffraction Anomalous Fine Structure (DAFS)","ja":"Revisit to Diffraction Anomalous Fine Structure (DAFS)"},"authors":{"en":[{"name":"Kawaguchi Tomoya"},{"name":"Fukuda Katsutoshi"},{"name":"Tokuda Kazuya"},{"name":"Shimada Koki"},{"name":"Ichitsubo Tetsu"},{"name":"Oishi Masatsugu"},{"name":"Mizuki Jun'ichiro"},{"name":"Matsubara Eiichiro"}],"ja":[{"name":"Kawaguchi Tomoya"},{"name":"Fukuda Katsutoshi"},{"name":"Tokuda Kazuya"},{"name":"Shimada Koki"},{"name":"Ichitsubo Tetsu"},{"name":"大石 昌嗣"},{"name":"Mizuki Jun'ichiro"},{"name":"Matsubara Eiichiro"}]},"description":{"en":"The diffraction anomalous fine structure (DAFS) method that is a spectroscopic analysis combined with resonant X-ray diffraction enables the determination of the valence state and local structure of a selected element at a specific crystalline site and/or phase. This method has been improved by using a polycrystalline sample, channel-cut monochromator optics with an undulator synchrotron radiation source, an area detector and direct determination of resonant terms with a logarithmic dispersion relation. This study makes the DAFS method more convenient and saves a large amount of measurement time in comparison with the conventional DAFS method with a single crystal. The improved DAFS method has been applied to some model samples, Ni foil and Fe3O4 powder, to demonstrate the validity of the measurement and the analysis of the present DAFS method.","ja":"The diffraction anomalous fine structure (DAFS) method that is a spectroscopic analysis combined with resonant X-ray diffraction enables the determination of the valence state and local structure of a selected element at a specific crystalline site and/or phase. This method has been improved by using a polycrystalline sample, channel-cut monochromator optics with an undulator synchrotron radiation source, an area detector and direct determination of resonant terms with a logarithmic dispersion relation. This study makes the DAFS method more convenient and saves a large amount of measurement time in comparison with the conventional DAFS method with a single crystal. The improved DAFS method has been applied to some model samples, Ni foil and Fe3O4 powder, to demonstrate the validity of the measurement and the analysis of the present DAFS method."},"publication_date":"2014-11","publication_name":{"en":"Journal of Synchrotron Radiation","ja":"Journal of Synchrotron Radiation"},"volume":"Vol.21","starting_page":"1247","ending_page":"1251","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1107/S1600577514015148"],"issn":["1600-5775"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:35, {"insert":{"user_id":"7000009000","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/24611637","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=312559","label":"url"}],"paper_title":{"en":"Three-dimensional nano electrode by metal nanowire nonwoven clothes","ja":"Three-dimensional nano electrode by metal nanowire nonwoven clothes"},"authors":{"en":[{"name":"Kawamori Makoto"},{"name":"Asai Takahiro"},{"name":"Shirai Yoshimasa"},{"name":"Yagi Shunsuke"},{"name":"Oishi Masatsugu"},{"name":"Ichitsubo Tetsu"},{"name":"Matsubara Eiichiro"}],"ja":[{"name":"Kawamori Makoto"},{"name":"Asai Takahiro"},{"name":"Shirai Yoshimasa"},{"name":"Yagi Shunsuke"},{"name":"大石 昌嗣"},{"name":"Ichitsubo Tetsu"},{"name":"Matsubara Eiichiro"}]},"description":{"en":"Metal nanowire nonwoven cloth (MNNC) is a metal sheet that has resulted from intertwined metal nanowires 100 nm in diameter with several dozen micrometers of length. Thus, it is a new metallic material having both a flexibility of the metal sheet and a large specific surface area of the nanowires. As an application that utilizes these properties, we propose a high-cyclability electrode for Li storage batteries, in which an active material is deposited or coated on MNNC. The proposed electrode can work without any binders, conductive additives, and current collectors, which might largely improve a practical gravimetric energy density. Huge electrode surfaces provide efficient ion/electron transports, and sufficient interspaces between the respective nanowires accommodate large volume expansions of the active material. To demonstrate these advantages, we have fabricated a NiO-covered nickel nanowire nonwoven cloth (NNNC) by electroless deposition under a magnetic field and annealing in air. The adequately annealed NNNC was shown to be an excellent conversion-type electrode that exhibits a quite high cyclability, 500 mAh/g at 1 C after 300 cycles, compared to that of a composite electrode consisting of NiO nanoparticles. Thus, the present design concept will contribute to a game-changing technology in future lithium ion battery (LIB) electrodes.","ja":"Metal nanowire nonwoven cloth (MNNC) is a metal sheet that has resulted from intertwined metal nanowires 100 nm in diameter with several dozen micrometers of length. Thus, it is a new metallic material having both a flexibility of the metal sheet and a large specific surface area of the nanowires. As an application that utilizes these properties, we propose a high-cyclability electrode for Li storage batteries, in which an active material is deposited or coated on MNNC. The proposed electrode can work without any binders, conductive additives, and current collectors, which might largely improve a practical gravimetric energy density. Huge electrode surfaces provide efficient ion/electron transports, and sufficient interspaces between the respective nanowires accommodate large volume expansions of the active material. To demonstrate these advantages, we have fabricated a NiO-covered nickel nanowire nonwoven cloth (NNNC) by electroless deposition under a magnetic field and annealing in air. The adequately annealed NNNC was shown to be an excellent conversion-type electrode that exhibits a quite high cyclability, 500 mAh/g at 1 C after 300 cycles, compared to that of a composite electrode consisting of NiO nanoparticles. Thus, the present design concept will contribute to a game-changing technology in future lithium ion battery (LIB) electrodes."},"publication_date":"2014-03-11","publication_name":{"en":"Nano Letters","ja":"Nano Letters"},"volume":"Vol.14","number":"No.4","starting_page":"1932","ending_page":"1937","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1021/nl404753e"],"issn":["1530-6992"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:36, {"insert":{"user_id":"7000009000","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-84904816334&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=312558","label":"url"}],"paper_title":{"en":"Electrochemical behavior of magnesium alloys in alkali metal-TFSA ionic liquid for magnesium-battery negative electrode","ja":"Electrochemical behavior of magnesium alloys in alkali metal-TFSA ionic liquid for magnesium-battery negative electrode"},"authors":{"en":[{"name":"Oishi Masatsugu"},{"name":"Ichitsubo Tetsu"},{"name":"Okamoto Shinya"},{"name":"Matsubara Eiichiro"},{"name":"Nohira Toshiyuki"},{"name":"Hagiwara Rika"}],"ja":[{"name":"大石 昌嗣"},{"name":"Ichitsubo Tetsu"},{"name":"Okamoto Shinya"},{"name":"Matsubara Eiichiro"},{"name":"Nohira Toshiyuki"},{"name":"Hagiwara Rika"}]},"publication_date":"2014","publication_name":{"en":"Journal of the Electrochemical Society","ja":"Journal of the Electrochemical Society"},"volume":"Vol.161","starting_page":"A943","ending_page":"A947","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1149/2.043406jes"],"issn":["0013-4651"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:37, {"insert":{"user_id":"7000009000","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-84906244728&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=312557","label":"url"}],"paper_title":{"en":"A new aspect of chevrel compounds as positive electrodes for magnesium batteries","ja":"A new aspect of chevrel compounds as positive electrodes for magnesium batteries"},"authors":{"en":[{"name":"Ichitsubo Tetsu"},{"name":"Yagi Shunsuke"},{"name":"Nakamura Ryosuke"},{"name":"Ichikawa Y."},{"name":"Okamoto Shinya"},{"name":"Sugimura K."},{"name":"Kawaguchi Tomoya"},{"name":"Kitada Atsushi"},{"name":"Oishi Masatsugu"},{"name":"Doi Takayuki"},{"name":"Matsubara Eiichiro"}],"ja":[{"name":"Ichitsubo Tetsu"},{"name":"Yagi Shunsuke"},{"name":"Nakamura Ryosuke"},{"name":"Ichikawa Y."},{"name":"Okamoto Shinya"},{"name":"Sugimura K."},{"name":"Kawaguchi Tomoya"},{"name":"Kitada Atsushi"},{"name":"大石 昌嗣"},{"name":"Doi Takayuki"},{"name":"Matsubara Eiichiro"}]},"publication_date":"2014","publication_name":{"en":"Journal of Materials Chemistry. A, Materials for Energy and Sustainability","ja":"Journal of Materials Chemistry. A, Materials for Energy and Sustainability"},"volume":"Vol.2","starting_page":"14858","ending_page":"14866","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1039/c4ta03063j"],"issn":["2050-7488"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:38, {"insert":{"user_id":"7000009000","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-84877317728&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=312577","label":"url"}],"paper_title":{"en":"In situ two-dimensional micro-imaging XAFS with CCD detector","ja":"In situ two-dimensional micro-imaging XAFS with CCD detector"},"authors":{"en":[{"name":"Tanida Hajime"},{"name":"Yamashige Hisao"},{"name":"Orikasa Yuki"},{"name":"Fujimoto Takahiro"},{"name":"Oishi Masatsugu"},{"name":"Murayama Haruno"},{"name":"Arai Hajime"},{"name":"Katayama Misaki"},{"name":"Inada Yasuhiro"},{"name":"Ohta Toshiaki"},{"name":"Uchimoto Yoshiharu"},{"name":"Ogumi Zempachi"}],"ja":[{"name":"Tanida Hajime"},{"name":"Yamashige Hisao"},{"name":"Orikasa Yuki"},{"name":"Fujimoto Takahiro"},{"name":"大石 昌嗣"},{"name":"Murayama Haruno"},{"name":"Arai Hajime"},{"name":"Katayama Misaki"},{"name":"Inada Yasuhiro"},{"name":"Ohta Toshiaki"},{"name":"Uchimoto Yoshiharu"},{"name":"Ogumi Zempachi"}]},"publication_date":"2013","publication_name":{"en":"Journal of Physics: Conference Series","ja":"Journal of Physics: Conference Series"},"volume":"Vol.430","starting_page":"012021","ending_page":"012021","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1088/1742-6596/430/1/012021"],"issn":["1742-6596"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:39, {"insert":{"user_id":"7000009000","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-84866056714&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=312561","label":"url"}],"paper_title":{"en":"Charge compensation mechanisms in Li1.16Ni0.15Co0.19Mn0.50O2 positive electrode material for Li-ion batteries analyzed by a combination of hard and soft X-ray absorption near edge structure","ja":"Charge compensation mechanisms in Li1.16Ni0.15Co0.19Mn0.50O2 positive electrode material for Li-ion batteries analyzed by a combination of hard and soft X-ray absorption near edge structure"},"authors":{"en":[{"name":"Oishi Masatsugu"},{"name":"Fujimoto Takahiro"},{"name":"Takanashi Yu"},{"name":"Orikasa Yuki"},{"name":"Kawamura Atsushi"},{"name":"Ina Toshiaki"},{"name":"Yamashige Hisao"},{"name":"Takamatsu Daiko"},{"name":"Sato Kenji"},{"name":"Murayama Haruno"},{"name":"Tanida Hajime"},{"name":"Arai Hajime"},{"name":"Ishii Hideshi"},{"name":"Yogi Chihiro"},{"name":"Watanabe Iwao"},{"name":"Ohta Toshiaki"},{"name":"Mineshige Atsushi"},{"name":"Uchimoto Yoshiharu"},{"name":"Ogumi Zempachi"}],"ja":[{"name":"大石 昌嗣"},{"name":"Fujimoto Takahiro"},{"name":"Takanashi Yu"},{"name":"Orikasa Yuki"},{"name":"Kawamura Atsushi"},{"name":"Ina Toshiaki"},{"name":"Yamashige Hisao"},{"name":"Takamatsu Daiko"},{"name":"Sato Kenji"},{"name":"Murayama Haruno"},{"name":"Tanida Hajime"},{"name":"Arai Hajime"},{"name":"Ishii Hideshi"},{"name":"Yogi Chihiro"},{"name":"Watanabe Iwao"},{"name":"Ohta Toshiaki"},{"name":"Mineshige Atsushi"},{"name":"Uchimoto Yoshiharu"},{"name":"Ogumi Zempachi"}]},"publication_date":"2013","publication_name":{"en":"Journal of Power Sources","ja":"Journal of Power Sources"},"volume":"Vol.222","number":"No.15","starting_page":"45","ending_page":"51","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1016/j.jpowsour.2012.08.023"],"issn":["0378-7753"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:40, {"insert":{"user_id":"7000009000","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-84876562870&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=312560","label":"url"}],"paper_title":{"en":"Elastically constrained phase-separation dynamics competing with charge process in LiFePO4/FePO4 system","ja":"Elastically constrained phase-separation dynamics competing with charge process in LiFePO4/FePO4 system"},"authors":{"en":[{"name":"Ichitsubo Tetsu"},{"name":"Tokuda Kazuya"},{"name":"Yagi Shunsuke"},{"name":"Kawamori Makoto"},{"name":"Kawaguchi Tomoya"},{"name":"Doi Takayuki"},{"name":"Oishi Masatsugu"},{"name":"Matsubara Eiichiro"}],"ja":[{"name":"Ichitsubo Tetsu"},{"name":"Tokuda Kazuya"},{"name":"Yagi Shunsuke"},{"name":"Kawamori Makoto"},{"name":"Kawaguchi Tomoya"},{"name":"Doi Takayuki"},{"name":"大石 昌嗣"},{"name":"Matsubara Eiichiro"}]},"publication_date":"2013","publication_name":{"en":"Journal of Materials Chemistry. A, Materials for Energy and Sustainability","ja":"Journal of Materials Chemistry. A, Materials for Energy and Sustainability"},"volume":"Vol.1","number":"No.7","starting_page":"2567","ending_page":"2577","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1039/c2ta01102f"],"issn":["2050-7488"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:41, {"insert":{"user_id":"7000009000","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.ncbi.nlm.nih.gov/pubmed/21850304","label":"url"},{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-80052537863&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=312564","label":"url"}],"paper_title":{"en":"An X-ray Absorption Spectroscopic Study on Mixed Conductive La0.6Sr0.4Co0.8Fe0.2O3- Cathodes I. Electrical Conductivity and Electronic Structure","ja":"An X-ray Absorption Spectroscopic Study on Mixed Conductive La0.6Sr0.4Co0.8Fe0.2O3- Cathodes I. Electrical Conductivity and Electronic Structure"},"authors":{"en":[{"name":"Orikasa Yuki"},{"name":"Ina Toshiaki"},{"name":"Nakao Takayuki"},{"name":"Mineshige Atsushi"},{"name":"Amezawa Koji"},{"name":"Oishi Masatsugu"},{"name":"Arai Hajime"},{"name":"Ogumi Zempachi"},{"name":"Uchimoto Yoshiharu"}],"ja":[{"name":"Orikasa Yuki"},{"name":"Ina Toshiaki"},{"name":"Nakao Takayuki"},{"name":"Mineshige Atsushi"},{"name":"Amezawa Koji"},{"name":"大石 昌嗣"},{"name":"Arai Hajime"},{"name":"Ogumi Zempachi"},{"name":"Uchimoto Yoshiharu"}]},"description":{"en":"The electrical conduction mechanism of mixed conductive perovskite oxides, La(0.6)Sr(0.4)Co(0.8)Fe(0.2)O(3-δ), for cathode materials of solid oxide fuel cells has been investigated from electronic structural changes during oxygen vacancy formation. La(0.6)Sr(0.4)Co(0.8)Fe(0.2)O(3-δ) was annealed under various oxygen partial pressures p(O(2))s at 1073 K and quenched. Iodometric titration indicated that the oxygen nonstoichiometry of La(0.6)Sr(0.4)Co(0.8)Fe(0.2)O(3-δ) depended on the annealing p(O(2)), with more oxygen vacancies introduced at lower than at higher p(O(2))s. X-Ray absorption spectroscopic measurements were performed at the O K-, Co L-, Fe L-, Co K-, and Fe K-edges. The valence states of the Co and Fe ions were investigated by the X-ray absorption near edge structure (XANES) at the Co and Fe L(III)-edges. While the Fe average valence was almost constant, the valence of the Co ions decreased with oxygen vacancy introduction. The O K-edge XANES spectra indicated that electrons were injected into the Co 3d/O 2p hybridization state with oxygen vacancy introduction. Both absorption edges at the Co and Fe K-edge XANES shifted towards lower energies with oxygen vacancy introduction. The shift at the Co K-edge resulted from the decrease in the Co average valence and that at the Fe K-edge appeared to be caused by changes in the coordination environment around the Fe ions. The total conductivity of La(0.6)Sr(0.4)Co(0.8)Fe(0.2)O(3-δ) decreased with decreasing p(O(2)), due to a decreasing hole concentration.","ja":"The electrical conduction mechanism of mixed conductive perovskite oxides, La(0.6)Sr(0.4)Co(0.8)Fe(0.2)O(3-δ), for cathode materials of solid oxide fuel cells has been investigated from electronic structural changes during oxygen vacancy formation. La(0.6)Sr(0.4)Co(0.8)Fe(0.2)O(3-δ) was annealed under various oxygen partial pressures p(O(2))s at 1073 K and quenched. Iodometric titration indicated that the oxygen nonstoichiometry of La(0.6)Sr(0.4)Co(0.8)Fe(0.2)O(3-δ) depended on the annealing p(O(2)), with more oxygen vacancies introduced at lower than at higher p(O(2))s. X-Ray absorption spectroscopic measurements were performed at the O K-, Co L-, Fe L-, Co K-, and Fe K-edges. The valence states of the Co and Fe ions were investigated by the X-ray absorption near edge structure (XANES) at the Co and Fe L(III)-edges. While the Fe average valence was almost constant, the valence of the Co ions decreased with oxygen vacancy introduction. The O K-edge XANES spectra indicated that electrons were injected into the Co 3d/O 2p hybridization state with oxygen vacancy introduction. Both absorption edges at the Co and Fe K-edge XANES shifted towards lower energies with oxygen vacancy introduction. The shift at the Co K-edge resulted from the decrease in the Co average valence and that at the Fe K-edge appeared to be caused by changes in the coordination environment around the Fe ions. The total conductivity of La(0.6)Sr(0.4)Co(0.8)Fe(0.2)O(3-δ) decreased with decreasing p(O(2)), due to a decreasing hole concentration."},"publication_date":"2011-10","publication_name":{"en":"Physical Chemistry Chemical Physics","ja":"Physical Chemistry Chemical Physics"},"volume":"Vol.13","number":"No.37","starting_page":"16637","ending_page":"16643","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1039/C1CP20982E"],"issn":["1463-9084"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
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line:44, {"insert":{"user_id":"7000009000","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=312567","label":"url"}],"paper_title":{"en":"Nanoscale Observation of the Electronic and Local Structures of LiCoO2 Thin Film Electrode by Depth-Resolved X-ray Absorption Spectroscopy","ja":"Nanoscale Observation of the Electronic and Local Structures of LiCoO2 Thin Film Electrode by Depth-Resolved X-ray Absorption Spectroscopy"},"authors":{"en":[{"name":"Takamatsu Daiko"},{"name":"Nakatsutsumi Takayuki"},{"name":"Mori Shinichiro"},{"name":"Orikasa Yuki"},{"name":"Mogi Masato"},{"name":"Yamashige Hisao"},{"name":"Sato Kenji"},{"name":"Fujimoto Takahiro"},{"name":"Takanashi Yu"},{"name":"Murayama Haruno"},{"name":"Oishi Masatsugu"},{"name":"Tanida Hajime"},{"name":"Uruga Tomoya"},{"name":"Arai Hajime"},{"name":"Uchimoto Yoshiharu"},{"name":"Ogumi Zempachi"}],"ja":[{"name":"Takamatsu Daiko"},{"name":"Nakatsutsumi Takayuki"},{"name":"Mori Shinichiro"},{"name":"Orikasa Yuki"},{"name":"Mogi Masato"},{"name":"Yamashige Hisao"},{"name":"Sato Kenji"},{"name":"Fujimoto Takahiro"},{"name":"Takanashi Yu"},{"name":"Murayama Haruno"},{"name":"大石 昌嗣"},{"name":"Tanida Hajime"},{"name":"Uruga Tomoya"},{"name":"Arai Hajime"},{"name":"Uchimoto Yoshiharu"},{"name":"Ogumi Zempachi"}]},"publication_date":"2011","publication_name":{"en":"The Journal of Physical Chemistry Letters","ja":"The Journal of Physical Chemistry Letters"},"volume":"Vol.2","number":"No.20","starting_page":"2511","ending_page":"2514","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1021/jz2011226"],"issn":["1948-7185"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:45, {"insert":{"user_id":"7000009000","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-80051936517&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=312566","label":"url"}],"paper_title":{"en":"X-ray Absorption Spectroscopic Study on La0.6Sr0.4CoO3-δ Cathode Materials Related with Oxygen Vacancy Formation","ja":"X-ray Absorption Spectroscopic Study on La0.6Sr0.4CoO3-δ Cathode Materials Related with Oxygen Vacancy Formation"},"authors":{"en":[{"name":"Orikasa Yuki"},{"name":"Ina Toshiaki"},{"name":"Nakao Takayuki"},{"name":"Mineshige Atsushi"},{"name":"Amezawa Koji"},{"name":"Oishi Masatsugu"},{"name":"Arai Hajime"},{"name":"Ogumi Zempachi"},{"name":"Uchimoto Yoshiharu"}],"ja":[{"name":"Orikasa Yuki"},{"name":"Ina Toshiaki"},{"name":"Nakao Takayuki"},{"name":"Mineshige Atsushi"},{"name":"Amezawa Koji"},{"name":"大石 昌嗣"},{"name":"Arai Hajime"},{"name":"Ogumi Zempachi"},{"name":"Uchimoto Yoshiharu"}]},"publication_date":"2011","publication_name":{"en":"The Journal of Physical Chemistry C","ja":"The Journal of Physical Chemistry C"},"volume":"Vol.115","number":"No.33","starting_page":"16433","ending_page":"16438","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1021/jp2029642"],"issn":["1932-7447"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:46, {"insert":{"user_id":"7000009000","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-80052305102&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=312565","label":"url"}],"paper_title":{"en":"Local structural analysis for oxide ion transport in La0.6Sr0.4FeO3-δ Cathodes","ja":"Local structural analysis for oxide ion transport in La0.6Sr0.4FeO3-δ Cathodes"},"authors":{"en":[{"name":"Orikasa Yuki"},{"name":"Nakao Takayuki"},{"name":"Oishi Masatsugu"},{"name":"Ina Toshiaki"},{"name":"Mineshige Atsushi"},{"name":"Amezawa Koji"},{"name":"Arai Hajime"},{"name":"Ogumi Zempachi"},{"name":"Uchimoto Yoshiharu"}],"ja":[{"name":"Orikasa Yuki"},{"name":"Nakao Takayuki"},{"name":"大石 昌嗣"},{"name":"Ina Toshiaki"},{"name":"Mineshige Atsushi"},{"name":"Amezawa Koji"},{"name":"Arai Hajime"},{"name":"Ogumi Zempachi"},{"name":"Uchimoto Yoshiharu"}]},"publication_date":"2011","publication_name":{"en":"Journal of Materials Chemistry","ja":"Journal of Materials Chemistry"},"volume":"Vol.21","starting_page":"14013","ending_page":"14019","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1039/c1jm11358e"],"issn":["0959-9428"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
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line:48, {"insert":{"user_id":"7000009000","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=312570","label":"url"}],"paper_title":{"en":"Defect structure analysis of proton-oxide ion mixed conductor BaCe0.9Nd0.1O3 - δ","ja":"Defect structure analysis of proton-oxide ion mixed conductor BaCe0.9Nd0.1O3 - δ"},"authors":{"en":[{"name":"Oishi Masatsugu"},{"name":"Akoshima Satoshi"},{"name":"Yashiro Keiji"},{"name":"Sato Kazuhisa"},{"name":"Kawada Tatsuya"},{"name":"Mizusaki Junichiro"}],"ja":[{"name":"大石 昌嗣"},{"name":"Akoshima Satoshi"},{"name":"Yashiro Keiji"},{"name":"Sato Kazuhisa"},{"name":"Kawada Tatsuya"},{"name":"Mizusaki Junichiro"}]},"publication_date":"2010","publication_name":{"en":"Solid State Ionics","ja":"Solid State Ionics"},"volume":"Vol.181","number":"No.29-30","starting_page":"1336","ending_page":"1343","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1016/j.ssi.2010.07.034"],"issn":["0167-2738"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:49, {"insert":{"user_id":"7000009000","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=312569","label":"url"}],"paper_title":{"en":"Reaction kinetics on platinum electrode / yttrium-doped barium cerate interface under H2H2O atmosphere","ja":"Reaction kinetics on platinum electrode / yttrium-doped barium cerate interface under H2H2O atmosphere"},"authors":{"en":[{"name":"Akoshima Satoshi"},{"name":"Oishi Masatsugu"},{"name":"Yashiro Keiji"},{"name":"Sato Kazuhisa"},{"name":"Mizusaki Junichiro"}],"ja":[{"name":"Akoshima Satoshi"},{"name":"大石 昌嗣"},{"name":"Yashiro Keiji"},{"name":"Sato Kazuhisa"},{"name":"Mizusaki Junichiro"}]},"publication_date":"2010","publication_name":{"en":"Solid State Ionics","ja":"Solid State Ionics"},"volume":"Vol.181","number":"No.3-4","starting_page":"240","ending_page":"248","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1016/j.ssi.2009.05.003"],"issn":["0167-2738"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:50, {"insert":{"user_id":"7000009000","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=312571","label":"url"}],"paper_title":{"en":"Defect structure analysis of B-site doped perovskite-type proton conducting oxide BaCeO3 Part 1: The defect concentration of BaCe0.9M0.1O3-δ (M = Y and Yb)","ja":"Defect structure analysis of B-site doped perovskite-type proton conducting oxide BaCeO3 Part 1: The defect concentration of BaCe0.9M0.1O3-δ (M = Y and Yb)"},"authors":{"en":[{"name":"Oishi Masatsugu"},{"name":"Akoshima Satoshi"},{"name":"Yashiro Keiji"},{"name":"Sato Kazuhisa"},{"name":"Mizusaki Junichiro"},{"name":"Kawada Tatsuya"}],"ja":[{"name":"大石 昌嗣"},{"name":"Akoshima Satoshi"},{"name":"Yashiro Keiji"},{"name":"Sato Kazuhisa"},{"name":"Mizusaki Junichiro"},{"name":"Kawada Tatsuya"}]},"publication_date":"2009","publication_name":{"en":"Solid State Ionics","ja":"Solid State Ionics"},"volume":"Vol.180","number":"No.2-3","starting_page":"127","ending_page":"131","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1016/j.ssi.2008.12.025"],"issn":["0167-2738"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
line:51, {"insert":{"user_id":"7000009000","type":"published_papers"},"similar_merge":{"see_also":[{"@id":"https://www.scopus.com/record/display.url?eid=2-s2.0-56949098148&origin=inward","label":"url"},{"@id":"https://web.db.tokushima-u.ac.jp/cgi-bin/edb_browse?EID=312574","label":"url"}],"paper_title":{"en":"Defect structure analysis of B-site doped perovskite-type proton conducting oxide BaCeO3: Part 2: The electrical conductivity and diffusion coefficient of BaCe0.9Y0.1O3-δ","ja":"Defect structure analysis of B-site doped perovskite-type proton conducting oxide BaCeO3: Part 2: The electrical conductivity and diffusion coefficient of BaCe0.9Y0.1O3-δ"},"authors":{"en":[{"name":"Oishi Masatsugu"},{"name":"Akoshima Satoshi"},{"name":"Yashiro Keiji"},{"name":"Sato Kazuhisa"},{"name":"Mizusaki Junichiro"},{"name":"Kawada Tatsuya"}],"ja":[{"name":"大石 昌嗣"},{"name":"Akoshima Satoshi"},{"name":"Yashiro Keiji"},{"name":"Sato Kazuhisa"},{"name":"Mizusaki Junichiro"},{"name":"Kawada Tatsuya"}]},"publication_date":"2008","publication_name":{"en":"Solid State Ionics","ja":"Solid State Ionics"},"volume":"Vol.179","number":"No.39","starting_page":"2240","ending_page":"2247","languages":["eng"],"referee":true,"identifiers":{"doi":["10.1016/j.ssi.2008.08.005"],"issn":["0167-2738"]},"published_paper_type":"scientific_journal"},"priority":"input_data"}
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